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Title: Spin canting of Ni/CoO/Fe films grown on curved MgO(0 0 1) substrate

Abstract

Using element-resolved x-ray magnetic circular dichroism (XMCD) and x-ray magnetic linear dichroism (XMLD) measurements, we determined the spin orientations of Ni, CoO and Fe films in Ni/CoO/Fe films grown on a curved MgO(0 0 1) substrate. We find that the vicinal surface of MgO(0 0 1) substrate results in a spin canting towards out-of-plane direction in the Ni and CoO films as a result of the interfacial coupling. The Ni spin canting angle increases monotonically with the vicinal angle in the studied range of 0–17° and the CoO spin canting angle increases more rapidly towards saturation only at a few degrees of the vicinal angle. The uniaxial magnetic anisotropy induced in the Ni layer by the Ni/CoO interfacial coupling is quantitatively determined and is shown to increase monotonically with the vicinal angle. Our result provides a new pathway for tailoring the spin orientation by modifying the substrate surface symmetry in combining with the ferromagnetic/antiferromagnetic interfacial interaction in thin-film based spintronic devices.

Authors:
 [1];  [2];  [3];  [3];  [3];  [4];  [5];  [6];  [7];  [4]
  1. Anhui University, Hefei (China); Univ. of California, Berkeley, CA (United States)
  2. Univ. of Science and Technology of China, Hefei (China); Univ. of California, Berkeley, CA (United States)
  3. Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States). Advanced Light Source (ALS)
  4. Univ. of California, Berkeley, CA (United States)
  5. Fudan Univ., Shanghai (China)
  6. King Abdullah University of Science and Technology (KAUST), Thuwal (Saudi Arabia)
  7. Korea Research Institute of Standards and Science, Daejeon (Korea, Republic of)
Publication Date:
Research Org.:
Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES). Scientific User Facilities (SUF); USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division (MSE); USDOE Office of Science (SC), Basic Energy Sciences (BES)
OSTI Identifier:
1994321
Alternate Identifier(s):
OSTI ID: 1879112
Grant/Contract Number:  
AC02-05CH11231; AC02-05-CH11231; KCWF16
Resource Type:
Accepted Manuscript
Journal Name:
Journal of Magnetism and Magnetic Materials
Additional Journal Information:
Journal Volume: 561; Journal ID: ISSN 0304-8853
Publisher:
Elsevier
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE

Citation Formats

Yang, M., Li, Q., N'Diaye, A. T., Shafer, P., Klewe, C., Wang, T. Y., Wu, Y. Z., Zhang, Xixiang, Hwang, C., and Qiu, Z. Q. Spin canting of Ni/CoO/Fe films grown on curved MgO(0 0 1) substrate. United States: N. p., 2022. Web. doi:10.1016/j.jmmm.2022.169668.
Yang, M., Li, Q., N'Diaye, A. T., Shafer, P., Klewe, C., Wang, T. Y., Wu, Y. Z., Zhang, Xixiang, Hwang, C., & Qiu, Z. Q. Spin canting of Ni/CoO/Fe films grown on curved MgO(0 0 1) substrate. United States. https://doi.org/10.1016/j.jmmm.2022.169668
Yang, M., Li, Q., N'Diaye, A. T., Shafer, P., Klewe, C., Wang, T. Y., Wu, Y. Z., Zhang, Xixiang, Hwang, C., and Qiu, Z. Q. Fri . "Spin canting of Ni/CoO/Fe films grown on curved MgO(0 0 1) substrate". United States. https://doi.org/10.1016/j.jmmm.2022.169668. https://www.osti.gov/servlets/purl/1994321.
@article{osti_1994321,
title = {Spin canting of Ni/CoO/Fe films grown on curved MgO(0 0 1) substrate},
author = {Yang, M. and Li, Q. and N'Diaye, A. T. and Shafer, P. and Klewe, C. and Wang, T. Y. and Wu, Y. Z. and Zhang, Xixiang and Hwang, C. and Qiu, Z. Q.},
abstractNote = {Using element-resolved x-ray magnetic circular dichroism (XMCD) and x-ray magnetic linear dichroism (XMLD) measurements, we determined the spin orientations of Ni, CoO and Fe films in Ni/CoO/Fe films grown on a curved MgO(0 0 1) substrate. We find that the vicinal surface of MgO(0 0 1) substrate results in a spin canting towards out-of-plane direction in the Ni and CoO films as a result of the interfacial coupling. The Ni spin canting angle increases monotonically with the vicinal angle in the studied range of 0–17° and the CoO spin canting angle increases more rapidly towards saturation only at a few degrees of the vicinal angle. The uniaxial magnetic anisotropy induced in the Ni layer by the Ni/CoO interfacial coupling is quantitatively determined and is shown to increase monotonically with the vicinal angle. Our result provides a new pathway for tailoring the spin orientation by modifying the substrate surface symmetry in combining with the ferromagnetic/antiferromagnetic interfacial interaction in thin-film based spintronic devices.},
doi = {10.1016/j.jmmm.2022.169668},
journal = {Journal of Magnetism and Magnetic Materials},
number = ,
volume = 561,
place = {United States},
year = {Fri Jul 08 00:00:00 EDT 2022},
month = {Fri Jul 08 00:00:00 EDT 2022}
}

