This content will become publicly available on Wed Nov 20 00:00:00 EST 2024
Effects of diffusion barriers on reaction wave stability in Co/Al reactive multilayers
Abstract
Bimetallic, reactive multilayers are uniformly structured materials composed of alternating sputter-deposited layers that may be ignited to produce self-propagating mixing and formation reactions. These nanolaminates are most commonly used as rapid-release heat sources. The specific chemical composition at each metal/metal interface determines the rate of mass transport in a mixing and formation reaction. The inclusion of engineered diffusion barriers at each interface will not only inhibit solid-state mixing but also may impede the self-propagating reactions by introducing instabilities to wavefront morphology. Here, this work examines the effect of adding diffusion barriers on the propagation of reaction waves in Co/Al multilayers. The Co/Al system has been shown to exhibit a reaction propagation instability that is dependent on the bilayer thickness, which allows for the occurrence of unstable modes in otherwise stable designs from the inclusion of diffusion barriers. Based on the known stability criteria in the Co/Al multilayer system, the way in which the inclusion of diffusion barriers changes a multilayer's heat of reaction, thermal conductivity, and material mixing mechanisms can be determined. These factors, in aggregate, lead to changes in the wavefront velocity and stability.
- Authors:
-
[1];
[2];
[1];
[1];
[1];
[1]
- Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
- Lawrence Livermore National Laboratory (LLNL), Livermore, CA (United States)
- Publication Date:
- Research Org.:
- Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
- Sponsoring Org.:
- USDOE National Nuclear Security Administration (NNSA); USDOE Laboratory Directed Research and Development (LDRD) Program
- OSTI Identifier:
- 2311345
- Report Number(s):
- SAND-2023-13865J
Journal ID: ISSN 0021-8979
- Grant/Contract Number:
- NA0003525
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Journal of Applied Physics
- Additional Journal Information:
- Journal Volume: 134; Journal Issue: 19; Journal ID: ISSN 0021-8979
- Publisher:
- American Institute of Physics (AIP)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY; thermal conductivity; chemical energy; heat transfer; energetic materials; nanomaterials; diffusion barriers; mass diffusivity; differential scanning calorimetry; reaction mechanisms
Citation Formats
Abere, Michael Joseph Kim, Reeves, Robert Veeh, Sobczak, Catherine Elizabeth, Choi, Hyein, Kotula, Paul G., and Adams, David P. Effects of diffusion barriers on reaction wave stability in Co/Al reactive multilayers. United States: N. p., 2023.
Web. doi:10.1063/5.0171539.
Abere, Michael Joseph Kim, Reeves, Robert Veeh, Sobczak, Catherine Elizabeth, Choi, Hyein, Kotula, Paul G., & Adams, David P. Effects of diffusion barriers on reaction wave stability in Co/Al reactive multilayers. United States. https://doi.org/10.1063/5.0171539
Abere, Michael Joseph Kim, Reeves, Robert Veeh, Sobczak, Catherine Elizabeth, Choi, Hyein, Kotula, Paul G., and Adams, David P. Mon .
"Effects of diffusion barriers on reaction wave stability in Co/Al reactive multilayers". United States. https://doi.org/10.1063/5.0171539.
