Ultrafast dense DNA functionalization of quantum dots and rods for scalable 2D array fabrication with nanoscale precision

Chen, Chi; Luo, Xin; Kaplan, Alexander E. K.; Bawendi, Moungi G.; Macfarlane, Robert J.; Bathe, Mark

doi:10.1126/sciadv.adh8508

Title: Ultrafast dense DNA functionalization of quantum dots and rods for scalable 2D array fabrication with nanoscale precision

Journal Article · Fri Aug 11 00:00:00 UTC 2023 · Science Advances

DOI: https://doi.org/10.1126/sciadv.adh8508 · OSTI ID:2424649

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Massachusetts Institute of Technology (MIT), Cambridge, MA (United States)

Scalable fabrication of two-dimensional (2D) arrays of quantum dots (QDs) and quantum rods (QRs) with nanoscale precision is required for numerous device applications. However, self-assembly–based fabrication of such arrays using DNA origami typically suffers from low yield due to inefficient QD and QR DNA functionalization. In addition, it is challenging to organize solution-assembled DNA origami arrays on 2D device substrates while maintaining their structural fidelity. Here, we reduced manufacturing time from a few days to a few minutes by preparing high-density DNA-conjugated QDs/QRs from organic solution using a dehydration and rehydration process. We used a surface-assisted large-scale assembly (SALSA) method to construct 2D origami lattices directly on solid substrates to template QD and QR 2D arrays with orientational control, with overall loading yields exceeding 90%. Our fabrication approach enables the scalable, high fidelity manufacturing of 2D addressable QDs and QRs with nanoscale orientational and spacing control for functional 2D photonic devices.

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Research Organization:: Massachusetts Institute of Technology (MIT), Cambridge, MA (United States)

Sponsoring Organization:: Army Research Office; National Institutes of Health (NIH); National Science Foundation (NSF); Office of Naval Research; USDOE

OSTI ID:: 2424649

Journal Information:: Science Advances, Journal Name: Science Advances Journal Issue: 32 Vol. 9; ISSN 2375-2548

Publisher:: AAASCopyright Statement

Country of Publication:: United States

Language:: English

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