Filament-Induced Failure in Lithium-Reservoir-Free Solid-State Batteries

Park, Se Hwan; Ayyaswamy, Abhinand; Gjerde, Jonathan; Andrews, W. Beck; Vishnugopi, Bairav S.; Drakopoulos, Michael; Vo, Nghia T.; Zhong, Zhong; Thornton, Katsuyo; Mukherjee, Partha P.; Hatzell, Kelsey B.

doi:10.1021/acsenergylett.5c00004

Title: Filament-Induced Failure in Lithium-Reservoir-Free Solid-State Batteries

Journal Article · Sat Feb 22 00:00:00 UTC 2025 · ACS Energy Letters

DOI: https://doi.org/10.1021/acsenergylett.5c00004 · OSTI ID:2531029

;

; Gjerde, Jonathan; Andrews, W. Beck; Vishnugopi, Bairav S.; Drakopoulos, Michael;

; Zhong, Zhong;

; Mukherjee, Partha P.;

Not Available

View Journal Article

Cite

Export

Save

Research Organization:: Brookhaven National Laboratory (BNL), Upton, NY (United States); Princeton University, NJ (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE Office of Science (SC), Basic Energy Sciences (BES). Scientific User Facilities (SUF)

Grant/Contract Number:: SC0012704; SC0023438; SC0023462

OSTI ID:: 2531029

Report Number(s):: BNL--227670-2025-JAAM

Journal Information:: ACS Energy Letters, Journal Name: ACS Energy Letters Journal Issue: 3 Vol. 10; ISSN 2380-8195

Publisher:: American Chemical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

References (41)