@article{osti_2311345,
title = {Effects of diffusion barriers on reaction wave stability in Co/Al reactive multilayers},
author = {Abere, Michael Joseph Kim and Reeves, Robert Veeh and Sobczak, Catherine Elizabeth and Choi, Hyein and Kotula, Paul G. and Adams, David P.},
abstractNote = {Bimetallic, reactive multilayers are uniformly structured materials composed of alternating sputter-deposited layers that may be ignited to produce self-propagating mixing and formation reactions. These nanolaminates are most commonly used as rapid-release heat sources. The specific chemical composition at each metal/metal interface determines the rate of mass transport in a mixing and formation reaction. The inclusion of engineered diffusion barriers at each interface will not only inhibit solid-state mixing but also may impede the self-propagating reactions by introducing instabilities to wavefront morphology. Here, this work examines the effect of adding diffusion barriers on the propagation of reaction waves in Co/Al multilayers. The Co/Al system has been shown to exhibit a reaction propagation instability that is dependent on the bilayer thickness, which allows for the occurrence of unstable modes in otherwise stable designs from the inclusion of diffusion barriers. Based on the known stability criteria in the Co/Al multilayer system, the way in which the inclusion of diffusion barriers changes a multilayer's heat of reaction, thermal conductivity, and material mixing mechanisms can be determined. These factors, in aggregate, lead to changes in the wavefront velocity and stability.},
doi = {10.1063/5.0171539},
journal = {Journal of Applied Physics},
number = 19,
volume = 134,
place = {United States},
year = {Mon Nov 20 00:00:00 EST 2023},
month = {Mon Nov 20 00:00:00 EST 2023}
}
Free Publicly Available Full Text
This content will become publicly available on November 20, 2024
Publisher's Version of Record
Other availability
Search WorldCat to find libraries that may hold this journal
Save to My Library
You must Sign In or Create an Account in order to save documents to your library.
Works referenced in this record:
A generalized reduced model of uniform and self-propagating reactions in reactive nanolaminates
journal, September 2013
- Alawieh, Leen; Weihs, Timothy P.; Knio, Omar M.
- Combustion and Flame, Vol. 160, Issue 9
The influence of premixed interlayers on the reaction propagation in Al–Ni multilayers —An MD approach
journal, February 2022
- Schwarz, Fabian; Spolenak, Ralph
- Journal of Applied Physics, Vol. 131, Issue 7
Nucleation and growth during reactions in multilayer Al/Ni films: The early stage of Al 3 Ni formation
journal, February 1991
- Ma, E.; Thompson, C. V.; Clevenger, L. A.
- Journal of Applied Physics, Vol. 69, Issue 4
A diffusion-limited reaction model for self-propagating Al/Pt multilayers with quench limits
journal, April 2018
- Kittell, D. E.; Yarrington, C. D.; Hobbs, M. L.
- Journal of Applied Physics, Vol. 123, Issue 14
In situ dynamic TEM characterization of unsteady crystallization during laser processing of amorphous germanium
journal, January 2018
- Egan, Garth C.; Li, Tian T.; Roehling, John D.
- Acta Materialia, Vol. 143
Joining bulk metallic glass using reactive multilayer foils
journal, June 2003
- Swiston, A. J.; Hufnagel, T. C.; Weihs, T. P.
- Scripta Materialia, Vol. 48, Issue 12, p. 1575-1580
Thermodynamic analysis of the Co–Al–C and Ni–Al–C systems by incorporating ab initio energetic calculations into the CALPHAD approach
journal, June 2004
- Ohtani, Hiroshi; Yamano, Maki; Hasebe, Mitsuhiro
- Calphad, Vol. 28, Issue 2
Numerical predictions of oscillatory combustion in reactive multilayers
journal, July 1999
- Jayaraman, S.; Knio, O. M.; Mann, A. B.
- Journal of Applied Physics, Vol. 86, Issue 2
Improved Exploding Properties of Al/Cu Multilayer Initiators
journal, August 2020
- Wang, Yao; Guo, Fei; Wang, Wanjun
- Propellants, Explosives, Pyrotechnics, Vol. 45, Issue 11
Simulation of reactive nanolaminates using reduced models: I. Basic formulation
journal, February 2010
- Salloum, Maher; Knio, Omar M.
- Combustion and Flame, Vol. 157, Issue 2
Reaction pathway of Ni/Al clad particles under thermal loading: A molecular dynamics simulation
journal, December 2013
- Wu, Hong-Zhang; Zhao, Shi-Jin
- Journal of Alloys and Compounds, Vol. 581
Complexion dictated thermal resistance with interface density in reactive metal multilayers
journal, June 2020
- Saltonstall, Christopher B.; McClure, Zachary D.; Abere, Michael J.
