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Title: Magnetism and fermiology of kagome magnet YMn6Sn4Ge2

Journal Article · · npj Quantum Materials

Kagome lattice magnets are an interesting class of materials as they can host topological properties in their magnetic and electronic structures. YMn6Sn6 is one such compound in which various exotic magnetic and electronic topological properties have been realized. Here, by means of a partial substitution of Sn with an isovalent and slightly smaller atom Ge, we demonstrate the sensitivity of such chemical substitution on the magnetic structure and its influence in the electronic properties. Magnetic structure of YMn6Sn4Ge2 determined by neutron diffraction reveals an incommensurate staggered magnetic spiral with a slightly larger spiral pitch than in YMn6Sn6. This change in magnetic structure influences the Fermi surface enhancing the out-of-plane conductivity. Such a sensitivity to the partial chemical substitution provides a great potential for engineering the magnetic phases and associated electronic properties not only in YMn6Sn6, but also in the large family of 166 rare-earth kagome magnet.

Research Organization:
Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division (MSE); USDOE Office of Science (SC), Basic Energy Sciences (BES). Scientific User Facilities (SUF); National Science Foundation (NSF)
Grant/Contract Number:
AC05-00OR22725; SC0021089
OSTI ID:
2281156
Journal Information:
npj Quantum Materials, Journal Name: npj Quantum Materials Journal Issue: 1 Vol. 9; ISSN 2397-4648
Publisher:
Nature Publishing GroupCopyright Statement
Country of Publication:
United States
Language:
English

References (40)

Large Room Temperature Anomalous Transverse Thermoelectric Effect in Kagome Antiferromagnet YMn6Sn6 journal August 2022
Recent advances in magnetic structure determination by neutron powder diffraction journal October 1993
Incommensurate magnetic structures of RMn6Sn6(R = Sc, Y, Lu) compounds from neutron diffraction study journal April 1996
Efficiency of ab-initio total energy calculations for metals and semiconductors using a plane-wave basis set journal July 1996
Neutron diffraction study of HfFe6Ge6-type TmMn6Sn6−Ga compounds (0.0≤x≤2.5) journal November 2002
A neutron diffraction study of HfFe6Ge6-type YMn6Sn6−xInx compounds (0.03≤x≤0.72) journal October 2003
Double-flat-spiral magnetic structures: Theory and application to the compounds journal May 2008
Massive Dirac fermions in a ferromagnetic kagome metal journal March 2018
Evidence for magnetic Weyl fermions in a correlated metal journal September 2017
Dirac cone, flat band and saddle point in kagome magnet YMn6Sn6 journal May 2021
Dirac fermions and flat bands in the ideal kagome metal FeSn journal December 2019
Topology and correlations on the kagome lattice journal January 2020
Negative flat band magnetism in a spin–orbit-coupled correlated kagome magnet journal February 2019
Manipulation of Dirac band curvature and momentum-dependent g factor in a kagome magnet journal March 2022
Magnetization-driven Lifshitz transition and charge-spin coupling in the kagome metal YMn6Sn6 journal March 2022
WIEN2k: An APW+lo program for calculating the properties of solids journal February 2020
Manifestation of axion electrodynamics through magnetic ordering on edges of a topological insulator journal August 2015
Emergent electromagnetic induction beyond room temperature journal August 2021
The TAIPAN thermal triple-axis spectrometer at the OPAL reactor journal January 2007
The quantum anomalous Hall effect in kagomé lattices journal August 2011
Field-induced topological Hall effect and double-fan spin structure with a c -axis component in the metallic kagome antiferromagnetic compound Y Mn 6 Sn 6 journal January 2021
Chiral properties of the zero-field spiral state and field-induced magnetic phases of the itinerant kagome metal YMn 6 Sn 6 journal March 2021
Electronic properties of the topological kagome metals YV6Sn6 and GdV6Sn6 journal December 2021
Uniaxial ferromagnetism in the kagome metal TbV6Sn6 journal September 2022
Efficient iterative schemes for ab initio total-energy calculations using a plane-wave basis set journal October 1996
Generalized gradient approximation for the exchange-correlation hole of a many-electron system journal December 1996
Spin anisotropy and quantum Hall effect in the kagomé lattice: Chiral spin state based on a ferromagnet journal September 2000
Majorana flat bands, chiral Majorana edge states, and unidirectional Majorana edge states in noncentrosymmetric superconductors journal April 2017
Electrically Detected Interferometry of Majorana Fermions in a Topological Insulator journal May 2009
Rare Earth Engineering in R Mn 6 Sn 6 ( R = Gd − Tm , Lu) Topological Kagome Magnets journal June 2021
Charge Density Wave in Kagome Lattice Intermetallic ScV6Sn6 journal November 2022
Model for a Quantum Hall Effect without Landau Levels: Condensed-Matter Realization of the "Parity Anomaly" journal October 1988
Highly anisotropic magnetism in the vanadium-based kagome metal TbV6Sn6 journal October 2022
Weyl and Dirac semimetals in three-dimensional solids journal January 2018
Rietveld refinement guidelines journal February 1999
Competing magnetic phases and fluctuation-driven scalar spin chirality in the kagome metal YMn 6 Sn 6 journal December 2020
Experimental Observation of the Quantum Anomalous Hall Effect in a Magnetic Topological Insulator journal March 2013
Quantized Faraday and Kerr rotation and axion electrodynamics of a 3D topological insulator journal December 2016
The Quantum Anomalous Hall Effect: Theory and Experiment journal March 2016
Interplay between magnetism and band topology in Kagome magnets RMn6Sn6 audiovisual January 2022