Nondestructively Visualizing and Understanding the Mechano‐Electro‐chemical Origins of “Soft Short” and “Creeping” in All‐Solid‐State Batteries Cao, Daxian; Zhang, Kena; Li, Wei Advanced Functional Materials https://doi.org/10.1002/adfm.202307998	journal	September 2023
Designing 3D Anode Based on Pore‐Size‐Dependent Li Deposition Behavior for Reversible Li‐Free All‐Solid‐State Batteries Park, Se Hwan; Jun, Dayoung; Lee, Gyu Hyeon Advanced Science, Vol. 9, Issue 28 https://doi.org/10.1002/advs.202203130	journal	August 2022
Mechanism of Lithium Metal Penetration through Inorganic Solid Electrolytes Porz, Lukas; Swamy, Tushar; Sheldon, Brian W. Advanced Energy Materials, Vol. 7, Issue 20 https://doi.org/10.1002/aenm.201701003	journal	July 2017
Asymmetric Contact Loss Dynamics during Plating and Stripping in Solid‐State Batteries Vishnugopi, Bairav S.; Naik, Kaustubh G.; Kawakami, Hiroki Advanced Energy Materials, Vol. 13, Issue 8 https://doi.org/10.1002/aenm.202203671	journal	December 2022
Operando Investigation on the Role of Densification and Chemo‐Mechanics on Solid‐State Cathodes Jeong, Min‐Gi; Naik, Kaustubh G.; Zheng, Yanjie Advanced Energy Materials, Vol. 14, Issue 23 https://doi.org/10.1002/aenm.202304544	journal	May 2024
Evaluating Pressure‐dependent Discharge Behavior of Foil Versus In situ Plated Lithium Metal Anodes in Solid‐State Batteries Haslam, Catherine G.; Eckhardt, Janis K.; Ayyaswamy, Abhinand Advanced Energy Materials https://doi.org/10.1002/aenm.202403614	journal	November 2024
Lithium Kinetics in Ag–C Porous Interlayer in Reservoir‐Free Solid‐State Batteries Park, Se Hwan; Naik, Kaustubh G.; Vishnugopi, Bairav S. Advanced Energy Materials https://doi.org/10.1002/aenm.202405129	journal	December 2024
Stress Concentration at Notches Savruk, Mykhaylo P.; Kazberuk, Andrzej https://doi.org/10.1007/978-3-319-44555-7	book	January 2017
Stress concentration at slightly undulating surfaces Gao, Huajian Journal of the Mechanics and Physics of Solids, Vol. 39, Issue 4 https://doi.org/10.1016/0022-5096(91)90035-M	journal	January 1991
Mechanical properties of metallic lithium: from nano to bulk scales Fincher, Cole D.; Ojeda, Daniela; Zhang, Yuwei Acta Materialia, Vol. 186 https://doi.org/10.1016/j.actamat.2019.12.036	journal	March 2020
Fracture toughness of porous materials – Experimental methods and data Jelitto, Hans; Schneider, Gerold A. Data in Brief, Vol. 23 https://doi.org/10.1016/j.dib.2019.103709	journal	April 2019
Large-scale automotive battery cell manufacturing: Analyzing strategic and operational effects on manufacturing costs Duffner, Fabian; Mauler, Lukas; Wentker, Marc International Journal of Production Economics, Vol. 232 https://doi.org/10.1016/j.ijpe.2020.107982	journal	February 2021
Characterizing the Li-Solid-Electrolyte Interface Dynamics as a Function of Stack Pressure and Current Density Wang, Michael J.; Choudhury, Rishav; Sakamoto, Jeff Joule, Vol. 3, Issue 9 https://doi.org/10.1016/j.joule.2019.06.017	journal	September 2019
Controlling dendrite propagation in solid-state batteries with engineered stress Fincher, Cole D.; Athanasiou, Christos E.; Gilgenbach, Colin Joule, Vol. 6, Issue 12 https://doi.org/10.1016/j.joule.2022.10.011	journal	December 2022
Structural and electrochemical evolution of alloy interfacial layers in anode-free solid-state batteries Sandoval, Stephanie Elizabeth; Lewis, John A.; Vishnugopi, Bairav S. Joule, Vol. 7, Issue 9 https://doi.org/10.1016/j.joule.2023.07.022	journal	September 2023
Aligning lithium metal battery research and development across academia and industry Hatzell, Kelsey; Chang, Wesley; Bao, Wurigumula Joule, Vol. 8, Issue 6 https://doi.org/10.1016/j.joule.2024.04.007	journal	June 2024
Mechanical behavior of inorganic lithium-conducting solid electrolytes Papakyriakou, Marc; Lu, Mu; Liu, Yuhgene Journal of Power Sources, Vol. 516 https://doi.org/10.1016/j.jpowsour.2021.230672	journal	December 2021
Laplace-Fourier transform solution to the electrochemical kinetics of a symmetric lithium cell affected by interface conformity Zhao, Le; Wang, Q. Jane; Zhang, Xin Journal of Power Sources, Vol. 531 https://doi.org/10.1016/j.jpowsour.2022.231305	journal	May 2022
Li Penetration in Ceramic Solid Electrolytes: Operando Microscopy Analysis of Morphology, Propagation, and Reversibility Kazyak, Eric; Garcia-Mendez, Regina; LePage, William S. Matter, Vol. 2, Issue 4 https://doi.org/10.1016/j.matt.2020.02.008	journal	April 2020
In Situ Investigation of Chemomechanical Effects in Thiophosphate Solid Electrolytes Dixit, Marm B.; Singh, Nikhilendra; Horwath, James P. Matter, Vol. 3, Issue 6 https://doi.org/10.1016/j.matt.2020.09.018	journal	December 2020
Understanding the electro-chemo-mechanics of Li plating in anode-free solid-state batteries with operando 3D microscopy Kazyak, Eric; Wang, Michael J.; Lee, Kiwoong Matter, Vol. 5, Issue 11 https://doi.org/10.1016/j.matt.2022.07.020	journal	November 2022
Operando measurements of dendrite-induced stresses in ceramic electrolytes using photoelasticity Athanasiou, Christos E.; Fincher, Cole D.; Gilgenbach, Colin Matter, Vol. 7, Issue 1 https://doi.org/10.1016/j.matt.2023.10.014	journal	January 2024
