DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Metal-Encapsulated, Polymer-Containing Halide Salt Composites as Potential Long-Term Hosts for Radioiodine: Evaluating Halmets, Polyhalmets, and Halcermets

Journal Article · · ACS Omega

Not Available

Research Organization:
Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)
Sponsoring Organization:
USDOE; USDOE Laboratory Directed Research and Development (LDRD) Program; USDOE Office of Science (SC), Basic Energy Sciences (BES)
Grant/Contract Number:
AC05-76RL01830
OSTI ID:
2426675
Report Number(s):
PNNL-SA--196206
Journal Information:
ACS Omega, Journal Name: ACS Omega Journal Issue: 32 Vol. 9; ISSN 2470-1343
Publisher:
American Chemical SocietyCopyright Statement
Country of Publication:
United States
Language:
English

References (63)

Review and experimental comparison of the durability of iodine waste forms in semi-dynamic leach testing journal August 2022
Bismuth-based materials for iodine capture and storage: A review journal August 2021
Comprehensive comparison of bismuth and silver functionalized nickel foam composites in capturing radioactive gaseous iodine journal September 2021
Effects of NO2 aging on bismuth nanoparticles and bismuth-loaded silica xerogels for iodine capture journal March 2023
Candidate waste forms for immobilisation of waste chloride salt from pyroprocessing of spent nuclear fuel journal January 2012
Bismuth-embedded SBA-15 mesoporous silica for radioactive iodine capture and stable storage journal October 2015
Materials and processes for the effective capture and immobilization of radioiodine: A review journal March 2016
Glass binder development for a glass-bonded sodalite ceramic waste form journal June 2017
Glass-bonded iodosodalite waste form for immobilization of 129I journal June 2018
Immobilization of iodine via copper iodide journal July 2018
Iodosodalite synthesis with hot isostatic pressing of precursors produced from aqueous and hydrothermal processes journal September 2020
Glass-bonded ceramic waste forms for immobilization of radioiodine from caustic scrubber wastes journal April 2024
Molten salt reactor waste and effluent management strategies: A review journal April 2019
Examining the role of nuclear and renewable energy in reducing carbon footprint: Does the role of technological innovation really create some difference? journal October 2022
Noble gas management with radiation-tolerant MOF for molten salt reactors journal February 2024
Electrochemical Salt Wasteform Development: A Review of Salt Treatment and Immobilization Options journal May 2020
Iodine Vapor Reactions with Pure Metal Wires at Temperatures of 100–139 °C in Air journal November 2021
Iodine Capture by Ag-Loaded Solid Sorbents Followed by Ag Recycling and Iodine Immobilization: An End-to-End Process journal February 2023
Polyacrylonitrile in the Preparation of Separation Membranes: A Review journal April 2023
Densification and Immobilization of AgI-Containing Iodine Waste Forms Using Spark Plasma Sintering journal May 2023
Ceramic–Metal (Cermet) Composites: A Review of Key Properties and Synthesis Methods Focused on Nuclear Waste Immobilization journal March 2024
A Multifunctional Technology Platform for Sorbent Construction Using Polyacrylonitrile Scaffolds journal May 2024
Porous Copper-Loaded Zeolites for High-Efficiency Capture of Iodine from Spent Fuel Reprocessing Off-Gas journal May 2022
Chemical Surface Reactivity and Morphological Changes of Bismuth Triiodide (BiI3) under Different Environmental Conditions journal May 2020
Hybrid Sorbents for 129 I Capture from Contaminated Groundwater journal May 2020
Evaluation of Getter Metals in Na–Al–Si–O Aerogels and Xerogels for the Capture of Iodine Gas journal April 2020
Metal–Organic Framework–Polyacrylonitrile Composite Beads for Xenon Capture journal September 2020
Role of Zeolite Structural Properties toward Iodine Capture: A Head-to-head Evaluation of Framework Type and Chemical Composition journal April 2022
Silver-Loaded Aluminosilicate Aerogels As Iodine Sorbents journal September 2017
