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Title: Method for reprocessing and separating spent nuclear fuels

Patent ·
OSTI ID:864669

Spent nuclear fuels, including actinide fuels, volatile and non-volatile fission products, are reprocessed and separated in a molten metal solvent housed in a separation vessel made of a carbon-containing material. A first catalyst, which promotes the solubility and permeability of carbon in the metal solvent, is included. By increasing the solubility and permeability of the carbon in the solvent, the rate at which actinide oxides are reduced (carbothermic reduction) is greatly increased. A second catalyst, included to increase the affinity for nitrogen in the metal solvent, is added to increase the rate at which actinide nitrides form after carbothermic reduction is complete.

Research Organization:
Lawrence Livermore National Laboratory (LLNL), Livermore, CA (United States)
DOE Contract Number:
W-7405-ENG-48
Assignee:
Krikorian, Oscar H. (Danville, CA);Grens, John Z. (Livermore, CA);Parrish, Sr., William H. (Walnut Creek, CA)
Patent Number(s):
US 4399108
OSTI ID:
864669
Country of Publication:
United States
Language:
English