Resonantly enhanced second-harmonic generation using III–V semiconductor all-dielectric metasurfaces

Liu, Sheng; Sinclair, Michael B.; Saravi, Sina; Keeler, Gordon A.; Yang, Yuanmu; Reno, John; Peake, Gregory M.; Setzpfandt, Frank; Staude, Isabelle; Pertsch, Thomas; Brener, Igal

doi:10.1021/acs.nanolett.6b01816

Title: Resonantly enhanced second-harmonic generation using III–V semiconductor all-dielectric metasurfaces

Journal Article · Mon Aug 08 00:00:00 EDT 2016 · Nano Letters

DOI:https://doi.org/10.1021/acs.nanolett.6b01816· OSTI ID:1326369

Liu, Sheng ^[1]; Sinclair, Michael B. ^[1]; Saravi, Sina ^[2]; Keeler, Gordon A. ^[1]; Yang, Yuanmu ^[1]; Reno, John ^[1]; Peake, Gregory M. ^[1]; Setzpfandt, Frank ^[2]; Staude, Isabelle ^[2]; Pertsch, Thomas ^[2]; Brener, Igal ^[1]

Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
Friedrich-Schiller-Univ. Jena, Jena (Germany)

Nonlinear optical phenomena in nanostructured materials have been challenging our perceptions of nonlinear optical processes that have been explored since the invention of lasers. For example, the ability to control optical field confinement, enhancement, and scattering almost independently allows nonlinear frequency conversion efficiencies to be enhanced by many orders of magnitude compared to bulk materials. Also, the subwavelength length scale renders phase matching issues irrelevant. Compared with plasmonic nanostructures, dielectric resonator metamaterials show great promise for enhanced nonlinear optical processes due to their larger mode volumes. Here, we present, for the first time, resonantly enhanced second-harmonic generation (SHG) using gallium arsenide (GaAs) based dielectric metasurfaces. Using arrays of cylindrical resonators we observe SHG enhancement factors as large as 10⁴ relative to unpatterned GaAs. At the magnetic dipole resonance, we measure an absolute nonlinear conversion efficiency of ~2 × 10^–5 with ~3.4 GW/cm² pump intensity. In conclusion, the polarization properties of the SHG reveal that both bulk and surface nonlinearities play important roles in the observed nonlinear process.

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Research Organization:: Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC04-94AL85000

OSTI ID:: 1326369

Report Number(s):: SAND-2016-9155J; 647439

Journal Information:: Nano Letters, Vol. 16, Issue 9; ISSN 1530-6984

Publisher:: American Chemical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 286 works

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Inverse-designed photonic fibers and metasurfaces for nonlinear frequency conversion [Invited] Sitawarin, Chawin; Jin, Weiliang; Lin, Zin Photonics Research, Vol. 6, Issue 5 https://doi.org/10.1364/prj.6.000b82	journal	January 2018
Numerical Study on Mie Resonances in Single GaAs Nanomembranes Raya, Andrés M.; Fuster, David; Llorens, José M. Nanomaterials, Vol. 9, Issue 6 https://doi.org/10.3390/nano9060856	journal	June 2019
Degenerate optical nonlinear enhancement in epsilon-near-zero transparent conducting oxides Carnemolla, Enrico Giuseppe; Caspani, Lucia; DeVault, Clayton Optical Materials Express, Vol. 8, Issue 11 https://doi.org/10.1364/ome.8.003392	journal	January 2018
Revealing Low-Radiative Modes of Nanoresonators with Internal Raman Scattering Baryshnikova, K. V.; Frizyuk, K.; Zograf, G. ПИСЬМА В ЖУРНАЛ ЭКСПЕРИМЕНТАЛЬНОЙ И ТЕОРЕТИЧЕСКОЙ ФИЗИКИ, Vol. 110, Issue 1(7) https://doi.org/10.1134/s0370274x19130046	journal	January 2019
Enhanced Nonlinear Yield from Barium Titanate Metasurface Down to the Near Ultraviolet Timpu, Flavia; Reig Escalé, Marc; Timofeeva, Maria ETH Zurich https://doi.org/10.3929/ethz-b-000366859	text	January 2019
MEMS-tunable dielectric metasurface lens Arbabi, Ehsan; Arbabi, Amir; Kamali, Seyedeh Mahsa CLEO: Science and Innovations, Conference on Lasers and Electro-Optics https://doi.org/10.1364/cleo_si.2018.sf1j.2	conference	January 2018
All-dielectric nanophotonics: the quest for better materials and fabrication techniques Baranov, Denis G.; Zuev, Dmitry A.; Lepeshov, Sergey I. arXiv https://doi.org/10.48550/arxiv.1702.00677	preprint	January 2017
Gradient metasurfaces: a review of fundamentals and applications Ding, Fei; Pors, Anders; Bozhevolnyi, Sergey I. arXiv https://doi.org/10.48550/arxiv.1704.03032	text	January 2017
Thermal tuning capabilities of semiconductor metasurface resonators Lewi, Tomer; Butakov, Nikita A.; Schuller, Jon A. arXiv https://doi.org/10.48550/arxiv.1802.09664	preprint	January 2018
Giant nonlinear response at the nanoscale driven by bound states in the continuum Carletti, Luca; Koshelev, Kirill; De Angelis, Costantino arXiv https://doi.org/10.48550/arxiv.1804.02947	text	January 2018
Reconfiguring structured light beams using nonlinear metasurfaces Xu, Yun; Sun, Jingbo; Frantz, Jesse arXiv https://doi.org/10.48550/arxiv.1805.07327	text	January 2018
All-dielectric metasurfaces with trapped modes: group-theoretical description Yu, Pengchao; Kupriianov, Anton S.; Dmitriev, Victor arXiv https://doi.org/10.48550/arxiv.1812.10817	text	January 2018
Coherent Control of the Non-instantaneous Nonlinear Power-law Response in Resonant Nanostructures Bahar, Eyal; Arieli, Uri; Mrejen, Michael arXiv https://doi.org/10.48550/arxiv.1909.06126	text	January 2019
An all-dielectric metasurface as a broadband optical frequency mixer Liu, Sheng; Vabishchevich, Polina P.; Vaskin, Aleksandr Nature Communications, Vol. 9, Issue 1 https://doi.org/10.1038/s41467-018-04944-9	journal	June 2018

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