Multifunctional polymer composite coatings and adhesives by incorporating cellulose nanomaterials

Wang, Lu; Kelly, Peter V.; Ozveren, Nihan; Zhang, Xuefeng; Korey, Matthew; Chen, Cong; Li, Kai; Bhandari, Sunil; Tekinalp, Halil; Zhao, Xianhui; Wang, Jinwu; Seydibeyoğlu, M. Özgür; Alyamac-Seydibeyoglu, Elif; Gramlich, William M.; Tajvidi, Mehdi; Webb, Erin; Ozcan, Soydan; Gardner, Douglas J.

doi:10.1016/j.matt.2022.11.024

Title: Multifunctional polymer composite coatings and adhesives by incorporating cellulose nanomaterials

Journal Article · Thu Dec 22 00:00:00 UTC 2022 · Matter (Online)

DOI: https://doi.org/10.1016/j.matt.2022.11.024 · OSTI ID:1928939

^[1]; Kelly, Peter V. ^[1]; Ozveren, Nihan ^[2]; Zhang, Xuefeng ^[3]; Korey, Matthew ^[4]; Chen, Cong ^[1];

^[5]; Bhandari, Sunil ^[1]; Tekinalp, Halil ^[4]; Zhao, Xianhui ^[6]; Wang, Jinwu ^[7]; Seydibeyoğlu, M. Özgür ^[8]; Alyamac-Seydibeyoglu, Elif ^[8]; Gramlich, William M. ^[1]; Tajvidi, Mehdi ^[1];

^[9];

^[4]; Gardner, Douglas J. ^[1]

Univ. of Maine, Orono, ME (United States)
Izmir Katip Celebi University (Turkey)
Mississippi State Univ., Mississippi State, MS (United States)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Manufacturing Science Division
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Buildings and Transportation Science Division
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Manufacturing Science Division; Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Environmental Science Division
US Forest Service, Madison, WI (United States)
Univ. of Maine, Orono, ME (United States); Izmir Katip Celebi University (Turkey)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Environmental Science Division

Regardless of their applications, polymers are still considered mechanically weak and functionally insufficient for certain demanding coating and adhesive uses. To address those issues, nanomaterials have been extensively studied as reinforcing fillers, which have been proven to effectively promote the performance of polymer coatings/adhesives. However, conventional nanofillers are expensive and non-biodegradable. Meanwhile, cellulose nanomaterials (CNMs), a class of nanomaterials produced from biomass feedstocks, can circumvent the drawbacks of conventional nanofillers. Here, this review paper first focuses on the multi-functionalities CNMs bring to polymer coatings, including mechanical reinforcement (wear resistance and hardness enhancement), gas barrier, flame resistance, corrosion resistance, self-healing (controlled-release), optical regulation, self-cleaning/antifouling, and antimicrobial characteristics. Then we discuss the benefits of CNM addition to polymer adhesives, such as mechanical enhancement, curing promotion, volatile organic compound (VOC) suppression, and electrical conductivity. Finally, we provide insights into future research efforts with CNMs. The goal of this paper is to promote the pilot-scale study and commercial use of CNMs as multifunctional additives in green and sustainable polymer composite coating and adhesive formulations.

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Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: USDOE Office of Energy Efficiency and Renewable Energy (EERE)

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 1928939

Journal Information:: Matter (Online), Journal Name: Matter (Online) Journal Issue: 2 Vol. 6; ISSN 2590-2385

