Global Chemical Composition of Ambient Fine Particulate Matter for Exposure Assessment

Philip, Sajeev; Martin, Randall V.; van Donkelaar, Aaron; Lo, Jason Wai-Ho; Wang, Yuxuan; Chen, Dan; Zhang, Lin; Kasibhatla, Prasad S.; Wang, Siwen; Zhang, Qiang; Lu, Zifeng; Streets, David G.; Bittman, Shabtai; Macdonald, Douglas J.

doi:10.1021/es502965b

Title: Global Chemical Composition of Ambient Fine Particulate Matter for Exposure Assessment

Journal Article · Fri Oct 24 00:00:00 EDT 2014 · Environmental Science and Technology

DOI:https://doi.org/10.1021/es502965b· OSTI ID:1261137

Philip, Sajeev ^[1]; Martin, Randall V. ^[2]; van Donkelaar, Aaron ^[1]; Lo, Jason Wai-Ho ^[1]; Wang, Yuxuan ^[3]; Chen, Dan ^[4]; Zhang, Lin ^[5]; Kasibhatla, Prasad S. ^[6]; Wang, Siwen ^[7]; Zhang, Qiang ^[8]; Lu, Zifeng ^[9]; Streets, David G. ^[9]; Bittman, Shabtai ^[10]; Macdonald, Douglas J. ^[11]

Dalhousie Univ., Halifax, NS (Canada). Dept. of Physics and Atmospheric Science
Dalhousie Univ., Halifax, NS (Canada). Dept. of Physics and Atmospheric Science; Harvard-Smithsonian Center for Astrophysics, Cambridge, MA (United States)
Tsinghua Univ., Beijing (China). Ministry of Education Key Lab. for Earth System Modeling
Univ. of California, Los Angeles, CA (United States). Dept. of Atmospheric and Oceanic Sciences
Peking Univ., Beijing (China). Dept. of Atmospheric and Oceanic Sciences, School of Physics
Duke Univ., Durham, NC (United States). Nicholas School of the Environment and Earth Sciences
Tsinghua Univ., Beijing (China). State Key Joint Lab. of Environment Simulation and Pollution Control
Tsinghua Univ., Beijing (China). Center for Earth System Science
Argonne National Lab. (ANL), Argonne, IL (United States). Decision and Information Sciences Division
Agriculture and Agri-Food Canada, Agassiz, BC (Canada)
Environment Canada, Gatineau, QC (Canada)

Epidemiologic and health impact studies are inhibited by the paucity of global, long-term measurements of the chemical composition of fine particulate matter. We inferred PM_2.5 chemical composition at 0.1° × 0.1° spatial resolution for 2004–2008 by combining aerosol optical depth retrieved from the MODIS and MISR satellite instruments, with coincident profile and composition information from the GEOS-Chem global chemical transport model. Evaluation of the satellite-model PM_2.5 composition data set with North American in situ measurements indicated significant spatial agreement for secondary inorganic aerosol, particulate organic mass, black carbon, mineral dust, and sea salt. We found that global population-weighted PM_2.5 concentrations were dominated by particulate organic mass (11.9 ± 7.3 μg/m³), secondary inorganic aerosol (11.1 ± 5.0 μg/m³), and mineral dust (11.1 ± 7.9 μg/m³). Secondary inorganic PM_2.5 concentrations exceeded 30 μg/m³ over East China. Sensitivity simulations suggested that population-weighted ambient PM_2.5 from biofuel burning (11 μg/m³) could be almost as large as from fossil fuel combustion sources (17 μg/m³). In conclusion, these estimates offer information about global population exposure to the chemical components and sources of PM_2.5.

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Research Organization:: Argonne National Laboratory (ANL), Argonne, IL (United States)

Sponsoring Organization:: USDOE; Natural Sciences and Engineering Research Council of Canada (NSERC); U.S. National Inst. of Health (NIH)

OSTI ID:: 1261137

Journal Information:: Environmental Science and Technology, Vol. 48, Issue 22; ISSN 0013-936X

Publisher:: American Chemical Society (ACS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 138 works

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