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Title: Pulse-fluence-specified optimal control simulation with applications to molecular orientation and spin-isomer-selective molecular alignment

We propose an optimal control simulation with specified pulse fluence and amplitude. The simulation is applied to the orientation control of CO molecules to examine the optimal combination of THz and laser pulses, and to discriminate nuclear-spin isomers of {sup 14}N{sub 2} as spatially anisotropic distributions.
Authors:
; ;  [1]
  1. Department of Chemistry, Graduate School of Science, Tohoku University 6-3 Aza-Aoba, Aramaki, Aoba-ku, Sendai 980-8578 (Japan)
Publication Date:
OSTI Identifier:
22499149
Resource Type:
Journal Article
Resource Relation:
Journal Name: AIP Conference Proceedings; Journal Volume: 1702; Journal Issue: 1; Conference: ICCMSE 2015: International conference of computational methods in sciences and engineering 2015, Athens (Greece), 20-23 Mar 2015; Other Information: (c) 2015 AIP Publishing LLC; Country of input: International Atomic Energy Agency (IAEA)
Country of Publication:
United States
Language:
English
Subject:
71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS; ALIGNMENT; AMPLITUDES; ANISOTROPY; CARBON MONOXIDE; DISTRIBUTION; ISOMERS; LASER RADIATION; MOLECULES; NITROGEN 14; OPTIMAL CONTROL; PULSES; SIMULATION; SPIN