- Physical Review B, Vol. 101, Issue 24
Thermodynamics and defect structure of intermetallic phases with the B2 (CsCl) structure
journal, January 1982
- Chang, Y. Austin; Neumann, Joachim P.
- Progress in Solid State Chemistry, Vol. 14, Issue 4
Stability Criteria for Self-Propagating Reaction Waves in Co/Al Multilayers
journal, April 2023
- Abere, Michael J.; Reeves, Robert V.; Kittell, David E.
- ACS Applied Materials & Interfaces, Vol. 15, Issue 17
Exploring the Interfacial Reaction of Nano Al/CuO Energetic Films through Thermal Analysis and Ab Initio Molecular Dynamics Simulation
journal, June 2022
- Shi, Anran; Zheng, Han; Chen, Zhiyi
- Molecules, Vol. 27, Issue 11
Heating rate dependent ignition of Al/Pt nanolaminates through pulsed laser irradiation
journal, June 2018
- Abere, Michael J.; Yarrington, Cole D.; Adams, David P.
- Journal of Applied Physics, Vol. 123, Issue 23
Dissolution process at solid/liquid interface in nanometric metallic multilayers: Molecular dynamics simulations versus diffusion modeling
journal, October 2015
- Turlo, V.; Politano, O.; Baras, F.
- Acta Materialia, Vol. 99
Self-propagating reactions in Al/Zr multilayers: Anomalous dependence of reaction velocity on bilayer thickness
journal, December 2013
- Barron, S. C.; Kelly, S. T.; Kirchhoff, J.
- Journal of Applied Physics, Vol. 114, Issue 22, Article No. 223517
Reaction instabilities in Co/Al nanolaminates due to chemical kinetics variation over micron-scales
journal, January 2014
- Reeves, Robert V.; Adams, David P.
- Journal of Applied Physics, Vol. 115, Issue 4, Article No. 044911
Ignition in ternary Ru/Al-based reactive multilayers—Effects of chemistry and stacking sequence
journal, November 2018
- Pauly, C.; Woll, K.; Gallino, I.
- Journal of Applied Physics, Vol. 124, Issue 19
Enhancing the Reactivity of Al/CuO Nanolaminates by Cu Incorporation at the Interfaces
journal, May 2015
- Marín, Lorena; Nanayakkara, Charith E.; Veyan, Jean-Francois
- ACS Applied Materials & Interfaces, Vol. 7, Issue 22
Simulation of reactive nanolaminates using reduced models: II. Normal propagation
journal, March 2010
- Salloum, Maher; Knio, Omar M.
- Combustion and Flame, Vol. 157, Issue 3
Microstructural study of an oscillatory formation reaction in nanostructured reactive multilayer foils
journal, October 2005
- Trenkle, J. C.; Wang, J.; Weihs, T. P.
- Applied Physics Letters, Vol. 87, Issue 15
Phase mediated dynamics of self-propagating Co/Al nanolaminate reactions
journal, August 2020
- Abere, Michael J.; Egan, Garth C.; Kittell, David E.
- AIP Advances, Vol. 10, Issue 8
Deposition and characterization of a self-propagating CuOx/Al thermite reaction in a multilayer foil geometry
journal, September 2003
- Blobaum, K. J.; Reiss, M. E.; Plitzko, J. M.
- Journal of Applied Physics, Vol. 94, Issue 5
Controlling diffusion in Ni/Al reactive multilayers by Nb-alloying
journal, October 2017
- Schnabel, Volker; Sologubenko, Alla S.; Danzi, Stefano
- Applied Physics Letters, Vol. 111, Issue 17
Underwater Robotic Welding of Lap Joints with Sandwiched Reactive Multilayers: Thermal, Mechanical and Material Analysis
journal, March 2018
- Hussein, Aseel; Alkhoori, Ayesha; Zaabi, Abdelaziz Al
- MRS Advances, Vol. 3, Issue 17
Nanoenergetic Materials for MEMS: A Review
journal, August 2007
- Rossi, Carole; Zhang, Kaili; Esteve, Daniel
- Journal of Microelectromechanical Systems, Vol. 16, Issue 4
Atomic Scale Insights into the First Reaction Stages Prior to Al/CuO Nanothermite Ignition: Influence of Porosity
journal, June 2022
- Jabraoui, Hicham; Esteve, Alain; Schoenitz, Mirko
- ACS Applied Materials & Interfaces, Vol. 14, Issue 25
Effect of thermal properties on self-propagating fronts in reactive nanolaminates
journal, July 2011
- Alawieh, Leen; Knio, Omar M.; Weihs, Timothy P.
