Epitaxial growth, magnetoresistance, and electronic band structure of GdSb magnetic semimetal films

Inbar, Hadass Shifra; Ho, Dai Q.; Chatterjee, Shouvik; Pendharkar, Mihir; Engel, Aaron N.; Dong, Jason T.; Khalid, Shoaib; Chang, Yu Hao; Guo, Taozhi; Fedorov, Alexei V.; Lu, Donghui; Hashimoto, Makoto; Read, Dan; Janotti, Anderson; Palmstrøm, Christopher J.

doi:10.1103/physrevmaterials.6.l121201

Title: Epitaxial growth, magnetoresistance, and electronic band structure of GdSb magnetic semimetal films

Journal Article · Fri Dec 09 00:00:00 UTC 2022 · Physical Review Materials

DOI: https://doi.org/10.1103/physrevmaterials.6.l121201 · OSTI ID:1985504

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University of California Santa Barbara, Santa Barbara, CA (United States)
University of Delaware, Newark, DE (United States); Quy Nhon University, Quy Nhon (Vietnam)
University of California Santa Barbara, Santa Barbara, CA (United States); Tata Institute of Fundamental Research Mumbai, (India)
University of California Santa Barbara, Santa Barbara, CA (United States); Stanford University, Stanford, CA (United States)
University of Delaware, Newark, DE (United States); National University of Science and Technology, Islamabad (Pakistan)
University of California Santa Barbara, Santa Barbara, CA (United States); Stanford University, Stanford, CA (United States) Princeton University, Princeton, NJ (United States)
Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)
SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)
University of California Santa Barbara, Santa Barbara, CA (United States); Cardiff University, Cardiff (United Kingdom)
University of Delaware, Newark, DE (United States)

Motivated by observations of extreme magnetoresistance (XMR) in bulk crystals of rare-earth monopnictide (RE-V) compounds and emerging applications in novel spintronic and plasmonic devices based on thin-film semimetals, we have investigated the electronic band structure and transport behavior of epitaxial GdSb thin films grown on III-V semiconductor surfaces. The Gd³+ ion in GdSb has a high spin S=7/2 and no orbital angular momentum, serving as a model system for studying the effects of antiferromagnetic order and strong exchange coupling on the resulting Fermi surface and magnetotransport properties of RE-Vs. Here, we present a surface and structural characterization study mapping the optimal synthesis window of thin epitaxial GdSb films grown on III-V lattice-matched buffer layers via molecular-beam epitaxy. To determine the factors limiting XMR in RE-V thin films and provide a benchmark for band-structure predictions of topological phases of RE-Vs, the electronic band structure of GdSb thin films is studied, comparing carrier densities extracted from magnetotransport, angle-resolved photoemission spectroscopy (ARPES), and density-functional theory (DFT) calculations. ARPES shows a hole-carrier rich, topologically trivial, semimetallic band structure close to complete electron-hole compensation, with quantum confinement effects in the thin films observed through the presence of quantum-well states. DFT-predicted Fermi wave vectors are in excellent agreement with values obtained from quantum oscillations observed in magnetic field-dependent resistivity measurements. An electron-rich Hall coefficient is measured despite the higher hole-carrier density, attributed to the higher electron Hall mobility. The carrier mobilities are limited by surface and interface scattering, resulting in lower magnetoresistance than that measured for bulk crystals.

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Research Organization:: Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES). Scientific User Facilities (SUF)

Grant/Contract Number:: AC02-05CH11231; AC02-76SF00515; SC0014388

OSTI ID:: 1985504

Journal Information:: Physical Review Materials, Journal Name: Physical Review Materials Journal Issue: 12 Vol. 6; ISSN 2475-9953

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Title: Epitaxial growth, magnetoresistance, and electronic band structure of GdSb magnetic semimetal films

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