Escalated Phase Separation Driven Enhanced Magnetoresistance in Manganite/Iridate Epitaxial Heterostructures
Abstract
Phase separation in manganites leads to unique magnetic and electronic properties. 50% Ca-doped LaMnO3 (LCMO), at the boundary of ferromagnetic (FM) and antiferromagnetic (AFM) states in La1-xCaxMnO3 (0 ≤ x ≤ 1), is an ideal system to study phase separation behavior. The investigation reveals the effect of a 5d-metal perovskite SrIrO3 (SIO) on the phase separation, magnetic, and magnetoresistance (MR) properties of LCMO. Single-layer and bilayer LCMO films, both appear purely ferromagnetic along the in-plane (IP) magnetic field direction, but show the tendency of temperature-dependent ferromagnetic and antiferromagnetic or charge-ordered (CO) phase separation with the out-of-plane (OOP) applied field. The MR, and colossal magnetoresistance (CMR), observed in LCMO/SIO bilayers are two orders and an order of magnitude (in %) larger, respectively than that in the single-layer film. The coexistence of FM and AFM/CO phases is responsible for the CMR and MR enhancement in the LCMO/SIO bilayer, pointing toward the importance of the phase separation and competition of both the individual materials in enhancing their magnetic and electronic properties.
- Authors:
-
[1];
[2];
[1];
[2];
[3]
- State Univ. of New York (SUNY), Buffalo, NY (United States); Los Alamos National Laboratory (LANL), Los Alamos, NM (United States). Center for Integrated Nanotechnologies (CINT)
- Los Alamos National Laboratory (LANL), Los Alamos, NM (United States). Center for Integrated Nanotechnologies (CINT)
- State Univ. of New York (SUNY), Buffalo, NY (United States)
- Publication Date:
- Research Org.:
- Los Alamos National Laboratory (LANL), Los Alamos, NM (United States). Center for Integrated Nanotechnologies (CINT)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division (MSE); National Science Foundation (NSF); USDOE National Nuclear Security Administration (NNSA); USDOE Laboratory Directed Research and Development (LDRD) Program
- OSTI Identifier:
- 2217517
- Report Number(s):
- LA-UR-23-32756
Journal ID: ISSN 2751-1200
- Grant/Contract Number:
- 89233218CNA000001; ECCS-1902623
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Advanced Physics Research
- Additional Journal Information:
- Journal Volume: 3; Journal Issue: 1; Journal ID: ISSN 2751-1200
- Publisher:
- Wiley
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; colossal magnetoresistance (CMR); heterostructures; manganite; phase separation; SrIrO3
Citation Formats
Roy, Pinku, Zhang, Di, Kunwar, Sundar, Cucciniello, Nicholas, Mazza, Alessandro R., Chen, Aiping, and Jia, Quanxi. Escalated Phase Separation Driven Enhanced Magnetoresistance in Manganite/Iridate Epitaxial Heterostructures. United States: N. p., 2023.
Web. doi:10.1002/apxr.202300087.
Roy, Pinku, Zhang, Di, Kunwar, Sundar, Cucciniello, Nicholas, Mazza, Alessandro R., Chen, Aiping, & Jia, Quanxi. Escalated Phase Separation Driven Enhanced Magnetoresistance in Manganite/Iridate Epitaxial Heterostructures. United States. https://doi.org/10.1002/apxr.202300087
Roy, Pinku, Zhang, Di, Kunwar, Sundar, Cucciniello, Nicholas, Mazza, Alessandro R., Chen, Aiping, and Jia, Quanxi. Wed .
"Escalated Phase Separation Driven Enhanced Magnetoresistance in Manganite/Iridate Epitaxial Heterostructures". United States. https://doi.org/10.1002/apxr.202300087. https://www.osti.gov/servlets/purl/2217517.
@article{osti_2217517,
title = {Escalated Phase Separation Driven Enhanced Magnetoresistance in Manganite/Iridate Epitaxial Heterostructures},
author = {Roy, Pinku and Zhang, Di and Kunwar, Sundar and Cucciniello, Nicholas and Mazza, Alessandro R. and Chen, Aiping and Jia, Quanxi},
abstractNote = {Phase separation in manganites leads to unique magnetic and electronic properties. 50% Ca-doped LaMnO3 (LCMO), at the boundary of ferromagnetic (FM) and antiferromagnetic (AFM) states in La1-xCaxMnO3 (0 ≤ x ≤ 1), is an ideal system to study phase separation behavior. The investigation reveals the effect of a 5d-metal perovskite SrIrO3 (SIO) on the phase separation, magnetic, and magnetoresistance (MR) properties of LCMO. Single-layer and bilayer LCMO films, both appear purely ferromagnetic along the in-plane (IP) magnetic field direction, but show the tendency of temperature-dependent ferromagnetic and antiferromagnetic or charge-ordered (CO) phase separation with the out-of-plane (OOP) applied field. The MR, and colossal magnetoresistance (CMR), observed in LCMO/SIO bilayers are two orders and an order of magnitude (in %) larger, respectively than that in the single-layer film. The coexistence of FM and AFM/CO phases is responsible for the CMR and MR enhancement in the LCMO/SIO bilayer, pointing toward the importance of the phase separation and competition of both the individual materials in enhancing their magnetic and electronic properties.},
doi = {10.1002/apxr.202300087},
journal = {Advanced Physics Research},
number = 1,
volume = 3,
place = {United States},
year = {Wed Oct 25 00:00:00 EDT 2023},
month = {Wed Oct 25 00:00:00 EDT 2023}
}
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