2022 roadmap on low temperature electrochemical CO 2 reduction

Stephens, Ifan E. L.; Chan, Karen; Bagger, Alexander; Boettcher, Shannon W.; Bonin, Julien; Boutin, Etienne; Buckley, Aya K.; Buonsanti, Raffaella; Cave, Etosha R.; Chang, Xiaoxia; Chee, See Wee; da Silva, Alisson H. M.; de Luna, Phil; Einsle, Oliver; Endrődi, Balázs; Escudero-Escribano, Maria; Ferreira de Araujo, Jorge V.; Figueiredo, Marta C.; Hahn, Christopher; Hansen, Kentaro U.; Haussener, Sophia; Hunegnaw, Sara; Huo, Ziyang; Hwang, Yun Jeong; Janáky, Csaba; Jayathilake, Buddhinie S.; Jiao, Feng; Jovanov, Zarko P.; Karimi, Parisa; Koper, Marc T. M.; Kuhl, Kendra P.; Lee, Woong Hee; Liang, Zhiqin; Liu, Xuan; Ma, Sichao; Ma, Ming; Oh, Hyung-Suk; Robert, Marc; Cuenya, Beatriz Roldan; Rossmeisl, Jan; Roy, Claudie; Ryan, Mary P.; Sargent, Edward H.; Sebastián-Pascual, Paula; Seger, Brian; Steier, Ludmilla; Strasser, Peter; Varela, Ana Sofia; Vos, Rafaël E.; Wang, Xue; Xu, Bingjun; Yadegari, Hossein; Zhou, Yuxiang

doi:10.1088/2515-7655/ac7823

Title: 2022 roadmap on low temperature electrochemical CO ₂ reduction

Journal Article · Mon Oct 03 00:00:00 UTC 2022 · JPhys Energy

DOI: https://doi.org/10.1088/2515-7655/ac7823 · OSTI ID:1890534

;

; Buckley, Aya K.;

; Cave, Etosha R.;

;

; Hansen, Kentaro U. more »

Abstract Electrochemical CO ₂ reduction (CO ₂ R) is an attractive option for storing renewable electricity and for the sustainable production of valuable chemicals and fuels. In this roadmap, we review recent progress in fundamental understanding, catalyst development, and in engineering and scale-up. We discuss the outstanding challenges towards commercialization of electrochemical CO ₂ R technology: energy efficiencies, selectivities, low current densities, and stability. We highlight the opportunities in establishing rigorous standards for benchmarking performance, advances in in operando characterization, the discovery of new materials towards high value products, the investigation of phenomena across multiple-length scales and the application of data science towards doing so. We hope that this collective perspective sparks new research activities that ultimately bring us a step closer towards establishing a low- or zero-emission carbon cycle.

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Research Organization:: Lawrence Livermore National Laboratory (LLNL), Livermore, CA (United States)

Sponsoring Organization:: USDOE; USDOE National Nuclear Security Administration (NNSA); USDOE Office of Energy Efficiency and Renewable Energy (EERE)

Grant/Contract Number:: AC52-07NA27344; EE0008841; FE0031910; SC0021266

OSTI ID:: 1890534

Report Number(s):: LLNL-JRNL--825464

Journal Information:: JPhys Energy, Journal Name: JPhys Energy Journal Issue: 4 Vol. 4; ISSN 2515-7655

Publisher:: IOP PublishingCopyright Statement

Country of Publication:: United Kingdom

Language:: English

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How copper catalyzes the electroreduction of carbon dioxide into hydrocarbon fuels Peterson, Andrew A.; Abild-Pedersen, Frank; Studt, Felix Energy & Environmental Science, Vol. 3, Issue 9 https://doi.org/10.1039/c0ee00071j	journal	January 2010
Structure sensitivity and nanoscale effects in electrocatalysis Koper, Marc T. M. Nanoscale, Vol. 3, Issue 5, p. 2054-2073 https://doi.org/10.1039/c0nr00857e	journal	January 2011
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