Silver-Loaded Xerogel Nanostructures for Iodine Capture: A Comparison of Thiolated versus Unthiolated Sorbents journal June 2022
Polyacrylonitrile Composites of Ag–Al–Si–O Aerogels and Xerogels as Iodine and Iodide Sorbents journal June 2021
Iodine Capture with Metal-Functionalized Polyacrylonitrile Composite Beads Containing Ag0, Bi0, Cu0, or Sn0 Particles journal November 2022
Evaluating the Physisorption and Chemisorption of Iodine on Bismuth-Functionalized Carbon Foams journal August 2022
Iodine Capture with Mechanically Robust Heat-Treated Ag–Al–Si–O Xerogel Sorbents journal April 2021
Concentration-Dependent Mobility, Retardation, and Speciation of Iodine in Surface Sediment from the Savannah River Site journal July 2011
Radioactive Iodine Capture in Silver-Containing Mordenites through Nanoscale Silver Iodide Formation journal July 2010
Thyroid cancer risk in Belarus among children and adolescents exposed to radioiodine after the Chornobyl accident journal November 2010
Thyroid doses for evacuees from the Fukushima nuclear accident journal July 2012
Wet chemical synthesis of apatite-based waste forms – A novel room temperature method for the immobilization of radioactive iodine journal January 2017
Millimeter-sized Bi2S3@polyacrylonitrile hybrid beads for highly efficient iodine capture journal January 2020
Synthesis of and iodine capture with MSx (Ag2S, Bi2S3, Cu2S)–polyacrylonitrile composites journal January 2024
Static iodine loading comparisons between activated carbon, zeolite, alumina, aerogel, and xerogel sorbents journal January 2024
A Simple Model Predicting Iodine Profile in a Packed Bed of Silica-Gel Impregnated with Silver Nitrate journal March 2002
Applicability of a Model Predicting Iodine-129 Profile in a Silver Nitrate Silica-Gel Column for Dissolver Off-Gas Treatment of Fuel Reprocessing journal January 2003
Development of Polymer-Ceramic-Metal Graded Acoustic Matching Layers via Cold Sintering journal April 2022
Low-Temperature Sintering Bi-Si-Zn-Oxide Glasses for Use in Either Glass Composite Materials or Core/Shell 129I Waste Forms: Sintered Glass Iodine-129 Waste Forms journal April 2011
Synthesis and characterization of iodosodalite journal March 2017
The density and interdiffusion coefficients of bismuth-tin melts of eutectic and near-eutectic composition journal April 2010
Treatment of gas-air flows to remove radioiodine using metallic copper journal August 2009
Cold Sintering: Progress, Challenges, and Future Opportunities journal July 2019
Radioactive Iodine and Krypton Control for Nuclear Fuel Reprocessing Facilities journal January 2013
Removal of Radioiodine from Gas Streams by Electrolytic Scrubbing journal September 1976
Iodosodalite Waste Forms from Low-Temperature Aqueous Process journal February 2018
Caustic scrubber waste converted to aluminosilicates: Structures determined by nuclear magnetic resonance journal February 2023
Expanded Analysis of Hot Isostatic Pressed Iodine-Loaded Silver-Exchanged Mordenite report September 2014
Preparation of Four Large-format Hot Isostatically Pressed I-AgZ Waste Form Samples for Performance Testing report September 2018
Compatibility of technologies with regulations in the waste management of H-3, I-129, C-14, and Kr-85. Part I. Initial information base report August 1983
Literature survey: methods for the removal of iodine species from off-gases and liquid waste streams of nuclear power and nuclear fuel reprocessing plants, with emphasis on solid sorbents report January 1979
Airborne elemental iodine loading capacities of metal zeolites and a method for recycling silver zeolite report July 1977
Molten Hydroxide Trapping Process for Radioiodine report January 2003
Abatement of radioiodine in aqueous reprocessing off-gas journal January 2023
Recent advances in the removal of radioactive iodine by bismuth-based materials journal January 2023
Development of New Waste Forms to Immobilize Iodine-129 Released from a Spent Fuel Reprocessing Plant journal October 2010