Photoinduced Electron and Energy Transfer Pathways and Photocatalytic Mechanisms in Hybrid Plasmonic Photocatalysis
Abstract
Abstract Hybrid plasmonic nanostructures are built on plasmonic metalnanostructures surrounded by catalytic metals or metal oxides. Recent studies have shown that hybrid plasmonic nanocatalysts can concurrently utilize thermal energy and photon stimuli and exhibit high catalytic activity, selectivity, and stability that are not attainable in conventional purely thermally activated catalytic processes. The hybrid plasmonic photocatalytic approach has recently emerged as an attractive concept for the conversion of solar energy into chemical energy, the distributed synthesis of valuable chemicals such as ammonia with little to no requirement of external heating, and the development of coke‐resistant and selective catalytic processes. The field of hybrid plasmonic photocatalysis has grown tremendously in the last decade. In this review article, the advantages of visible‐light‐augmented hybrid plasmonic photocatalysis over conventional pure thermally activated heterogeneous catalysis are discussed. Fundamental insights are provided into photocatalytic mechanisms by which the photoexcited charge carriers (electrons and holes) are formed and transferred to adsorbates triggering chemical transformations on the surface of hybrid plasmonic nanocatalysts. Computational modeling used for predicting and understanding the photocatalytic activity and selectivity on hybrid plasmonic nanostructures is also reviewed. The review closes with a discussion of the current challenges, new opportunities, and future outlook for hybrid plasmonicmore »
- Authors:
-
[1]
- Oklahoma State University, Stillwater, OK (United States)
- University of Oklahoma, Norman, OK (United States)
- University of Illinois at Urbana-Champaign, IL (United States)
- Publication Date:
- Research Org.:
- Univ. of Oklahoma, Norman, OK (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC); Oklahoma Center for the Advancement of Science and Technology; National Science Foundation (NSF)
- OSTI Identifier:
- 1976227
- Alternate Identifier(s):
- OSTI ID: 1831549
- Grant/Contract Number:
- SC0020300; CBET-2102238; CHE-1455011; DE‐SC0020300
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Advanced Optical Materials
- Additional Journal Information:
- Journal Volume: 9; Journal Issue: 22; Journal ID: ISSN 2195-1071
- Publisher:
- Wiley
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; solar; nanoparticles; surface plasmon; oxide; energy
Citation Formats
Ramakrishnan, Sundaram Bhardwaj, Mohammadparast, Farshid, Dadgar, Andishaeh P., Mou, Tong, Le, Tien, Wang, Bin, Jain, Prashant K., and Andiappan, Marimuthu. Photoinduced Electron and Energy Transfer Pathways and Photocatalytic Mechanisms in Hybrid Plasmonic Photocatalysis. United States: N. p., 2021.
Web. doi:10.1002/adom.202101128.
Ramakrishnan, Sundaram Bhardwaj, Mohammadparast, Farshid, Dadgar, Andishaeh P., Mou, Tong, Le, Tien, Wang, Bin, Jain, Prashant K., & Andiappan, Marimuthu. Photoinduced Electron and Energy Transfer Pathways and Photocatalytic Mechanisms in Hybrid Plasmonic Photocatalysis. United States. https://doi.org/10.1002/adom.202101128
Ramakrishnan, Sundaram Bhardwaj, Mohammadparast, Farshid, Dadgar, Andishaeh P., Mou, Tong, Le, Tien, Wang, Bin, Jain, Prashant K., and Andiappan, Marimuthu. Thu .
"Photoinduced Electron and Energy Transfer Pathways and Photocatalytic Mechanisms in Hybrid Plasmonic Photocatalysis". United States. https://doi.org/10.1002/adom.202101128. https://www.osti.gov/servlets/purl/1976227.
@article{osti_1976227,
title = {Photoinduced Electron and Energy Transfer Pathways and Photocatalytic Mechanisms in Hybrid Plasmonic Photocatalysis},
author = {Ramakrishnan, Sundaram Bhardwaj and Mohammadparast, Farshid and Dadgar, Andishaeh P. and Mou, Tong and Le, Tien and Wang, Bin and Jain, Prashant K. and Andiappan, Marimuthu},
abstractNote = {Abstract Hybrid plasmonic nanostructures are built on plasmonic metalnanostructures surrounded by catalytic metals or metal oxides. Recent studies have shown that hybrid plasmonic nanocatalysts can concurrently utilize thermal energy and photon stimuli and exhibit high catalytic activity, selectivity, and stability that are not attainable in conventional purely thermally activated catalytic processes. The hybrid plasmonic photocatalytic approach has recently emerged as an attractive concept for the conversion of solar energy into chemical energy, the distributed synthesis of valuable chemicals such as ammonia with little to no requirement of external heating, and the development of coke‐resistant and selective catalytic processes. The field of hybrid plasmonic photocatalysis has grown tremendously in the last decade. In this review article, the advantages of visible‐light‐augmented hybrid plasmonic photocatalysis over conventional pure thermally activated heterogeneous catalysis are discussed. Fundamental insights are provided into photocatalytic mechanisms by which the photoexcited charge carriers (electrons and holes) are formed and transferred to adsorbates triggering chemical transformations on the surface of hybrid plasmonic nanocatalysts. Computational modeling used for predicting and understanding the photocatalytic activity and selectivity on hybrid plasmonic nanostructures is also reviewed. The review closes with a discussion of the current challenges, new opportunities, and future outlook for hybrid plasmonic photocatalysis.},
doi = {10.1002/adom.202101128},
journal = {Advanced Optical Materials},
number = 22,
volume = 9,
place = {United States},
year = {Thu Sep 09 00:00:00 EDT 2021},
month = {Thu Sep 09 00:00:00 EDT 2021}
}
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