Excitations in a Four-Leg Antiferromagnetic Heisenberg Spin Tube,
Journal Article
·
· Physical Review Letters
- ORNL
- French Atomic Energy Commission (CEA), Grenoble
- National Institute of Standards and Technology (NIST)
- Institut Laue-Langevin (ILL)
- Hahn-Meitner Institut, Berlin, Germany
Inelastic neutron scattering is used to investigate magnetic excitations in the quasi-one-dimensional quantum spin-liquid system Cu2Cl4 D8C4SO2. Contrary to previously conjectured models that relied on bond-alternating nearest-neighbor interactions in the spin chains, the dominant interactions are actually next-nearest-neighbor in-chain antiferromagnetic couplings. The appropriate Heisenberg Hamiltonian is equivalent to that of a S 1=2 4-leg spin-tube with almost perfect one dimensionality and no bond alternation. A partial geometric frustration of rung interactions induces a small incommensurability of short-range spin correlations.
- Research Organization:
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). High Flux Isotope Reactor (HFIR)
- Sponsoring Organization:
- USDOE Office of Science (SC)
- DOE Contract Number:
- DE-AC05-00OR22725
- OSTI ID:
- 968280
- Journal Information:
- Physical Review Letters, Vol. 100, Issue 3
- Country of Publication:
- United States
- Language:
- English
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