Homogeneously dispersed multimetal oxygen-evolving catalysts

Zhang, B.; Zheng, X.; Voznyy, O.; Comin, R.; Bajdich, M.; Garcia-Melchor, M.; Han, L.; Xu, J.; Liu, M.; Zheng, L.; Garcia de Arquer, F. P.; Dinh, C. T.; Fan, F.; Yuan, M.; Yassitepe, E.; Chen, N.; Regier, T.; Liu, P.; Li, Y.; De Luna, P.; Janmohamed, A.; Xin, H. L.; Yang, H.; Vojvodic, A.; Sargent, E. H.

doi:10.1126/science.aaf1525

Title: Homogeneously dispersed multimetal oxygen-evolving catalysts

Journal Article · Thu Mar 24 00:00:00 EDT 2016 · Science

DOI:https://doi.org/10.1126/science.aaf1525· OSTI ID:1355859

Zhang, B.; Zheng, X.; Voznyy, O.; Comin, R.; Bajdich, M.; Garcia-Melchor, M.; Han, L.; Xu, J.; Liu, M.; Zheng, L.; Garcia de Arquer, F. P.; Dinh, C. T.; Fan, F.; Yuan, M.; Yassitepe, E.; Chen, N.; Regier, T.; Liu, P.; Li, Y.; De Luna, P. more »

Earth-abundant first-row (3d) transition-metal-based catalysts have been developed for the oxygen-evolution reaction (OER); however, they operate at overpotentials significantly above thermodynamic requirements. Density functional theory suggested that non-3d high-valency metals such as tungsten can modulate 3d metal oxides, providing near-optimal adsorption energies for OER intermediates. We developed a room-temperature synthesis to produce gelled oxy-hydroxide materials with an atomically homogeneous metal distribution. These gelled FeCoW oxy-hydroxide exhibits the lowest overpotential (191 mV) reported at 10 mA per square centimeter in alkaline electrolyte. Here, the catalyst shows no evidence of degradation following more than 500 hours of operation. X-ray absorption and computational studies reveal a synergistic interplay between W, Fe and Co in producing a favorable local coordination environment and electronic structure that enhance the energetics for OER.

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Research Organization:: Brookhaven National Laboratory (BNL), Upton, NY (United States); SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: SC0012704; AC02-76SF00515

OSTI ID:: 1355859

Alternate ID(s):: OSTI ID: 1245398; OSTI ID: 1248381

Report Number(s):: BNL-111992-2016-JA; science.aaf1525

Journal Information:: Science, Journal Name: Science Vol. 352 Journal Issue: 6283; ISSN 0036-8075

Publisher:: American Association for the Advancement of Science (AAAS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 1586 works

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Co–Fe Bimetal Phosphate Composite Loaded on Reduced Graphene Oxide for Oxygen Evolution Zhu, Guoxing; Xie, Xulan; Xiao, Lisong Nano, Vol. 14, Issue 01 https://doi.org/10.1142/s1793292019500036	journal	January 2019
WS(1−x)Sex Nanoparticles Decorated Three-Dimensional Graphene on Nickel Foam: A Robust and Highly Efficient Electrocatalyst for the Hydrogen Evolution Reaction Hussain, Sajjad; Akbar, Kamran; Vikraman, Dhanasekaran Nanomaterials, Vol. 8, Issue 11 https://doi.org/10.3390/nano8110929	journal	November 2018

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