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Title: Application of an Online-Coupled Regional Climate Model, WRF-CAM5, over East Asia for Examination of Ice Nucleation Schemes: Part I. Comprehensive Model Evaluation and Trend Analysis for 2006 and 2011

Journal Article · · Climate
DOI:https://doi.org/10.3390/cli3030627· OSTI ID:1344065

Online-coupled climate and chemistry models are necessary to realistically represent the interactions between climate variables and chemical species and accurately simulate aerosol direct and indirect effects on cloud, precipitation, and radiation. In this Part I of a two-part paper, simulations from the Weather Research and Forecasting model coupled with the physics package of Community Atmosphere Model (WRF-CAM5) are conducted with the default heterogeneous ice nucleation parameterization over East Asia for two full years: 2006 and 2011. A comprehensive model evaluation is performed using satellite and surface observations. The model shows an overall acceptable performance for major meteorological variables at the surface and in the boundary layer, as well as column variables (e.g., precipitation, cloud fraction, precipitating water vapor, downward longwave and shortwave radiation). Moderate to large biases exist for cloud condensation nuclei over oceanic areas, cloud variables (e.g., cloud droplet number concentration, cloud liquid and ice water paths, cloud optical depth, longwave and shortwave cloud forcing). These biases indicate a need to improve the model treatments for cloud processes, especially cloud droplets and ice nucleation, as well as to reduce uncertainty in the satellite retrievals. The model simulates well the column abundances of chemical species except for column SO2 but relatively poor for surface concentrations of several species such as CO, NO2, SO2, PM2.5, and PM10. Several reasons could contribute to the underestimation of major chemical species in East Asia including underestimations of anthropogenic emissions and natural dust emissions, uncertainties in the spatial and vertical distributions of the anthropogenic emissions, as well as biases in meteorological, radiative, and cloud predictions. Despite moderate to large biases in the chemical predictions, the model performance is generally consistent with or even better than that reported for East Asia with only a few exceptions. The model generally reproduces the observed seasonal variations and the difference between 2006 and 2011 for most variables or chemical species. Overall, these results demonstrate promising skills of WRF-CAM5 for long-term simulations at a regional scale and suggest several areas of potential improvements.

Research Organization:
Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)
Sponsoring Organization:
USDOE
DOE Contract Number:
AC05-76RL01830
OSTI ID:
1344065
Report Number(s):
PNNL-SA-113254; CLIMC9; KP1703010
Journal Information:
Climate, Vol. 3, Issue 3; ISSN 2225-1154
Publisher:
MDPI
Country of Publication:
United States
Language:
English

References (62)

