Structure–Composition Relationships for Mg–Ni and Mg–Fe Olivine

Morfin, Arianna M.; Stanfield, Charles Heath; Murchland, Madeline A.; Bartels, Madeline F.; Nagurney, Alexandra B.; Miller, Quin R.S.; Schaef, Herbert Todd

doi:10.1021/acsearthspacechem.4c00044

Title: Structure–Composition Relationships for Mg–Ni and Mg–Fe Olivine

Journal Article · Tue Aug 20 00:00:00 UTC 2024 · ACS Earth and Space Chemistry

DOI: https://doi.org/10.1021/acsearthspacechem.4c00044 · OSTI ID:2483646

Morfin, Arianna M. ^[1];

^[2]; Murchland, Madeline A. ^[3]; Bartels, Madeline F. ^[4];

^[5];

^[5]

Pacific Northwest National Laboratory (PNNL), Richland, WA (United States); Yakima Valley College, WA (United States)
Pacific Northwest National Laboratory (PNNL), Richland, WA (United States); Univ. of Chicago, IL (United States)
Pacific Northwest National Laboratory (PNNL), Richland, WA (United States); Univ. of Idaho, Moscow, ID (United States)
Pacific Northwest National Laboratory (PNNL), Richland, WA (United States); Yale Univ., New Haven, CT (United States)
Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)

Olivine is a dynamic and important mineral in the crust and mantle with relevance to processes important to climate change technology, such as geologic carbon storage and critical mineral recovery. In this work, we critically evaluated and compiled a new database of olivine diffraction data, lattice parameters, and composition to enable rapid Ni-Mg-Fe olivine composition determination. A compilation of olivine X-ray diffraction data and chemical compositions from both the literature and the International Centre for Diffraction Data (ICDD) powder database was assembled to plot both the forsterite-fayalite and forsterite-liebenbergite solid solution lines. Here we present an expanded dataset to delineate equations and relationships used for quantifying the correlations between olivine lattice parameters and chemical compositions in Mg₂SiO₄-Fe₂SiO₄ (forsterite-fayalite) and Mg₂SiO₄-Ni₂SiO₄ (forsterite-liebenbergite) olivine solid solution series.

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Research Organization:: Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)

Sponsoring Organization:: USDOE Advanced Research Projects Agency - Energy (ARPA-E); USDOE Office of Fossil Energy and Carbon Management (FECM); USDOE Office of Science (SC), Office of Workforce Development for Teachers & Scientists (WDTS)

Grant/Contract Number:: AC05-76RL01830

OSTI ID:: 2483646

Report Number(s):: PNNL-SA--194602

Journal Information:: ACS Earth and Space Chemistry, Journal Name: ACS Earth and Space Chemistry Journal Issue: 9 Vol. 8; ISSN 2472-3452

Publisher:: American Chemical Society (ACS)Copyright Statement

Country of Publication:: United States

Language:: English

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