Novel Co‐Catalytic Activities of Solid and Liquid Phase Catalysts in High‐Rate Li‐Air Batteries
Abstract
Abstract Li‐air batteries are considered strong candidates for the next‐generation energy storage systems designed for electrical transportation. However, low cyclability and current rates are two major drawbacks that hinder them from further realization. These issues necessitate the discovery of novel materials to significantly enhance the redox process of discharge products. In this study, a novel catalytic system comprised of tin sulfide (SnS) nanoflakes as a solid catalyst and tin iodide (SnI 2 ) as a dual‐functional electrolyte additive is discovered. This system enables operating the battery at high current rates up to 10 000 mA g −1 (corresponding to 1 mA cm −2 ). The SnS catalyst shows outstanding catalytic activity for both oxygen reduction and evolution reactions compared to carbon, noble metals, and other transition metal dichalcogenides. It also exhibits good structural integrity at high rates. The computations indicate numerous possible oxygen reduction sites without oxygen dissociations on the SnS surface through solution mechanism that is likely responsible for the formation of Li 2 O 2 . The calculations also indicate that the role of the SnI 2 is not only reacting with the lithium anode to provide protection but reducing the charge potential by promoting catalytic decomposition of the Li 2more »
- Authors:
-
[1];
[2]
- Department of Mechanical and Industrial Engineering University of Illinois at Chicago Chicago IL 60607 USA, Materials Science Division Argonne National Laboratory Argonne IL 60439 USA
- Department of Mechanical and Industrial Engineering University of Illinois at Chicago Chicago IL 60607 USA
- Materials Science Division Argonne National Laboratory Argonne IL 60439 USA, Department of Chemical Engineering University of Illinois at Chicago Chicago IL 60607 USA
- Department of Physics University of Illinois at Chicago Chicago IL 60607 USA
- Materials Science Division Argonne National Laboratory Argonne IL 60439 USA
- Publication Date:
- Sponsoring Org.:
- USDOE
- OSTI Identifier:
- 1892365
- Alternate Identifier(s):
- OSTI ID: 1901488
- Resource Type:
- Published Article
- Journal Name:
- Advanced Energy Materials
- Additional Journal Information:
- Journal Name: Advanced Energy Materials Journal Volume: 12 Journal Issue: 45; Journal ID: ISSN 1614-6832
- Publisher:
- Wiley Blackwell (John Wiley & Sons)
- Country of Publication:
- Germany
- Language:
- English
Citation Formats
Zhang, Chengji, Jaradat, Ahmad, Singh, Sachin Kumar, Rojas, Tomas, Ahmadiparidari, Alireza, Rastegar, Sina, Wang, Shuxi, Majidi, Leily, Redfern, Paul, Subramanian, Arunkumar, Ngo, Anh T., Curtiss, Larry A., and Salehi‐khojin, Amin. Novel Co‐Catalytic Activities of Solid and Liquid Phase Catalysts in High‐Rate Li‐Air Batteries. Germany: N. p., 2022.
Web. doi:10.1002/aenm.202201616.
Zhang, Chengji, Jaradat, Ahmad, Singh, Sachin Kumar, Rojas, Tomas, Ahmadiparidari, Alireza, Rastegar, Sina, Wang, Shuxi, Majidi, Leily, Redfern, Paul, Subramanian, Arunkumar, Ngo, Anh T., Curtiss, Larry A., & Salehi‐khojin, Amin. Novel Co‐Catalytic Activities of Solid and Liquid Phase Catalysts in High‐Rate Li‐Air Batteries. Germany. https://doi.org/10.1002/aenm.202201616
Zhang, Chengji, Jaradat, Ahmad, Singh, Sachin Kumar, Rojas, Tomas, Ahmadiparidari, Alireza, Rastegar, Sina, Wang, Shuxi, Majidi, Leily, Redfern, Paul, Subramanian, Arunkumar, Ngo, Anh T., Curtiss, Larry A., and Salehi‐khojin, Amin. Thu .
"Novel Co‐Catalytic Activities of Solid and Liquid Phase Catalysts in High‐Rate Li‐Air Batteries". Germany. https://doi.org/10.1002/aenm.202201616.
@article{osti_1892365,
title = {Novel Co‐Catalytic Activities of Solid and Liquid Phase Catalysts in High‐Rate Li‐Air Batteries},
author = {Zhang, Chengji and Jaradat, Ahmad and Singh, Sachin Kumar and Rojas, Tomas and Ahmadiparidari, Alireza and Rastegar, Sina and Wang, Shuxi and Majidi, Leily and Redfern, Paul and Subramanian, Arunkumar and Ngo, Anh T. and Curtiss, Larry A. and Salehi‐khojin, Amin},
abstractNote = {Abstract Li‐air batteries are considered strong candidates for the next‐generation energy storage systems designed for electrical transportation. However, low cyclability and current rates are two major drawbacks that hinder them from further realization. These issues necessitate the discovery of novel materials to significantly enhance the redox process of discharge products. In this study, a novel catalytic system comprised of tin sulfide (SnS) nanoflakes as a solid catalyst and tin iodide (SnI 2 ) as a dual‐functional electrolyte additive is discovered. This system enables operating the battery at high current rates up to 10 000 mA g −1 (corresponding to 1 mA cm −2 ). The SnS catalyst shows outstanding catalytic activity for both oxygen reduction and evolution reactions compared to carbon, noble metals, and other transition metal dichalcogenides. It also exhibits good structural integrity at high rates. The computations indicate numerous possible oxygen reduction sites without oxygen dissociations on the SnS surface through solution mechanism that is likely responsible for the formation of Li 2 O 2 . The calculations also indicate that the role of the SnI 2 is not only reacting with the lithium anode to provide protection but reducing the charge potential by promoting catalytic decomposition of the Li 2 O 2 . This work provides new novel additives for designing high‐rate Li‐air batteries.},
doi = {10.1002/aenm.202201616},
journal = {Advanced Energy Materials},
number = 45,
volume = 12,
place = {Germany},
year = {Thu Oct 13 00:00:00 EDT 2022},
month = {Thu Oct 13 00:00:00 EDT 2022}
}
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