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Title: Atomic-Scale Modulation of Synthetic Magnetic Order in Oxide Superlattices

Abstract

Abstract Atomic‐scale precision control of magnetic interactions facilitates a synthetic spin order useful for spintronics, including advanced memory and quantum logic devices. Conventional modulation of synthetic spin order has been limited to metallic heterostructures that exploit Ruderman–Kittel–Kasuya–Yosida interaction through a nonmagnetic metallic spacer; however, they face issues arising from Joule heating and/or electric breakdown. The practical realization and observation of a synthetic spin order across a nonmagnetic insulating spacer will lead to the development of spin‐related devices with a completely different concept. Herein, the atomic‐scale modulation of the synthetic spiral spin order in oxide superlattices composed of ferromagnetic metal and nonmagnetic insulator layers is reported. The atomically controlled superlattice exhibits an oscillatory magnetic behavior, representing the existence of a spiral spin structure. Depth‐sensitive polarized neutron reflectometry evidences modulated spiral spin structures as a function of the nonmagnetic insulator layer thickness. Atomic‐scale customization of the spin state can move the field one step further to actual spintronic applications.

Authors:
ORCiD logo [1];  [2];  [2]; ORCiD logo [3]; ORCiD logo [1]
  1. Sungkyunkwan University, Suwon (Korea, Republic of)
  2. Pusan National University, Busan (Korea, Republic of)
  3. Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
Publication Date:
Research Org.:
Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
OSTI Identifier:
1907222
Alternate Identifier(s):
OSTI ID: 1995880
Grant/Contract Number:  
AC05-00OR22725
Resource Type:
Accepted Manuscript
Journal Name:
Small Methods
Additional Journal Information:
Journal Volume: 0; Journal Issue: 0; Journal ID: ISSN 2366-9608
Publisher:
Wiley
Country of Publication:
United States
Language:
English
Subject:
74 ATOMIC AND MOLECULAR PHYSICS; atomic-scale modulation; synthetic magnetic order; tunable magnetic noncollinearity; magnetic oxide superlattices; polarized neutron reflectometry

Citation Formats

Jeong, Seung Gyo, Song, Sehwan, Park, Sungkyun, Lauter, Valeria, and Choi, Woo Seok. Atomic-Scale Modulation of Synthetic Magnetic Order in Oxide Superlattices. United States: N. p., 2022. Web. doi:10.1002/smtd.202201386.
Jeong, Seung Gyo, Song, Sehwan, Park, Sungkyun, Lauter, Valeria, & Choi, Woo Seok. Atomic-Scale Modulation of Synthetic Magnetic Order in Oxide Superlattices. United States. https://doi.org/10.1002/smtd.202201386
Jeong, Seung Gyo, Song, Sehwan, Park, Sungkyun, Lauter, Valeria, and Choi, Woo Seok. Fri . "Atomic-Scale Modulation of Synthetic Magnetic Order in Oxide Superlattices". United States. https://doi.org/10.1002/smtd.202201386. https://www.osti.gov/servlets/purl/1907222.
@article{osti_1907222,
title = {Atomic-Scale Modulation of Synthetic Magnetic Order in Oxide Superlattices},
author = {Jeong, Seung Gyo and Song, Sehwan and Park, Sungkyun and Lauter, Valeria and Choi, Woo Seok},
abstractNote = {Abstract Atomic‐scale precision control of magnetic interactions facilitates a synthetic spin order useful for spintronics, including advanced memory and quantum logic devices. Conventional modulation of synthetic spin order has been limited to metallic heterostructures that exploit Ruderman–Kittel–Kasuya–Yosida interaction through a nonmagnetic metallic spacer; however, they face issues arising from Joule heating and/or electric breakdown. The practical realization and observation of a synthetic spin order across a nonmagnetic insulating spacer will lead to the development of spin‐related devices with a completely different concept. Herein, the atomic‐scale modulation of the synthetic spiral spin order in oxide superlattices composed of ferromagnetic metal and nonmagnetic insulator layers is reported. The atomically controlled superlattice exhibits an oscillatory magnetic behavior, representing the existence of a spiral spin structure. Depth‐sensitive polarized neutron reflectometry evidences modulated spiral spin structures as a function of the nonmagnetic insulator layer thickness. Atomic‐scale customization of the spin state can move the field one step further to actual spintronic applications.},
doi = {10.1002/smtd.202201386},
journal = {Small Methods},
number = 0,
volume = 0,
place = {United States},
year = {Fri Dec 23 00:00:00 EST 2022},
month = {Fri Dec 23 00:00:00 EST 2022}
}

