Novel Nanotube Multiquantum Dot Devices
Abstract
Addressable quantum states well isolated from the environment are of considerable interest for quantum information science and technology. Carbon nanotubes are an appealing system, since a perfect crystal can be grown without any missing atoms and its cylindrical structure prevents ill-defined atomic arrangement at the surface. Here, we develop a reliable process to fabricate compact multielectrode circuits that can sustain the harsh conditions of the nanotube growth. Nanotubes are suspended over multiple gate electrodes, which are themselves structured over narrow dielectric ridges to reduce the effect of the charge fluctuators of the substrate. We measure high-quality double- and triple-quantum dot charge stability diagrams. Transport measurements through the triplequantum dot indicate long-range tunneling of single electrons between the left and right quantum dots. This work paves the way to the realization of a new generation of condensed-matter devices in an ultraclean environment, including spin qubits, mechanical qubits, and quantum simulators.
- Authors:
-
- ICFO - Institut De Ciencies Fotoniques, The Barcelona Institute of Science and Technology, 08860 Castelldefels, Barcelona, Spain
- Center for Nanoscale Materials, Argonne National Laboratory, Argonne, Illinois 60439, United States
- Publication Date:
- Research Org.:
- Inst. de Ciencies Fotoniques, Barcelona (Spain)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1894748
- Alternate Identifier(s):
- OSTI ID: 1897611
- Grant/Contract Number:
- AC02- 06CH11357; AC02-06CH11357
- Resource Type:
- Published Article
- Journal Name:
- Nano Letters
- Additional Journal Information:
- Journal Name: Nano Letters Journal Volume: 22 Journal Issue: 21; Journal ID: ISSN 1530-6984
- Publisher:
- American Chemical Society
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 77 NANOSCIENCE AND NANOTECHNOLOGY; quantum device; carbon nanotube; double-quantum dot; charge fluctuators; electrical conductivity; electrodes; electrostatic potential; nanotubes
Citation Formats
Tormo-Queralt, R., Møller, C. B., Czaplewski, D. A., Gruber, G., Cagetti, M., Forstner, S., Urgell-Ollé, N., Sanchez-Naranjo, J. A., Samanta, C., Miller, C. S., and Bachtold, A. Novel Nanotube Multiquantum Dot Devices. United States: N. p., 2022.
Web. doi:10.1021/acs.nanolett.2c03034.
Tormo-Queralt, R., Møller, C. B., Czaplewski, D. A., Gruber, G., Cagetti, M., Forstner, S., Urgell-Ollé, N., Sanchez-Naranjo, J. A., Samanta, C., Miller, C. S., & Bachtold, A. Novel Nanotube Multiquantum Dot Devices. United States. https://doi.org/10.1021/acs.nanolett.2c03034
Tormo-Queralt, R., Møller, C. B., Czaplewski, D. A., Gruber, G., Cagetti, M., Forstner, S., Urgell-Ollé, N., Sanchez-Naranjo, J. A., Samanta, C., Miller, C. S., and Bachtold, A. Wed .
"Novel Nanotube Multiquantum Dot Devices". United States. https://doi.org/10.1021/acs.nanolett.2c03034.
@article{osti_1894748,
title = {Novel Nanotube Multiquantum Dot Devices},
author = {Tormo-Queralt, R. and Møller, C. B. and Czaplewski, D. A. and Gruber, G. and Cagetti, M. and Forstner, S. and Urgell-Ollé, N. and Sanchez-Naranjo, J. A. and Samanta, C. and Miller, C. S. and Bachtold, A.},
abstractNote = {Addressable quantum states well isolated from the environment are of considerable interest for quantum information science and technology. Carbon nanotubes are an appealing system, since a perfect crystal can be grown without any missing atoms and its cylindrical structure prevents ill-defined atomic arrangement at the surface. Here, we develop a reliable process to fabricate compact multielectrode circuits that can sustain the harsh conditions of the nanotube growth. Nanotubes are suspended over multiple gate electrodes, which are themselves structured over narrow dielectric ridges to reduce the effect of the charge fluctuators of the substrate. We measure high-quality double- and triple-quantum dot charge stability diagrams. Transport measurements through the triplequantum dot indicate long-range tunneling of single electrons between the left and right quantum dots. This work paves the way to the realization of a new generation of condensed-matter devices in an ultraclean environment, including spin qubits, mechanical qubits, and quantum simulators.},
doi = {10.1021/acs.nanolett.2c03034},
journal = {Nano Letters},
number = 21,
volume = 22,
place = {United States},
year = {Wed Oct 26 00:00:00 EDT 2022},
month = {Wed Oct 26 00:00:00 EDT 2022}
}
https://doi.org/10.1021/acs.nanolett.2c03034
Works referenced in this record:
Electron transport in very clean, as-grown suspended carbon nanotubes
journal, September 2005
- Cao, Jien; Wang, Qian; Dai, Hongjie
- Nature Materials, Vol. 4, Issue 10
Strong Coupling Between Single-Electron Tunneling and Nanomechanical Motion
journal, August 2009
- Steele, G. A.; Hüttel, A. K.; Witkamp, B.