Works referenced in this record:

Magnetic uniaxial anisotropy of Fe films grown on vicinal Ag(001)
journal, April 2002


Multiple in-plane spin reorientation transitions in Fe / CoO bilayers grown on vicinal MgO ( 001 )
journal, March 2015


Magnetic versus crystal-field linear dichroism in NiO thin films
journal, January 2004


Coherent ac spin current transmission across an antiferromagnetic CoO insulator
journal, November 2019


Influence of crystal field on anisotropic x-ray magnetic linear dichroism at the Co 2 + L 2 , 3 edges
journal, February 2008


Complex strain evolution of polar and magnetic order in multiferroic BiFeO3 thin films
journal, September 2018


Ni spin switching induced by magnetic frustration in FeMn/Ni/Cu(001)
journal, June 2009


Fe/CoO(001) and Fe/CoO(111) bilayers: Effect of crystal orientation on the exchange bias
journal, August 2013


Interface-induced phenomena in magnetism
journal, June 2017


Néel vector reorientation in ferromagnetic/antiferromagnetic complex oxide nanostructures
journal, May 2019

  • Bang, A. D.; Hallsteinsen, I.; Olsen, F. K.
  • Applied Physics Letters, Vol. 114, Issue 19
  • DOI: 10.1063/1.5094604

Exchange bias theory
journal, September 2001


Role of interfacial structure on exchange-biased FeF 2 Fe
journal, March 1999


Temperature and thickness dependence of magnetic moments in NiO epitaxial films
journal, May 1998


Effect of CoO/Ni orthogonal exchange coupling on perpendicular anisotropy of Ni films on Pd(001)
journal, April 2015


Exchange-Induced Anisotropies at Ferromagnetic-Antiferromagnetic Interfaces above and below the Néel Temperature
journal, June 2003


Direct Measurement of Rotatable and Frozen CoO Spins in Exchange Bias System of CoO / Fe / Ag ( 001 )
journal, May 2010


Tailoring the spin direction of antiferromagnetic NiO thin films grown on vicinal Ag ( 001 )
journal, December 2006


Consequences of Spin-Flop Coupling in Exchange Biased Films
journal, November 1998


Activation of antiferromagnetic domain switching in exchange-coupled Fe/CoO/MgO(001) systems
journal, April 2015


Magnetic skyrmions: advances in physics and potential applications
journal, June 2017


Exchange bias
journal, February 1999


How Antiferromagnetism Drives the Magnetization of a Ferromagnetic Thin Film to Align Out of Plane
journal, March 2013


Substrate-modulated ferromagnetism of two-dimensional Fe 3 GeTe 2
journal, January 2020

  • Zhang, Luman; Song, Luyao; Dai, Hongwei
  • Applied Physics Letters, Vol. 116, Issue 4
  • DOI: 10.1063/1.5142077

Chirality switching of an antiferromagnetic spiral wall and its effect on magnetic anisotropy
journal, November 2019


Controlling Orbital Moment and Spin Orientation in CoO Layers by Strain
journal, October 2005


Ni and CoO spin cantings induced by Fe layer in Ni/CoO/Fe/vicinal MgO(001)
journal, December 2017


Independence of the spin current from the Néel vector orientation in antiferromagnet CoO
journal, June 2020