Publisher:: Cell Press/ElsevierCopyright Statement

Country of Publication:: United States

Language:: English

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Biobased Poly(3-hydroxybutyrate)/Starch/Cellulose Nanofibrils for Nutrients Coatings França, Débora; Angelo, Luciana M.; Souza, Claudinei F. ACS Applied Polymer Materials, Vol. 3, Issue 6 https://doi.org/10.1021/acsapm.1c00418	journal	May 2021
High-Performance Waterborne Polyurethane Coating Based on a Blocked Isocyanate with Cellulose Nanocrystals (CNC) as the Polyol Chowdhury, Reaz A.; Clarkson, Caitlyn M.; Shrestha, Shikha ACS Applied Polymer Materials, Vol. 2, Issue 2 https://doi.org/10.1021/acsapm.9b00849	journal	December 2019
Toughening Effect of Rodlike Cellulose Nanocrystals in Epoxy Adhesive Pruksawan, Sirawit; Samitsu, Sadaki; Fujii, Yoshihisa ACS Applied Polymer Materials, Vol. 2, Issue 3 https://doi.org/10.1021/acsapm.9b01102	journal	January 2020
A Green Catechol-Containing Cellulose Nanofibrils-Cross-Linked Adhesive Tang, Zuwu; Zhang, Min; Xiao, He ACS Biomaterials Science & Engineering, Vol. 8, Issue 3 https://doi.org/10.1021/acsbiomaterials.1c01494	journal	February 2022
Cleaning of Oil Fouling with Water Enabled by Zwitterionic Polyelectrolyte Coatings: Overcoming the Imperative Challenge of Oil–Water Separation Membranes He, Ke; Duan, Haoran; Chen, George Y. ACS Nano, Vol. 9, Issue 9 https://doi.org/10.1021/acsnano.5b03791	journal	August 2015
High-Strength Polylactic Acid (PLA) Biocomposites Reinforced by Epoxy-Modified Pine Fibers Zhao, Xianhui; Li, Kai; Wang, Yu ACS Sustainable Chemistry & Engineering, Vol. 8, Issue 35 https://doi.org/10.1021/acssuschemeng.0c03463	journal	July 2020
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High Performance Biobased Epoxy Nanocomposite Reinforced with a Bacterial Cellulose Nanofiber Network Yue, Liang; Liu, Fei; Mekala, Shekar ACS Sustainable Chemistry & Engineering, Vol. 7, Issue 6 https://doi.org/10.1021/acssuschemeng.8b06073	journal	January 2019
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Cellulose Nanofibers Prepared by TEMPO-Mediated Oxidation of Native Cellulose Saito, Tsuguyuki; Kimura, Satoshi; Nishiyama, Yoshiharu Biomacromolecules, Vol. 8, Issue 8 https://doi.org/10.1021/bm0703970	journal	August 2007
Current characterization methods for cellulose nanomaterials Foster, E. Johan; Moon, Robert J.; Agarwal, Umesh P. Chemical Society Reviews, Vol. 47, Issue 8 https://doi.org/10.1039/C6CS00895J	journal	January 2018
Preparation of superhydrophobic coating with excellent abrasion resistance and durability using nanofibrillated cellulose Huang, Jingda; Lyu, Shaoyi; Fu, Feng RSC Advances, Vol. 6, Issue 108 https://doi.org/10.1039/C6RA23447J	journal	January 2016
Green preparation of a cellulose nanocrystals/polyvinyl alcohol composite superhydrophobic coating Huang, Jingda; Lyu, Shaoyi; Fu, Feng RSC Advances, Vol. 7, Issue 33 https://doi.org/10.1039/C6RA27663F	journal	January 2017
Cellulose microfibers (CMFs) as a smart carrier for autonomous self-healing in epoxy coatings Nawaz, Muddasir; Habib, Sehrish; Khan, Adnan New Journal of Chemistry, Vol. 44, Issue 15 https://doi.org/10.1039/C9NJ06436B	journal	January 2020
Progress in biomimetic leverages for marine antifouling using nanocomposite coatings Selim, Mohamed S.; El-Safty, Sherif A.; Shenashen, Mohamed A. Journal of Materials Chemistry B, Vol. 8, Issue 17 https://doi.org/10.1039/C9TB02119A	journal	January 2020
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Cottonseed protein-based wood adhesive reinforced with nanocellulose Cheng, H. N.; Kilgore, Kaylin; Ford, Catrina Journal of Adhesion Science and Technology, Vol. 33, Issue 12 https://doi.org/10.1080/01694243.2019.1596650	journal	April 2019
In-situmodification of low molar ratio urea–formaldehyde resins with cellulose nanofibrils for plywood Wibowo, Eko Setio; Lubis, Muhammad Adly Rahandi; Park, Byung-Dae Journal of Adhesion Science and Technology, Vol. 35, Issue 22 https://doi.org/10.1080/01694243.2021.1890370	journal	March 2021
Renewable UV-curable polyester methacrylate/cellulose nanocrystals composite resin for wood waterproof coating Tian, Yuan; Gao, Ya; Pan, Xueyi Nanotechnology, Vol. 32, Issue 27 https://doi.org/10.1088/1361-6528/abf20d	journal	April 2021
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Cellulose Nanocrystal Reinforced Chitosan Coatings for Improving the Storability of Postharvest Pears Under Both Ambient and Cold Storages Deng, Zilong; Jung, Jooyeoun; Simonsen, John Journal of Food Science, Vol. 82, Issue 2 https://doi.org/10.1111/1750-3841.13601	journal	February 2017
Micro- and Nanofibrillated Cellulose (MNFC) from Pineapple (Ananas comosus) Stems and Their Application on Polyvinyl Acetate (PVAc) and Urea-Formaldehyde (UF) Wood Adhesives Rigg-Aguilar, Priscilla; Moya, Roger; Oporto-Velásquez, Gloria S. Journal of Nanomaterials, Vol. 2020 https://doi.org/10.1155/2020/1393160	journal	August 2020
Nanocomposite coatings on steel for enhancing the corrosion resistance: A review Radhamani, Av; Lau, Hon Chung; Ramakrishna, S. Journal of Composite Materials, Vol. 54, Issue 5 https://doi.org/10.1177/0021998319857807	journal	July 2019
Epoxy/polyurethane nanocomposite coatings for anti-erosion/wear applications: A review Bahramnia, Hamed; Mohammadian Semnani, Hamidreza; Habibolahzadeh, Ali Journal of Composite Materials, Vol. 54, Issue 22 https://doi.org/10.1177/0021998320908299	journal	March 2020
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Easily Synthesized Polyaniline@Cellulose Nanowhiskers Better Tune Network Structures in Ag-Based Adhesives: Examining the Improvements in Conductivity, Stability, and Flexibility Cao, Ge; Gao, Xiaolan; Wang, Linlin Nanomaterials, Vol. 9, Issue 11 https://doi.org/10.3390/nano9111542	journal	October 2019
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