- Science, Vol. 325, Issue 5944
Imaging the electronic Wigner crystal in one dimension
journal, May 2019
- Shapir, I.; Hamo, A.; Pecker, S.
- Science, Vol. 364, Issue 6443
Hyperfine and Spin-Orbit Coupling Effects on Decay of Spin-Valley States in a Carbon Nanotube
journal, April 2017
- Pei, T.; Pályi, A.; Mergenthaler, M.
- Physical Review Letters, Vol. 118, Issue 17
Coupling Mechanics to Charge Transport in Carbon Nanotube Mechanical Resonators
journal, August 2009
- Lassagne, Benjamin; Tarakanov, Yury; Kinaret, Jari
- Science, Vol. 325, Issue 5944
Single-Electron Transport in Ropes of Carbon Nanotubes
journal, March 1997
- Bockrath, M.
- Science, Vol. 275, Issue 5308
Observation of the frozen charge of a Kondo resonance
journal, April 2017
- Desjardins, M. M.; Viennot, J. J.; Dartiailh, M. C.
- Nature, Vol. 545, Issue 7652
Quantum capacitance mediated carbon nanotube optomechanics
journal, April 2020
- Blien, Stefan; Steger, Patrick; Hüttner, Niklas
- Nature Communications, Vol. 11, Issue 1
Rapid gate-based spin read-out in silicon using an on-chip resonator
journal, July 2019
- Zheng, Guoji; Samkharadze, Nodar; Noordam, Marc L.
- Nature Nanotechnology, Vol. 14, Issue 8
Universality of non-equilibrium fluctuations in strongly correlated quantum liquids
journal, November 2015
- Ferrier, Meydi; Arakawa, Tomonori; Hata, Tokuro
- Nature Physics, Vol. 12, Issue 3
Evaluating charge noise acting on semiconductor quantum dots in the circuit quantum electrodynamics architecture
journal, August 2014
- Basset, J.; Stockklauser, A.; Jarausch, D. -D.
- Applied Physics Letters, Vol. 105, Issue 6
In situ
Tuning of the Electric-Dipole Strength of a Double-Dot Charge Qubit: Charge-Noise Protection and Ultrastrong Coupling
journal, July 2022
- Scarlino, P.; Ungerer, J. H.; van Woerkom, D. J.
- Physical Review X, Vol. 12, Issue 3
Layering Transition in Superfluid Helium Adsorbed on a Carbon Nanotube Mechanical Resonator
journal, April 2019
- Noury, Adrien; Vergara-Cruz, Jorge; Morfin, Pascal
- Physical Review Letters, Vol. 122, Issue 16
Stamping single wall nanotubes for circuit quantum electrodynamics
journal, March 2014
- Viennot, J. J.; Palomo, J.; Kontos, T.
- Applied Physics Letters, Vol. 104, Issue 11
Kondo physics in carbon nanotubes
journal, November 2000
- Nygård, Jesper; Cobden, David Henry; Lindelof, Poul Erik
- Nature, Vol. 408, Issue 6810
Coherent coupling of a single spin to microwave cavity photons
journal, July 2015
- Viennot, J. J.; Dartiailh, M. C.; Cottet, A.
- Science, Vol. 349, Issue 6246
Individual single-wall carbon nanotubes as quantum wires
journal, April 1997
- Tans, Sander J.; Devoret, Michel H.; Dai, Hongjie
- Nature, Vol. 386, Issue 6624
Ultraclean Single, Double, and Triple Carbon Nanotube Quantum Dots with Recessed Re Bottom Gates
journal, August 2013
- Jung, Minkyung; Schindele, Jens; Nau, Stefan
- Nano Letters, Vol. 13, Issue 9
The one-dimensional Wigner crystal in carbon nanotubes
journal, March 2008
- Deshpande, Vikram V.; Bockrath, Marc
- Nature Physics, Vol. 4, Issue 4
Quantum Interferences in Ultraclean Carbon Nanotubes
journal, May 2021
- Lotfizadeh, Neda; Senger, Mitchell J.; McCulley, Daniel R.
- Physical Review Letters, Vol. 126, Issue 21
A coherent nanomechanical oscillator driven by single-electron tunnelling
journal, October 2019
- Wen, Yutian; Ares, N.; Schupp, F. J.