Online-coupled meteorology and chemistry models: history, current status, and outlook journal January 2008
Integrated modeling for forecasting weather and air quality: A call for fully coupled approaches journal December 2011
A review of operational, regional-scale, chemical weather forecasting models in Europe journal January 2012
Online coupled regional meteorology chemistry models in Europe: current status and prospects journal January 2014
Fully coupled “online” chemistry within the WRF model journal December 2005
Assessing the CAM5 physics suite in the WRF-Chem model: implementation, resolution sensitivity, and a first evaluation for a regional case study journal January 2014
Investigation of aerosol indirect effects using a cumulus microphysics parameterization in a regional climate model: INVESTIGATION OF AIE ON REGIONAL CLIMATE journal January 2014
Toward a minimal representation of aerosols in climate models: description and evaluation in the Community Atmosphere Model CAM5 journal January 2012
New Primary Ice-Nucleation Parameterizations in an Explicit Cloud Model journal July 1992
A Particle-Surface-Area-Based Parameterization of Immersion Freezing on Desert Dust Particles journal October 2012
Improvements to an Empirical Parameterization of Heterogeneous Ice Nucleation and Its Comparison with Observations journal February 2013
Integrating laboratory and field data to quantify the immersion freezing ice nucleation activity of mineral dust particles journal January 2015
Air pollution and its control in China journal May 2007
Radiative transfer for inhomogeneous atmospheres: RRTM, a validated correlated-k model for the longwave journal July 1997
Radiative forcing by long-lived greenhouse gases: Calculations with the AER radiative transfer models journal January 2008
A New Moist Turbulence Parameterization in the Community Atmosphere Model journal June 2009
Sensitivity of climate simulations to the parameterization of cumulus convection in the Canadian climate centre general circulation model journal September 1995
Microphysics parameterization for convective clouds in a global climate model: Description and single-column model tests journal January 2011
A New Two-Moment Bulk Stratiform Cloud Microphysics Scheme in the Community Atmosphere Model, Version 3 (CAM3). Part I: Description and Numerical Tests journal August 2008
Photodissociation in the atmosphere: 1. Actinic flux and the effects of ground reflections and clouds journal January 1987
Effect of clouds on photolysis and oxidants in the troposphere journal January 2003
Uncertainties in global aerosol simulations: Assessment using three meteorological data sets journal January 2007
The formation of atmospheric ice crystals by the freezing of droplets journal October 1953
The Role of Contact Nucleation in Ice Phase Initiation in Clouds journal April 1974
A new lumped structure photochemical mechanism for large-scale applications journal December 1999
Sulfur chemistry in the National Center for Atmospheric Research Community Climate Model: Description, evaluation, features, and sensitivity to aqueous chemistry journal January 2000
Models‐3 Community Multiscale Air Quality (CMAQ) model aerosol component 1. Model description journal March 2003
Asian emissions in 2006 for the NASA INTEX-B mission journal January 2009
Estimates of global terrestrial isoprene emissions using MEGAN (Model of Emissions of Gases and Aerosols from Nature) journal January 2006
Mineral Dust Entrainment and Deposition (DEAD) model: Description and 1990s dust climatology journal January 2003
Implementation of dust emission and chemistry into the Community Multiscale Air Quality modeling system and initial application to an Asian dust storm episode journal January 2012
Canadian Aerosol Module (CAM): A size-segregated simulation of atmospheric aerosol processes for climate and air quality models 2. Global sea-salt aerosol and its budgets journal January 2002
Concentration and chemical characteristics of PM2.5 in Beijing, China: 2001–2002 journal February 2006
Impact of gas-phase mechanisms on Weather Research Forecasting Model with Chemistry (WRF/Chem) predictions: Mechanism implementation and comparative evaluation: IMPACT OF GAS-PHASE MECHANISMS journal January 2012
Evaluation of ERA-40, NCEP-1, and NCEP-2 reanalysis air temperatures with ground-based measurements in China journal January 2008
Application of MM5 in China: Model evaluation, seasonal variations, and sensitivity to horizontal grid resolutions journal June 2011
Incorporation of new particle formation and early growth treatments into WRF/Chem: Model improvement, evaluation, and impacts of anthropogenic aerosols over East Asia journal January 2016
Regional modeling of secondary organic aerosol over China using WRF/Chem journal January 2012
Impacts of different urban canopy schemes in WRF/Chem on regional climate and air quality in Yangtze River Delta, China journal August 2014
Comparative analysis of meteorological performance of coupled chemistry-meteorology models in the context of AQMEII phase 2 journal August 2015
Development and initial application of the global-through-urban weather research and forecasting model with chemistry (GU-WRF/Chem): THE GLOBAL-THROUGH-URBAN WRF/CHEM journal October 2012
Application of WRF/Chem-MADRID and WRF/Polyphemus in Europe – Part 1: Model description, evaluation of meteorological predictions, and aerosol–meteorology interactions journal January 2013
Application of Weather Research and Forecasting Model with Chemistry (WRF/Chem) over northern China: Sensitivity study, comparative evaluation, and policy implications journal January 2016
Application of online-coupled WRF/Chem-MADRID in East Asia: Model evaluation and climatic effects of anthropogenic aerosols journal January 2016
Incorporating an advanced aerosol activation parameterization into WRF-CAM5: Model evaluation and parameterization intercomparison: An Advanced Aerosol Activation Scheme journal July 2015
Introducing subgrid‐scale cloud feedbacks to radiation for regional meteorological and climate modeling journal December 2012
Incorporation of advanced aerosol activation treatments into CESM/CAM5: model evaluation and impacts on aerosol indirect effects journal January 2014
Seasonal and monthly variations of columnar aerosol optical properties over east Asia determined from multi-year MODIS, LIDAR, and AERONET Sun/sky radiometer measurements journal March 2007
WRF-Chem simulations of aerosols and anthropogenic aerosol radiative forcing in East Asia journal August 2014
A parameterization of sea-salt aerosol source function for sub- and super-micron particles: SEA-SALT AEROSOL PRODUCTION journal October 2003
Characterization of soil dust aerosol in China and its transport and distribution during 2001 ACE-Asia: 1. Network observations: SOIL DUST AEROSOL IN CHINA, 1 journal May 2003
Understanding of regional air pollution over China using CMAQ, part II. Process analysis and sensitivity of ozone and particulate matter to precursor emissions journal September 2010
Biomass burning in Asia: Annual and seasonal estimates and atmospheric emissions journal October 2003
Retrieval of vertical columns of sulfur dioxide from SCIAMACHY and OMI: Air mass factor algorithm development, validation, and error analysis journal January 2009
Twelve years of global observations of formaldehyde in the troposphere using GOME and SCIAMACHY sensors journal January 2008
Emission inventory and trends of NO x for China, 2000–2020 journal June 2014
Sulfate-nitrate-ammonium aerosols over China: response to 2000–2015 emission changes of sulfur dioxide, nitrogen oxides, and ammonia journal January 2013
Impact of aerosol size representation on modeling aerosol-cloud interactions: AEROSOL SIZE REPRESENTATION journal November 2002
A parameterization of aerosol activation 3. Sectional representation journal January 2002
Global assessment of marine boundary layer cloud droplet number concentration from satellite journal January 2007
Global assessment of AMSR-E and MODIS cloud liquid water path retrievals in warm oceanic clouds journal January 2010
Stationary and time periodic patterns of two-predator and one-prey systems with prey-taxis preprint January 2015

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