Ambient Aerosol Is Physically Larger on Cloudy Days in Bondville, Illinois

Flesch, Madison M.; Christiansen, Amy E.; Burns, Alyssa M.; Ghate, Virendra P.; Carlton, Annmarie G.

doi:10.1021/acsearthspacechem.2c00207

Title: Ambient Aerosol Is Physically Larger on Cloudy Days in Bondville, Illinois

Journal Article · Tue Nov 15 04:00:00 UTC 2022 · ACS Earth and Space Chemistry

DOI: https://doi.org/10.1021/acsearthspacechem.2c00207 · OSTI ID:2427957

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Univ. of California, Irvine, CA (United States)
Univ. of California, Irvine, CA (United States); Univ. of Missouri, Kansas City, MO (United States)
Univ. of California, Irvine, CA (United States); Argonne National Laboratory (ANL), Argonne, IL (United States)

Particle chemical composition affects aerosol optical and physical properties in ways important for the fate, transport, and impact of atmospheric particulate matter. For example, hygroscopic constituents take up water to increase the physical size of a particle, which can alter the extinction properties and atmospheric lifetime. At the collocated AERosol RObotic NETwork (AERONET) and Interagency Monitoring of PROtected Visual Environments (IMPROVE) network monitoring stations in rural Bondville, Illinois, we employ a novel cloudiness determination method to compare measured aerosol physicochemical properties on predominantly cloudy and clear sky days from 2010 to 2019. On cloudy days, aerosol optical depth (AOD) is significantly higher than on clear sky days in all seasons. Measured angstrom ngstro''m exponents are significantly smaller on cloudy days, indicating physically larger average particle size for the sampled populations in all seasons except winter. Mass concentrations of fine particulate matter that include estimates of aerosol liquid water (ALW) are higher on cloudy days in all seasons but winter. More ALW on cloudy days is consistent with larger particle sizes inferred from angstrom ngstro''m exponent measurements. Aerosol chemical composition that affects hygroscopicity plays a determining impact on cloudy versus clear sky differences in AOD, angstrom ngstro''m exponents, and ALW. This work highlights the need for simultaneous collocated, high-time-resolution measurements of both aerosol chemical and physical properties, in particular at cloudy times when quantitative understanding of tropospheric composition is most uncertain.

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Research Organization:: Argonne National Laboratory (ANL), Argonne, IL (United States)

Sponsoring Organization:: USDOE; National Aeronautic and Space Administration (NASA); National Science Foundation (NSF)

Grant/Contract Number:: AC02-06CH11357

OSTI ID:: 2427957

Journal Information:: ACS Earth and Space Chemistry, Journal Name: ACS Earth and Space Chemistry Journal Issue: 12 Vol. 6; ISSN 2472-3452

Publisher:: American Chemical Society (ACS)Copyright Statement

Country of Publication:: United States

Language:: English

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54 ENVIRONMENTAL SCIENCES
Angstrom exponent
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aerosol optical depth
clouds
fine particulate matter

Title: Ambient Aerosol Is Physically Larger on Cloudy Days in Bondville, Illinois

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