Pressure-Driven Interface Evolution in Solid-State Lithium Metal Batteries Zhang, Xin; Wang, Q. Jane; Harrison, Katharine L. Cell Reports Physical Science, Vol. 1, Issue 2 https://doi.org/10.1016/j.xcrp.2019.100012	journal	February 2020
Li6PS5Cl microstructure and influence on dendrite growth in solid-state batteries with lithium metal anode Singh, Dheeraj Kumar; Henss, Anja; Mogwitz, Boris Cell Reports Physical Science, Vol. 3, Issue 9 https://doi.org/10.1016/j.xcrp.2022.101043	journal	September 2022
Scalable Manufacturing of Hybrid Solid Electrolytes with Interface Control Dixit, Marm B.; Zaman, Wahid; Bootwala, Yousuf ACS Applied Materials & Interfaces, Vol. 11, Issue 48 https://doi.org/10.1021/acsami.9b15463	journal	November 2019
Anode-Less or Anode-Free? Hatzell, Kelsey B. ACS Energy Letters, Vol. 8, Issue 11 https://doi.org/10.1021/acsenergylett.3c02163	journal	November 2023
Nonintuitive Role of Solid Electrolyte Porosity on Failure Lin, Lin; Ayyaswamy, Abhinand; Zheng, Yanjie ACS Energy Letters, Vol. 9, Issue 5 https://doi.org/10.1021/acsenergylett.4c00744	journal	April 2024
Challenges in Lithium Metal Anodes for Solid-State Batteries Hatzell, Kelsey B.; Chen, Xi Chelsea; Cobb, Corie L. ACS Energy Letters, Vol. 5, Issue 3 https://doi.org/10.1021/acsenergylett.9b02668	journal	February 2020
Enabling “lithium-free” manufacturing of pure lithium metal solid-state batteries through in situ plating Wang, Michael J.; Carmona, Eric; Gupta, Arushi Nature Communications, Vol. 11, Issue 1 https://doi.org/10.1038/s41467-020-19004-4	journal	October 2020
Effect of pulse-current-based protocols on the lithium dendrite formation and evolution in all-solid-state batteries Reisecker, V.; Flatscher, F.; Porz, L. Nature Communications, Vol. 14, Issue 1 https://doi.org/10.1038/s41467-023-37476-y	journal	April 2023
Processing thin but robust electrolytes for solid-state batteries Balaish, Moran; Gonzalez-Rosillo, Juan Carlos; Kim, Kun Joong Nature Energy, Vol. 6, Issue 3 https://doi.org/10.1038/s41560-020-00759-5	journal	February 2021
Mechanical regulation of lithium intrusion probability in garnet solid electrolytes McConohy, Geoff; Xu, Xin; Cui, Teng Nature Energy, Vol. 8, 241–250 https://doi.org/10.1038/s41560-022-01186-4	journal	January 2023
Challenges in speeding up solid-state battery development Janek, Jürgen; Zeier, Wolfgang G. Nature Energy, Vol. 8, Issue 3 https://doi.org/10.1038/s41560-023-01208-9	journal	February 2023
Critical stripping current leads to dendrite formation on plating in lithium anode solid electrolyte cells Kasemchainan, Jitti; Zekoll, Stefanie; Spencer Jolly, Dominic Nature Materials, Vol. 18, Issue 10 https://doi.org/10.1038/s41563-019-0438-9	journal	July 2019
Electro-chemo-mechanics of anode-free solid-state batteries Sandoval, Stephanie Elizabeth; Haslam, Catherine G.; Vishnugopi, Bairav S. Nature Materials https://doi.org/10.1038/s41563-024-02055-z	journal	January 2025
Dendrite initiation and propagation in lithium metal solid-state batteries Ning, Ziyang; Li, Guanchen; Melvin, Dominic L. R. Nature, Vol. 618, Issue 7964 https://doi.org/10.1038/s41586-023-05970-4	journal	June 2023
Temperature Impact on Lithium Metal Morphology in Lithium Reservoir-Free Solid-State Batteries Jeong, Min-Gi; Hatzell, Kelsey B.; Banerjee, Sourim PRX Energy, Vol. 3, Issue 2 https://doi.org/10.1103/PRXEnergy.3.023003	journal	May 2024
Dependence of Fracture Toughness of Alumina on Grain Size and Test Technique Mussler, Bernhard; Swain, Michael V.; Claussen, Nils Journal of the American Ceramic Society, Vol. 65, Issue 11 https://doi.org/10.1111/j.1151-2916.1982.tb10783.x	journal	November 1982
ACCESS: Advancing Innovation Boerner, Timothy J.; Deems, Stephen; Furlani, Thomas R. Practice and Experience in Advanced Research Computing https://doi.org/10.1145/3569951.3597559	conference	July 2023
“Lithium-Free” Thin-Film Battery with In Situ Plated Li Anode Neudecker, B. J.; Dudney, N. J.; Bates, J. B. Journal of The Electrochemical Society, Vol. 147, Issue 2 https://doi.org/10.1149/1.1393226	journal	January 2000
The Effects of Electric Field Distribution on the Interface Stability in Solid Electrolytes Choudhury, Rishav; Wang, Michael; Sakamoto, Jeff Journal of The Electrochemical Society, Vol. 167, Issue 14 https://doi.org/10.1149/1945-7111/abc034	journal	October 2020

Similar Records

Transition metal oxides as lithium-free cathodes for solid-state lithium metal batteries

Journal Article · Sat Aug 01 00:00:00 UTC 2020 · Nano Energy · OSTI ID:1694286

Wu, Wei; Wang, Man; Wang, Jun; +5 more

Are solid-state batteries safer than lithium-ion batteries?

Journal Article · Fri Apr 01 00:00:00 UTC 2022 · Joule · OSTI ID:1970806

Bates, Alex M.; Preger, Yuliya; Torres-Castro, Loraine; +3 more

Texture Evolution of Plated Lithium in Anode-Free Solid-State Batteries

Journal Article · Thu Jan 29 00:00:00 UTC 2026 · ACS Energy Letters · OSTI ID:3027529

Li, Zhuo; Wu, Daren; Ji, Simon Si Ming; +4 more

Related Subjects

36 MATERIALS SCIENCE
deformation
filaments
lithium
solid electrolytes
stress

Title: Filament-Induced Failure in Lithium-Reservoir-Free Solid-State Batteries

Citation Formats

References (41)

Similar Records

Related Subjects