- Nature Physics, Vol. 16, Issue 1
Fabry - Perot interference in a nanotube electron waveguide
journal, June 2001
- Liang, Wenjie; Bockrath, Marc; Bozovic, Dolores
- Nature, Vol. 411, Issue 6838
Non-equilibrium singlet–triplet Kondo effect in carbon nanotubes
journal, July 2006
- Paaske, J.; Rosch, A.; Wölfle, P.
- Nature Physics, Vol. 2, Issue 7
Valley–spin blockade and spin resonance in carbon nanotubes
journal, September 2012
- Pei, Fei; Laird, Edward A.; Steele, Gary A.
- Nature Nanotechnology, Vol. 7, Issue 10
Electron–nuclear interaction in 13C nanotube double quantum dots
journal, April 2009
- Churchill, H. O. H.; Bestwick, A. J.; Harlow, J. W.
- Nature Physics, Vol. 5, Issue 5
A brief overview of gate oxide defect properties and their relation to MOSFET instabilities and device and circuit time-dependent variability
journal, February 2018
- Kaczer, B.; Franco, J.; Weckx, P.
- Microelectronics Reliability, Vol. 81
Observation and spectroscopy of a two-electron Wigner molecule in an ultraclean carbon nanotube
journal, July 2013
- Pecker, S.; Kuemmeth, F.; Secchi, A.
- Nature Physics, Vol. 9, Issue 9
Identification of oxide defects in semiconductor devices: A systematic approach linking DFT to rate equations and experimental evidence
journal, August 2018
- Goes, W.; Wimmer, Y.; El-Sayed, A. -M.
- Microelectronics Reliability, Vol. 87
Electrostatically defined serial triple quantum dot charged with few electrons
journal, August 2007
- Schröer, D.; Greentree, A. D.; Gaudreau, L.
- Physical Review B, Vol. 76, Issue 7
Fabry-Pérot Oscillations in Correlated Carbon Nanotubes
journal, October 2020
- Yang, W.; Urgell, C.; De Bonis, S. L.
- Physical Review Letters, Vol. 125, Issue 18
Microwave Spectroscopy of a Carbon Nanotube Charge Qubit
journal, May 2017
- Penfold-Fitch, Z. V.; Sfigakis, F.; Buitelaar, M. R.
- Physical Review Applied, Vol. 7, Issue 5
Secondary Electron Interference from Trigonal Warping in Clean Carbon Nanotubes
journal, October 2016
- Dirnaichner, A.; del Valle, M.; Götz, K. J. G.
- Physical Review Letters, Vol. 117, Issue 16
Measuring the Complex Admittance of a Carbon Nanotube Double Quantum Dot
journal, January 2012
- Chorley, S. J.; Wabnig, J.; Penfold-Fitch, Z. V.
- Physical Review Letters, Vol. 108, Issue 3
Relaxation and Dephasing in a Two-ElectronC 13 Nanotube Double Quantum Dot
journal, April 2009
- Churchill, H. O. H.; Kuemmeth, F.; Harlow, J. W.
- Physical Review Letters, Vol. 102, Issue 16
Nanomechanical pump–probe measurements of insulating electronic states in a carbon nanotube
journal, January 2019
- Khivrich, Ilya; Clerk, Aashish A.; Ilani, Shahal
- Nature Nanotechnology, Vol. 14, Issue 2
Molecular states in carbon nanotube double quantum dots
journal, August 2006
- Gräber, M. R.; Coish, W. A.; Hoffmann, C.
- Physical Review B, Vol. 74, Issue 7
All-Microwave Control and Dispersive Readout of Gate-Defined Quantum Dot Qubits in Circuit Quantum Electrodynamics
journal, May 2019
- Scarlino, P.; van Woerkom, D. J.; Stockklauser, A.
- Physical Review Letters, Vol. 122, Issue 20
Orbital Kondo effect in carbon nanotubes
journal, March 2005
- Jarillo-Herrero, Pablo; Kong, Jing; van der Zant, Herre S. J.
- Nature, Vol. 434, Issue 7032
Broken SU(4) symmetry in a Kondo-correlated carbon nanotube
journal, April 2015
- Schmid, Daniel R.; Smirnov, Sergey; Margańska, Magdalena
- Physical Review B, Vol. 91, Issue 15
Nanotube mechanical resonators with quality factors of up to 5 million
journal, October 2014
- Moser, J.; Eichler, A.; Güttinger, J.
