Zeolitic Imidazolate Framework Membranes: Novel Synthesis Methods and Progress Toward Industrial Use

Lee, Dennis T.; Corkery, Peter; Park, Sunghwan; Jeong, Hae-Kwon; Tsapatsis, Michael

doi:10.1146/annurev-chembioeng-092320-120148

Title: Zeolitic Imidazolate Framework Membranes: Novel Synthesis Methods and Progress Toward Industrial Use

Journal Article · Wed Apr 13 00:00:00 UTC 2022 · Annual Review of Chemical and Biomolecular Engineering

DOI: https://doi.org/10.1146/annurev-chembioeng-092320-120148 · OSTI ID:2903820

Lee, Dennis T. ^[1]; Corkery, Peter ^[1]; Park, Sunghwan ^[1]; Jeong, Hae-Kwon ^[2]; Tsapatsis, Michael ^[3]

Johns Hopkins University, Baltimore, MD (United States)
Texas A&M University, College Station, TX (United States)
Johns Hopkins University, Baltimore, MD (United States); Johns Hopkins University, Laurel, MD (United States)

In the last decade, zeolitic imidazolate frameworks (ZIFs) have been studied extensively for their potential as selective separation membranes. In this review, we highlight unique structural properties of ZIFs that allow them to achieve certain important separations, like that of propylene from propane, and summarize the state of the art in ZIF thin-film deposition on porous substrates and their modification by postsynthesis treatments. We also review the reported membrane performance for representative membrane synthesis approaches and attempt to rank the synthesis methods with respect to potential for scalability. To compare the dependence of membrane performance on membrane synthesis methods and operating conditions, we map out fluxes and separation factors of selected ZIF-8 membranes for propylene/propane separation. Lastly, we provide future directions considering the importance of further improvements in scalability, cost effectiveness, and stable performance under industrially relevant conditions.

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Research Organization:: The Johns Hopkins University, Baltimore, MD (United States)

Sponsoring Organization:: National Science Foundation (NSF); USDOE Office of Science (SC), Basic Energy Sciences (BES). Chemical Sciences, Geosciences & Biosciences Division (CSGB)

Grant/Contract Number:: SC0021212

OSTI ID:: 2903820

Journal Information:: Annual Review of Chemical and Biomolecular Engineering, Journal Name: Annual Review of Chemical and Biomolecular Engineering Journal Issue: 1 Vol. 13; ISSN 1947-5446; ISSN 1947-5438

Publisher:: Annual ReviewsCopyright Statement

Country of Publication:: United States

Language:: English

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Effect of Temperature on Synthesis of ZIF-8 Membranes for Propylene/propane Separation by Counter Diffusion Method Hara, Nobuo; Yoshimune, Miki; Negishi, Hideyuki Journal of the Japan Petroleum Institute, Vol. 58, Issue 4 https://doi.org/10.1627/jpi.58.237	journal	January 2015
Metal–Organic Framework Membranes: From Fabrication to Gas Separation Shekhah, Osama; Chernikova, Valeriya; Belmabkhout, Youssef Crystals, Vol. 8, Issue 11 https://doi.org/10.3390/cryst8110412	journal	October 2018
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