Lithium-coated polymeric matrix as a minimum volume-change and dendrite-free lithium metal anode

Liu, Yayuan; Lin, Dingchang; Liang, Zheng; Zhao, Jie; Yan, Kai; Cui, Yi

doi:10.1038/ncomms10992

Title: Lithium-coated polymeric matrix as a minimum volume-change and dendrite-free lithium metal anode

Journal Article · Fri Mar 18 00:00:00 EDT 2016 · Nature Communications

DOI:https://doi.org/10.1038/ncomms10992· OSTI ID:1256050

Liu, Yayuan ^[1]; Lin, Dingchang ^[1]; Liang, Zheng ^[1]; Zhao, Jie ^[1]; Yan, Kai ^[1]; Cui, Yi ^[2]

Stanford Univ., Stanford, CA (United States)
Stanford Univ., Stanford, CA (United States); SLAC National Accelerator Lab., Menlo Park, CA (United States)

Lithium metal is the ideal anode for the next generation of high-energy-density batteries. Nevertheless, dendrite growth, side reactions and infinite relative volume change have prevented it from practical applications. Here, we demonstrate a promising metallic lithium anode design by infusing molten lithium into a polymeric matrix. The electrospun polyimide employed is stable against highly reactive molten lithium and, via a conformal layer of zinc oxide coating to render the surface lithiophilic, molten lithium can be drawn into the matrix, affording a nano-porous lithium electrode. Importantly, the polymeric backbone enables uniform lithium stripping/plating, which successfully confines lithium within the matrix, realizing minimum volume change and effective dendrite suppression. The porous electrode reduces the effective current density; thus, flat voltage profiles and stable cycling of more than 100 cycles is achieved even at a high current density of 5 mA cm^-2 in both carbonate and ether electrolyte. Furthermore, the advantages of the porous, polymeric matrix provide important insights into the design principles of lithium metal anodes.

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Research Organization:: SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC)