- Nature Nanotechnology, Vol. 9, Issue 12
Phonon-Induced Pairing in Quantum Dot Quantum Simulator
journal, November 2021
- Bhattacharya, Utso; Grass, Tobias; Bachtold, Adrian
- Nano Letters, Vol. 21, Issue 22
Stochastic charge trapping in oxides: From random telegraph noise to bias temperature instabilities
journal, January 2012
- Grasser, Tibor
- Microelectronics Reliability, Vol. 52, Issue 1
Real-space tailoring of the electron–phonon coupling in ultraclean nanotube mechanical resonators
journal, January 2014
- Benyamini, A.; Hamo, A.; Kusminskiy, S. Viola
- Nature Physics, Vol. 10, Issue 2
Charge noise and spin noise in a semiconductor quantum device
journal, July 2013
- Kuhlmann, Andreas V.; Houel, Julien; Ludwig, Arne
- Nature Physics, Vol. 9, Issue 9
Proposal for a Nanomechanical Qubit
journal, August 2021
- Pistolesi, F.; Cleland, A. N.; Bachtold, A.
- Physical Review X, Vol. 11, Issue 3
Current-induced cleaning of adsorbates from suspended single-walled carbon nanotube diodes
journal, June 2011
- Malapanis, Argyrios; Comfort, Everett; Ung Lee, Ji
- Applied Physics Letters, Vol. 98, Issue 26
Clean carbon nanotubes coupled to superconducting impedance-matching circuits
journal, May 2015
- Ranjan, V.; Puebla-Hellmann, G.; Jung, M.
- Nature Communications, Vol. 6, Issue 1
Quantum transport in carbon nanotubes
journal, July 2015
- Laird, Edward A.; Kuemmeth, Ferdinand; Steele, Gary A.
- Reviews of Modern Physics, Vol. 87, Issue 3
Few-Hundred GHz Carbon Nanotube Nanoelectromechanical Systems (NEMS)
journal, August 2012
- Island, J. O.; Tayari, V.; McRae, A. C.
- Nano Letters, Vol. 12, Issue 9
A valley–spin qubit in a carbon nanotube
journal, July 2013
- Laird, E. A.; Pei, F.; Kouwenhoven, L. P.
- Nature Nanotechnology, Vol. 8, Issue 8
Electron transport through double quantum dots
journal, December 2002
- van der Wiel, W. G.; De Franceschi, S.; Elzerman, J. M.
- Reviews of Modern Physics, Vol. 75, Issue 1
Realization of pristine and locally tunable one-dimensional electron systems in carbon nanotubes
journal, August 2013
- Waissman, J.; Honig, M.; Pecker, S.
- Nature Nanotechnology, Vol. 8, Issue 8
Strong coupling of a single electron in silicon to a microwave photon
journal, December 2016
- Mi, X.; Cady, J. V.; Zajac, D. M.
- Science, Vol. 355, Issue 6321
Long-Range Spin Transfer in Triple Quantum Dots
journal, May 2014
- Sánchez, R.; Granger, G.; Gaudreau, L.
- Physical Review Letters, Vol. 112, Issue 17
Cooling and self-oscillation in a nanotube electromechanical resonator
journal, October 2019
- Urgell, C.; Yang, W.; De Bonis, S. L.
- Nature Physics, Vol. 16, Issue 1
Highly coherent spin states in carbon nanotubes coupled to cavity photons
journal, July 2019
- Cubaynes, T.; Delbecq, M. R.; Dartiailh, M. C.
- npj Quantum Information, Vol. 5, Issue 1
High-bias-induced structure and the corresponding electronic property changes in carbon nanotubes
journal, December 2005
- Chen, S.; Huang, J. Y.; Wang, Z.
- Applied Physics Letters, Vol. 87, Issue 26
Strong Coupling Cavity QED with Gate-Defined Double Quantum Dots Enabled by a High Impedance Resonator
journal, March 2017
- Stockklauser, A.; Scarlino, P.; Koski, J. V.
- Physical Review X, Vol. 7, Issue 1
A two-qubit logic gate in silicon
journal, October 2015
- Veldhorst, M.; Yang, C. H.; Hwang, J. C. C.
- Nature, Vol. 526, Issue 7573, p. 410-414
Nature of intrinsic and extrinsic electron trapping in SiO
journal, March 2014
- El-Sayed, Al-Moatasem; Watkins, Matthew B.; Afanas'ev, Valery V.
- Physical Review B, Vol. 89, Issue 12
Stability Diagram of a Few-Electron Triple Dot
journal, July 2006
- Gaudreau, L.; Studenikin, S. A.; Sachrajda, A. S.
- Physical Review Letters, Vol. 97, Issue 3
Nanomechanical Characterization of the Kondo Charge Dynamics in a Carbon Nanotube
journal, June 2018
- Götz, K. J. G.; Schmid, D. R.; Schupp, F. J.
- Physical Review Letters, Vol. 120, Issue 24
Tomonaga-Luttinger Liquid Features in Ballistic Single-Walled Carbon Nanotubes: Conductance and Shot Noise
journal, July 2007
- Kim, Na Young; Recher, Patrik; Oliver, William D.
- Physical Review Letters, Vol. 99, Issue 3