Photoinduced Electron and Energy Transfer Pathways and Photocatalytic Mechanisms in Hybrid Plasmonic Photocatalysis

Ramakrishnan, Sundaram Bhardwaj; Mohammadparast, Farshid; Dadgar, Andishaeh P.; Mou, Tong; Le, Tien; Wang, Bin; Jain, Prashant K.; Andiappan, Marimuthu

doi:10.1002/adom.202101128

Title: Photoinduced Electron and Energy Transfer Pathways and Photocatalytic Mechanisms in Hybrid Plasmonic Photocatalysis

Journal Article · 09 September 2021 · Advanced Optical Materials

DOI: https://doi.org/10.1002/adom.202101128 · OSTI ID:1976227

Ramakrishnan, Sundaram Bhardwaj ^[1]; Mohammadparast, Farshid ^[2]; Dadgar, Andishaeh P. ^[2]; Mou, Tong ^[3]; Le, Tien ^[3]; Wang, Bin ^[3]; Jain, Prashant K. ^[4];

^[2]

Oklahoma State University, Stillwater, OK (United States); OSTI
Oklahoma State University, Stillwater, OK (United States)
University of Oklahoma, Norman, OK (United States)
University of Illinois at Urbana-Champaign, IL (United States)

Hybrid plasmonic nanostructures are built on plasmonic metalnanostructures surrounded by catalytic metals or metal oxides. We report that recent studies have shown that hybrid plasmonic nanocatalysts can concurrently utilize thermal energy and photon stimuli and exhibit high catalytic activity, selectivity, and stability that are not attainable in conventional purely thermally activated catalytic processes. The hybrid plasmonic photocatalytic approach has recently emerged as an attractive concept for the conversion of solar energy into chemical energy, the distributed synthesis of valuable chemicals such as ammonia with little to no requirement of external heating, and the development of coke-resistant and selective catalytic processes. The field of hybrid plasmonic photocatalysis has grown tremendously in the last decade. In this review article, the advantages of visible-light-augmented hybrid plasmonic photocatalysis over conventional pure thermally activated heterogeneous catalysis are discussed. Fundamental insights are provided into photocatalytic mechanisms by which the photoexcited charge carriers (electrons and holes) are formed and transferred to adsorbates triggering chemical transformations on the surface of hybrid plasmonic nanocatalysts. Computational modeling used for predicting and understanding the photocatalytic activity and selectivity on hybrid plasmonic nanostructures is also reviewed. The review closes with a discussion of the current challenges, new opportunities, and future outlook for hybrid plasmonic photocatalysis.

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Research Organization:: University of Oklahoma, Norman, OK (United States)

Sponsoring Organization:: USDOE Office of Science (SC); Oklahoma Center for the Advancement of Science and Technology; National Science Foundation (NSF)

Grant/Contract Number:: SC0020300

OSTI ID:: 1976227

Journal Information:: Advanced Optical Materials, Journal Name: Advanced Optical Materials Journal Issue: 22 Vol. 9; ISSN 2195-1071

Publisher:: WileyCopyright Statement

Country of Publication:: United States

Language:: English

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