Chirality-Induced Spin Selectivity in Hybrid Organic-Inorganic Perovskite Semiconductors

Dong, Yifan; Hautzinger, Matthew P.; Haque, Md Azimul; Beard, Matthew C.

doi:10.1146/annurev-physchem-082423-032933

Title: Chirality-Induced Spin Selectivity in Hybrid Organic-Inorganic Perovskite Semiconductors

Journal Article · Fri Feb 14 00:00:00 UTC 2025 · Annual Review of Physical Chemistry

DOI: https://doi.org/10.1146/annurev-physchem-082423-032933 · OSTI ID:2566782

Dong, Yifan; Hautzinger, Matthew P.; Haque, Md Azimul;

The movement of charges through a chiral medium results in a spin-polarized charge current. This phenomenon, known as the chirality-induced spin selectivity (CISS) effect, enables control over spin populations without the need for magnetic components and operates at room temperature. CISS has been discovered in a range of chiral media and most prominently studied in chiral organic molecular species. Chiral hybrid organic-inorganic perovskite semiconductors combine the unique and functional aspects of inorganic semiconductors with chiral molecules. The inorganic component borrows the homochirality of the organic component to yield a unique family of highly tunable chiral semiconductors, where the enantiomeric purity is defined by the organic component. Semiconductors already form the backbone of modern-day technologies. Adding chirality and control over spin through CISS provides new avenues for creative technological development. This review is intended to be an introduction to these unique systems and the demonstrations of CISS and spin control.

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Research Organization:: National Renewable Energy Laboratory (NREL), Golden, CO (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC36-08GO28308

OSTI ID:: 2566782

Report Number(s):: NREL/JA-5F00-90313; MainId:92091; UUID:7aa64814-985f-4ff9-a64a-5e9bbd838c37; MainAdminId:76936

Journal Information:: Annual Review of Physical Chemistry, Journal Name: Annual Review of Physical Chemistry Vol. 76

Country of Publication:: United States

Language:: English

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Title: Chirality-Induced Spin Selectivity in Hybrid Organic-Inorganic Perovskite Semiconductors

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