Palm oil deoxygenation with glycerol as a hydrogen donor for renewable fuel production using nickel-molybdenum catalysts: The effect of support

Hongloi, Nitchakul; Rahman, Tawsif; Feyzbar-Khalkhali-Nejad, Farshad; Prapainainar, Chaiwat; Wongsurakul, Peerawat; Aransiola, Emmanuel; Zhang, Lihua; Bargiela, Pascal; Baltrusaitis, Jonas; Prapainainar, Paweena; Adhikari, Sushil

doi:10.1016/j.fuproc.2025.108196

Title: Palm oil deoxygenation with glycerol as a hydrogen donor for renewable fuel production using nickel-molybdenum catalysts: The effect of support

Journal Article · Fri Feb 28 00:00:00 UTC 2025 · Fuel Processing Technology

DOI: https://doi.org/10.1016/j.fuproc.2025.108196 · OSTI ID:2549235

Hongloi, Nitchakul ^[1];

^[2]; Feyzbar-Khalkhali-Nejad, Farshad ^[2];

^[3];

^[4]; Aransiola, Emmanuel ^[5];

^[6]; Bargiela, Pascal ^[7];

^[5];

^[8];

^[2]

Kasetsart University, Bangkok (Thailand); Auburn University, AL (United States)
Auburn University, AL (United States)
King Mongkut's University of Technology North Bangkok (Thailand)
Silpakorn University, Nakhon Pathom (Thailand)
Lehigh University, Bethlehem, PA (United States)
Brookhaven National Laboratory (BNL), Upton, NY (United States)
Universite de Pau et des Pays de l'Adour (France)
Kasetsart University, Bangkok (Thailand)

Palm oil, one of the most widely used vegetable oils, offers significant potential as a sustainable feedstock for biofuel production. This study explores the deoxygenation of palm oil using glycerol as a hydrogen donor, with nickel-molybdenum (NiMo) catalysts supported on commercial alumina (Al₂O₃), and zeolite (HZSM-5) comparing with self-prepared zirconia (ZrO₂). The catalysts were synthesized via incipient wetness impregnation and evaluated for their performance in biofuel production. NiMo/Al₂O₃ exhibited the lowest oxygen removal efficiency (68.5 %), while NiMo/HZSM-5 achieved a higher oxygen removal (74.3 %) but also demonstrated the highest coke formation. The type of support material influenced the resulting biofuel range, with NiMo/HZSM-5 and NiMo/ZrO₂ favoring jet fuel production, whereas NiMo/Al₂O₃ was more suitable for diesel production. Notably, NiMo/ZrO₂ exhibited the highest performance in palm oil deoxygenation while minimizing coke formation. These findings highlight NiMo/ZrO₂ as a promising catalyst for efficient and stable biofuel production, with the support material significantly influencing product yield and fuel quality.

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Research Organization:: Brookhaven National Laboratory (BNL), Upton, NY (United States)

Sponsoring Organization:: Alabama Agricultural Experiment Station and the Hatch program; Alabama Department of Economic and Community Affairs; Kasetsart University; Office of National Higher Education Science Research and Innovation Policy Counci; USDOE Office of Science (SC), Basic Energy Sciences (BES). Scientific User Facilities (SUF)

Grant/Contract Number:: SC0012704

OSTI ID:: 2549235

Report Number(s):: BNL--227979-2025-JAAM

Journal Information:: Fuel Processing Technology, Journal Name: Fuel Processing Technology Vol. 270; ISSN 0378-3820

Publisher:: ElsevierCopyright Statement

Country of Publication:: United States

Language:: English

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36 MATERIALS SCIENCE
Biofuels
Deoxygenation
Hydrogen donor
NiMo/Al2O3
NiMo/HZSM-5

Title: Palm oil deoxygenation with glycerol as a hydrogen donor for renewable fuel production using nickel-molybdenum catalysts: The effect of support

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