- Journal of Applied Physics, Vol. 110, Issue 1
Reactive multilayers fabricated by vapor deposition: A critical review
journal, February 2015
- Adams, D. P.
- Thin Solid Films, Vol. 576, p. 98-128
Importance of Bonding Atmosphere for Mechanical Reliability of Reactively Bonded Solder Joints
journal, December 2015
- Miyake, Shugo; Ohtani, Kohei; Inoue, Shozo
- Journal of Engineering Materials and Technology, Vol. 138, Issue 1
Reactive nanolayers for physiologically compatible microsystem packaging
journal, August 2009
- Qiu, Xiaotun; Welch, David; Christen, Jennifer Blain
- Journal of Materials Science: Materials in Electronics, Vol. 21, Issue 6
Models for Gasless Combustion in Layered Materials and Random Media
journal, June 1990
- Armstrong, Robert
- Combustion Science and Technology, Vol. 71, Issue 4-6
Intermetallic phase formation during annealing of Al/Ni multilayers
journal, December 1994
- Edelstein, A. S.; Everett, R. K.; Richardson, G. Y.
- Journal of Applied Physics, Vol. 76, Issue 12
Direct observation of spinlike reaction fronts in planar energetic multilayer foils
journal, January 2009
- McDonald, Joel P.; Hodges, V. Carter; Jones, Eric D.
- Applied Physics Letters, Vol. 94, Issue 3
Exothermic reactions in Co/Al nanolaminates
journal, August 2008
- Adams, D. P.; Hodges, V. C.; Bai, M. M.
- Journal of Applied Physics, Vol. 104, Issue 4, Article No. 043502
Modeling and characterizing the propagation velocity of exothermic reactions in multilayer foils
journal, August 1997
- Mann, A. B.; Gavens, A. J.; Reiss, M. E.
- Journal of Applied Physics, Vol. 82, Issue 3
Superheating and melting kinetics of confined thin films
journal, August 2006
- Zhang, L.; Zhang, L.; Sui, M.
- Acta Materialia, Vol. 54, Issue 13
Bayesian Inference of Atomic Diffusivity in a Binary Ni/Al System Based on Molecular Dynamics
journal, January 2011
- Rizzi, F.; Salloum, M.; Marzouk, Y. M.
- Multiscale Modeling & Simulation, Vol. 9, Issue 1
Exothermic reaction waves in multilayer nanofilms
journal, January 2008
- Rogachev, A. S.
- Russian Chemical Reviews, Vol. 77, Issue 1
Ultrafast formation of single phase B2 AlCoCrFeNi high entropy alloy films by reactive Ni/Al multilayers as heat source
journal, August 2021
- Wang, Anni; Gallino, Isabella; Riegler, Sascha Sebastian
- Materials & Design, Vol. 206
Reactive phase formation in sputter-deposited Ni/Al multilayer thin films
journal, January 1997
- Barmak, K.; Michaelsen, C.; Lucadamo, G.
- Journal of Materials Research, Vol. 12, Issue 1
Al/Ni reactive multilayer films enhancing the properties of plasma induced by nanosecond pulsed laser
journal, June 2021
- Wang, Yao; Qin, Wen-zhi; Li, Yong
- Energetic Materials Frontiers, Vol. 2, Issue 2
Multilayered Al/CuO thermite formation by reactive magnetron sputtering: Nano versus micro
journal, October 2010
- Petrantoni, M.; Rossi, C.; Salvagnac, L.