Works referenced in this record:

Spin-orientation dependence in neutron reflection from a single magnetic film
journal, April 1995


Switchable giant nonreciprocal frequency shift of propagating spin waves in synthetic antiferromagnets
journal, April 2020


Terahertz spin-transfer torque oscillator based on a synthetic antiferromagnet
journal, March 2020


Post-synthesis control of Berry phase driven magnetotransport in SrRuO3 films
journal, February 2021


Giant room-temperature magnetoresistance in single-crystal Fe/MgO/Fe magnetic tunnel junctions
journal, October 2004

  • Yuasa, Shinji; Nagahama, Taro; Fukushima, Akio
  • Nature Materials, Vol. 3, Issue 12
  • DOI: 10.1038/nmat1257

Unconventional interlayer exchange coupling via chiral phonons in synthetic magnetic oxide heterostructures
journal, January 2022


Spin polarized neutron reflectivity of magnetic films and superlattices
journal, April 1994


Spin–phonon coupling in epitaxial SrRuO3 heterostructures
journal, January 2020

  • Jeong, Seung Gyo; Lim, Soo Yeon; Kim, Jiwoong
  • Nanoscale, Vol. 12, Issue 26
  • DOI: 10.1039/D0NR03282D

GenX : an extensible X-ray reflectivity refinement program utilizing differential evolution
journal, November 2007


Giant magnetoresistance in spin-valve multilayers
journal, September 1994


Polarized Neutron Reflectometry for the Analysis of Nanomagnetic Systems
journal, July 2008


Polarized neutron reflectivity studies of magnetic semiconductor superlattices
journal, July 2003


Transverse and Lateral Structure of the Spin-Flop Phase in F e / C r Antiferromagnetic Superlattices
journal, September 2002


Highlights from the magnetism reflectometer at the SNS
journal, September 2009

  • Lauter, Valeria; Ambaye, Hailemariam; Goyette, Richard
  • Physica B: Condensed Matter, Vol. 404, Issue 17, p. 2543-2546
  • DOI: 10.1016/j.physb.2009.06.021

Magnetic structure in Fe/Sm-Co exchange spring bilayers with intermixed interfaces
journal, May 2011


Long-range p–d exchange interaction in a ferromagnet–semiconductor hybrid structure
journal, October 2015

  • Korenev, V. L.; Salewski, M.; Akimov, I. A.
  • Nature Physics, Vol. 12, Issue 1
  • DOI: 10.1038/nphys3497

Spin Hall effects
journal, October 2015

  • Sinova, Jairo; Valenzuela, Sergio O.; Wunderlich, J.
  • Reviews of Modern Physics, Vol. 87, Issue 4
  • DOI: 10.1103/RevModPhys.87.1213

Skyrmions in magnetic multilayers
journal, August 2017


One Million Percent Tunnel Magnetoresistance in a Magnetic van der Waals Heterostructure
journal, July 2018


Room-Temperature Spin Hall Effect in Graphene/MoS 2 van der Waals Heterostructures
journal, January 2019


Atomistic Engineering of Phonons in Functional Oxide Heterostructures
journal, January 2022

  • Jeong, Seung Gyo; Seo, Ambrose; Choi, Woo Seok
  • Advanced Science, Vol. 9, Issue 7
  • DOI: 10.1002/advs.202103403

Synthetic antiferromagnetic spintronics
journal, March 2018


Symmetry-Driven Spin-Wave Gap Modulation in Nanolayered SrRuO3/SrTiO3 Heterostructures: Implications for Spintronic Applications
journal, February 2021

  • Jeong, Seung Gyo; Kim, Hyeonbeom; Hong, Sung Ju
  • ACS Applied Nano Materials, Vol. 4, Issue 2
  • DOI: 10.1021/acsanm.0c03463

Tailoring topological Hall effect in SrRuO3/SrTiO3 superlattices
journal, September 2021


Phase Instability amid Dimensional Crossover in Artificial Oxide Crystal
journal, January 2020


Propagation Control of Octahedral Tilt in SrRuO 3 via Artificial Heterostructuring
journal, June 2020

  • Jeong, Seung Gyo; Han, Gyeongtak; Song, Sehwan
  • Advanced Science, Vol. 7, Issue 16
  • DOI: 10.1002/advs.202001643

Exploiting Symmetry Mismatch to Control Magnetism in a Ferroelastic Heterostructure
journal, May 2019