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Title: Aerosol Sample Inhomogeneity with Debris from the Fukushima Daiichi Nuclear Accident

Radionuclide aerosol sampling is a vital component in the detection of nuclear explosions, nuclear accidents, and other radiation releases. This was proven by the detection and tracking of emissions from the Fukushima Daiichi incident across the globe by IMS stations. Two separate aerosol samplers were operated in Richland, WA following the event and debris from the accident were measured at levels well above detection limits. While the atmospheric activity concentration of radionuclides generally compared well between the two stations, they did not agree within uncertainties. This paper includes a detailed study of the aerosol sample homogeneity of 134Cs and 137Cs, then relates it to the overall uncertainty of the original measurement. Our results show that sample inhomogeneity adds an additional 5–10% uncertainty to each aerosol measurement and that this uncertainty is in the same range as the discrepancies between the two aerosol sample measurements from Richland, WA.
Authors:
; ;
Publication Date:
OSTI Identifier:
1214079
Report Number(s):
PNNL-SA-100265
WN0219080
DOE Contract Number:
AC05-76RL01830
Resource Type:
Journal Article
Resource Relation:
Journal Name: Journal of Environmental Radioactivity, 135:1-5
Research Org:
Pacific Northwest National Laboratory (PNNL), Richland, WA (US)
Sponsoring Org:
USDOE
Country of Publication:
United States
Language:
English