- Journal of Applied Physics, Vol. 108, Issue 8
3D simulations of spinlike flames in Co/Al multilayers with enhanced conduction losses
journal, June 2022
- Kittell, D. E.; Abere, M. J.; Yarrington, C. D.
- Combustion and Flame, Vol. 240
Thermal conductivity of B2-type aluminides and titanides
journal, January 1995
- Terada, Yoshihiro; Ohkubo, Kenji; Nakagawa, Kiyotaka
- Intermetallics, Vol. 3, Issue 5
Diffusion and thermite reaction process of film-honeycomb Al/NiO nanothermite: Molecular dynamics simulations using ReaxFF reactive force field
journal, May 2017
- Zeng, Hua-Dong; Zhu, Zhi-Yang; Zhang, Ji-Dong
- Chinese Physics B, Vol. 26, Issue 5
Electron transport in amorphous metals
journal, January 1984
- Naugle, D. G.
- Journal of Physics and Chemistry of Solids, Vol. 45, Issue 4
Stabilizing effects of oxidation on propagating formation reactions occurring in nanometer-scale metal multilayers
journal, October 2019
- Adams, D. P.; Abere, M. J.; Sobczak, C.
- Thin Solid Films, Vol. 688
Exploring the reaction mechanism in self-propagating Al/Ni multilayers by adding inert material
journal, October 2016
- Grapes, Michael D.; Weihs, Timothy P.
- Combustion and Flame, Vol. 172
Room-temperature soldering with nanostructured foils
journal, November 2003
- Wang, J.; Besnoin, E.; Duckham, A.
- Applied Physics Letters, Vol. 83, Issue 19
The growth and nanothermite reaction of 2Al/3NiO multilayer thin films
journal, July 2022
- Abere, Michael J.; Beason, Matthew T.; Reeves, Robert V.
- Journal of Applied Physics, Vol. 132, Issue 3
Time-resolved x-ray microdiffraction studies of phase transformations during rapidly propagating reactions in Al/Ni and Zr/Ni multilayer foils
journal, June 2010
- Trenkle, J. C.; Koerner, L. J.; Tate, M. W.
- Journal of Applied Physics, Vol. 107, Issue 11
Reaction Kinetics in Differential Thermal Analysis
journal, November 1957
- Kissinger, H. E.
- Analytical Chemistry, Vol. 29, Issue 11
A hermetic and room-temperature wafer bonding technique based on integrated reactive multilayer systems
journal, October 2014
- Braeuer, J.; Gessner, T.
- Journal of Micromechanics and Microengineering, Vol. 24, Issue 11
Exothermic Formation Reactions as Local Heat Sources
journal, July 2022
- Arlington, Shane Q.; Fritz, Gregory M.; Weihs, Timothy P.
- Annual Review of Materials Research, Vol. 52, Issue 1
Ignition and self-propagating reactions in Al/Pt multilayers of varied design
journal, September 2018
- Adams, D. P.; Reeves, R. V.; Abere, M. J.
- Journal of Applied Physics, Vol. 124, Issue 9
Rare-earth transition-metal intermetallic compounds produced via self-propagating, high-temperature synthesis
journal, April 2010
- McDonald, Joel P.; Rodriguez, Mark A.; Jones, Eric D.
- Journal of Materials Research, Vol. 25, Issue 4
SHS in Ni/Al Nanofoils: A Review of Experiments and Molecular Dynamics Simulations
journal, April 2018
- Baras, Florence; Turlo, Vladyslav; Politano, Olivier
- Advanced Engineering Materials, Vol. 20, Issue 8
Simulation of reactive nanolaminates using reduced models: III. Ingredients for a general multidimensional formulation
journal, June 2010
- Salloum, Maher; Knio, Omar M.
- Combustion and Flame, Vol. 157, Issue 6
Interfacial Chemistry in Al/CuO Reactive Nanomaterial and Its Role in Exothermic Reaction
journal, January 2013
- Kwon, Jinhee; Ducéré, Jean Marie; Alphonse, Pierre
- ACS Applied Materials & Interfaces, Vol. 5, Issue 3