Grant/Contract Number:: AC02-76SF00515

OSTI ID:: 1256050

Journal Information:: Nature Communications, Vol. 7; ISSN 2041-1723

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 707 works

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Protected Lithium-Metal Anodes in Batteries: From Liquid to Solid Yang, Chunpeng; Fu, Kun; Zhang, Ying Advanced Materials, Vol. 29, Issue 36 https://doi.org/10.1002/adma.201701169	journal	July 2017
Straw-Brick-Like Carbon Fiber Cloth/Lithium Composite Electrode as an Advanced Lithium Metal Anode Liu, Sufu; Xia, Xinhui; Yao, Zhujun Small Methods, Vol. 2, Issue 8 https://doi.org/10.1002/smtd.201800035	journal	April 2018
A collaborative strategy for stable lithium metal anodes by using three-dimensional nitrogen-doped graphene foams Li, Zihao; Li, Xianglong; Zhou, Lu Nanoscale, Vol. 10, Issue 10 https://doi.org/10.1039/c7nr08727f	journal	January 2018
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Tough Gel Electrolyte Using Double Polymer Network Design for the Safe, Stable Cycling of Lithium Metal Anode Wu, Haiping; Cao, Yue; Su, Haiping Angewandte Chemie International Edition, Vol. 57, Issue 5 https://doi.org/10.1002/anie.201709774	journal	January 2018
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Directing lateral growth of lithium dendrites in micro-compartmented anode arrays for safe lithium metal batteries Zou, Peichao; Wang, Yang; Chiang, Sum-Wai Nature Communications, Vol. 9, Issue 1 https://doi.org/10.1038/s41467-018-02888-8	journal	January 2018
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A Hierarchical Silver-Nanowire-Graphene Host Enabling Ultrahigh Rates and Superior Long-Term Cycling of Lithium-Metal Composite Anodes Xue, Pan; Liu, Shuiren; Shi, Xinlei Advanced Materials, Vol. 30, Issue 44 https://doi.org/10.1002/adma.201804165	journal	September 2018
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MXene‐Based Dendrite‐Free Potassium Metal Batteries Tang, Xiao; Zhou, Dong; Li, Peng Advanced Materials, Vol. 32, Issue 4 https://doi.org/10.1002/adma.201906739	journal	November 2019
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Do imaging techniques add real value to the development of better post-Li-ion batteries? Conder, Joanna; Marino, Cyril; Novák, Petr Journal of Materials Chemistry A, Vol. 6, Issue 8 https://doi.org/10.1039/c7ta10622j	journal	January 2018
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N-Doped Graphene Modified 3D Porous Cu Current Collector toward Microscale Homogeneous Li Deposition for Li Metal Anodes Zhang, Rui; Wen, Shuaiwei; Wang, Ning Advanced Energy Materials, Vol. 8, Issue 23 https://doi.org/10.1002/aenm.201800914	journal	May 2018
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Large-scale production of silicon nanoparticles@graphene embedded in nanotubes as ultra-robust battery anodes Wang, Tao; Zhu, Jian; Chen, Yao Journal of Materials Chemistry A, Vol. 5, Issue 10 https://doi.org/10.1039/c6ta10631e	journal	January 2017
More Reliable Lithium-Sulfur Batteries: Status, Solutions and Prospects Fang, Ruopian; Zhao, Shiyong; Sun, Zhenhua Advanced Materials, Vol. 29, Issue 48 https://doi.org/10.1002/adma.201606823	journal	April 2017
Lithiophilic NiO hexagonal plates decorated Ni collector guiding uniform lithium plating for stable lithium metal anode Lu, Weiyi; Wu, Chen; Wei, Weifeng Journal of Materials Chemistry A, Vol. 7, Issue 42 https://doi.org/10.1039/c9ta09396f	journal	January 2019
Mixed Ionic and Electronic Conductor for Li-Metal Anode Protection Yan, Jianhua; Yu, Jianyong; Ding, Bin Advanced Materials, Vol. 30, Issue 7 https://doi.org/10.1002/adma.201705105	journal	January 2018
Hierarchical Co ₃ O ₄ Nanofiber–Carbon Sheet Skeleton with Superior Na/Li‐Philic Property Enabling Highly Stable Alkali Metal Batteries Li, Siyuan; Liu, Qilei; Zhou, Jiajun Advanced Functional Materials, Vol. 29, Issue 19 https://doi.org/10.1002/adfm.201808847	journal	February 2019
Active‐Oxygen‐Enhanced Homogeneous Nucleation of Lithium Metal on Ultrathin Layered Double Hydroxide Li, Zhenhua; Liu, Ke; Fan, Kui Angewandte Chemie International Edition, Vol. 58, Issue 12 https://doi.org/10.1002/anie.201814705	journal	March 2019
Recent advances in cathode materials for rechargeable lithium–sulfur batteries Li, Fang; Liu, Quanhui; Hu, Jiawen Nanoscale, Vol. 11, Issue 33 https://doi.org/10.1039/c9nr04415a	journal	January 2019
Structural Design of Lithium–Sulfur Batteries: From Fundamental Research to Practical Application Yang, Xiaofei; Li, Xia; Adair, Keegan Electrochemical Energy Reviews, Vol. 1, Issue 3 https://doi.org/10.1007/s41918-018-0010-3	journal	June 2018
Columnar Lithium Metal Anodes Zhang, Xue-Qiang; Chen, Xiang; Xu, Rui Angewandte Chemie, Vol. 129, Issue 45 https://doi.org/10.1002/ange.201707093	journal	September 2017
Electrode Edge Effects and the Failure Mechanism of Lithium-Metal Batteries Lee, Hongkyung; Chen, Shuru; Ren, Xiaodi ChemSusChem, Vol. 11, Issue 21 https://doi.org/10.1002/cssc.201801445	journal	October 2018
Active‐Oxygen‐Enhanced Homogeneous Nucleation of Lithium Metal on Ultrathin Layered Double Hydroxide Li, Zhenhua; Liu, Ke; Fan, Kui Angewandte Chemie, Vol. 131, Issue 12 https://doi.org/10.1002/ange.201814705	journal	February 2019
Reviving Lithium-Metal Anodes for Next-Generation High-Energy Batteries Guo, Yanpeng; Li, Huiqiao; Zhai, Tianyou Advanced Materials, Vol. 29, Issue 29 https://doi.org/10.1002/adma.201700007	journal	June 2017
Applications of 2D MXenes in energy conversion and storage systems Pang, Jinbo; Mendes, Rafael G.; Bachmatiuk, Alicja Chemical Society Reviews, Vol. 48, Issue 1 https://doi.org/10.1039/c8cs00324f	journal	January 2019
Mechanistic understanding and strategies to design interfaces of solid electrolytes: insights gained from transmission electron microscopy Hood, Zachary D.; Chi, Miaofang Journal of Materials Science, Vol. 54, Issue 15 https://doi.org/10.1007/s10853-019-03633-2	journal	May 2019
Vertically Aligned Lithiophilic CuO Nanosheets on a Cu Collector to Stabilize Lithium Deposition for Lithium Metal Batteries Zhang, Chen; Lv, Wei; Zhou, Guangmin Advanced Energy Materials, Vol. 8, Issue 21 https://doi.org/10.1002/aenm.201703404	journal	April 2018
Spatial separation of lithiophilic surface and superior conductivity for advanced Li metal anode: the case of acetylene black and N-doped carbon spheres Liang, Feng; Lin, Liangdong; Feng, Zhenyu Journal of Materials Chemistry A, Vol. 7, Issue 15 https://doi.org/10.1039/c9ta00742c	journal	January 2019
A Chemically Engineered Porous Copper Matrix with Cylindrical Core-Shell Skeleton as a Stable Host for Metallic Sodium Anodes Wang, Chuanlong; Wang, Huan; Matios, Edward Advanced Functional Materials, Vol. 28, Issue 30 https://doi.org/10.1002/adfm.201802282	journal	May 2018
Uniform Lithium Nucleation/Growth Induced by Lightweight Nitrogen-Doped Graphitic Carbon Foams for High-Performance Lithium Metal Anodes Liu, Lin; Yin, Ya-Xia; Li, Jin-Yi Advanced Materials, Vol. 30, Issue 10 https://doi.org/10.1002/adma.201706216	journal	January 2018
Implanting CNT Forest onto Carbon Nanosheets as Multifunctional Hosts for High-Performance Lithium Metal Batteries Zhao, Changtai; Wang, Zhao; Tan, Xinyi Small Methods, Vol. 3, Issue 5 https://doi.org/10.1002/smtd.201800546	journal	February 2019

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