Visualizing the out-of-plane electronic dispersions in an intercalated transition metal dichalcogenide
Abstract
Layered transition metal dichalcogenides have a rich phase diagram and they feature two-dimensionality in numerous physical properties. Co1/3NbS2 is one of the newest members of this family where Co atoms are intercalated into the van der Waals gaps between NbS2 layers. Here, we study the three-dimensional electronic band structure of Co1/3NbS2 using both surface and bulk sensitive angle-resolved photoemission spectroscopy. We show that the electronic bands do not fit into the rigid band shift picture after the Co intercalation. Instead, Co1/3NbS2 displays a different orbital character near the Fermi level compared to the pristine NbS2 compound and has a clear band dispersion in the kz direction despite its layered structure. Our photoemission study demonstrates the out-of-plane electronic correlations introduced by the Co intercalation, thus offering a different perspective on this compound. Finally, we propose how Fermi level tuning could lead to exotic phases such as spin density wave instability.
- Authors:
-
[1];
[2];
[1];
[1];
[6];
- Princeton Univ., NJ (United States)
- Arizona State Univ., Tempe, AZ (United States)
- George Mason Univ., Fairfax, VA (United States)
- Paul Scherrer Inst. (PSI), Villigen (Switzerland)
- National Inst. of Standards and Technology (NIST), Gaithersburg, MD (United States); Purdue Univ., West Lafayette, IN (United States)
- National Inst. of Standards and Technology (NIST), Gaithersburg, MD (United States)
- Publication Date:
- Research Org.:
- Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division; National Science Foundation (NSF)
- OSTI Identifier:
- 1885145
- Grant/Contract Number:
- AC02-05CH11231; FG02-05ER46200; DMR 1904716; DGE-1656466
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Physical Review. B
- Additional Journal Information:
- Journal Volume: 105; Journal Issue: 12; Journal ID: ISSN 2469-9950
- Publisher:
- American Physical Society (APS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; anomalous Hall effect; antiferromagnetism; atomic orbital; transition metal dichalcogenides; angle-resolved photoemission spectroscopy; first-principles calculations; topology
Citation Formats
Yang, Xian P., LaBollita, Harrison, Cheng, Zi-Jia, Bhandari, Hari, Cochran, Tyler A., Yin, Jia-Xin, Hossain, Md. Shafayat, Belopolski, Ilya, Zhang, Qi, Jiang, Yuxiao, Shumiya, Nana, Multer, Daniel, Liskevich, Maksim, Usanov, Dmitry A., Dang, Yanliu, Strocov, Vladimir N., Davydov, Albert V., Ghimire, Nirmal J., Botana, Antia S., and Hasan, M. Zahid. Visualizing the out-of-plane electronic dispersions in an intercalated transition metal dichalcogenide. United States: N. p., 2022.
Web. doi:10.1103/physrevb.105.l121107.
Yang, Xian P., LaBollita, Harrison, Cheng, Zi-Jia, Bhandari, Hari, Cochran, Tyler A., Yin, Jia-Xin, Hossain, Md. Shafayat, Belopolski, Ilya, Zhang, Qi, Jiang, Yuxiao, Shumiya, Nana, Multer, Daniel, Liskevich, Maksim, Usanov, Dmitry A., Dang, Yanliu, Strocov, Vladimir N., Davydov, Albert V., Ghimire, Nirmal J., Botana, Antia S., & Hasan, M. Zahid. Visualizing the out-of-plane electronic dispersions in an intercalated transition metal dichalcogenide. United States. https://doi.org/10.1103/physrevb.105.l121107
Yang, Xian P., LaBollita, Harrison, Cheng, Zi-Jia, Bhandari, Hari, Cochran, Tyler A., Yin, Jia-Xin, Hossain, Md. Shafayat, Belopolski, Ilya, Zhang, Qi, Jiang, Yuxiao, Shumiya, Nana, Multer, Daniel, Liskevich, Maksim, Usanov, Dmitry A., Dang, Yanliu, Strocov, Vladimir N., Davydov, Albert V., Ghimire, Nirmal J., Botana, Antia S., and Hasan, M. Zahid. Mon .
"Visualizing the out-of-plane electronic dispersions in an intercalated transition metal dichalcogenide". United States. https://doi.org/10.1103/physrevb.105.l121107. https://www.osti.gov/servlets/purl/1885145.
@article{osti_1885145,
title = {Visualizing the out-of-plane electronic dispersions in an intercalated transition metal dichalcogenide},
author = {Yang, Xian P. and LaBollita, Harrison and Cheng, Zi-Jia and Bhandari, Hari and Cochran, Tyler A. and Yin, Jia-Xin and Hossain, Md. Shafayat and Belopolski, Ilya and Zhang, Qi and Jiang, Yuxiao and Shumiya, Nana and Multer, Daniel and Liskevich, Maksim and Usanov, Dmitry A. and Dang, Yanliu and Strocov, Vladimir N. and Davydov, Albert V. and Ghimire, Nirmal J. and Botana, Antia S. and Hasan, M. Zahid},
abstractNote = {Layered transition metal dichalcogenides have a rich phase diagram and they feature two-dimensionality in numerous physical properties. Co1/3NbS2 is one of the newest members of this family where Co atoms are intercalated into the van der Waals gaps between NbS2 layers. Here, we study the three-dimensional electronic band structure of Co1/3NbS2 using both surface and bulk sensitive angle-resolved photoemission spectroscopy. We show that the electronic bands do not fit into the rigid band shift picture after the Co intercalation. Instead, Co1/3NbS2 displays a different orbital character near the Fermi level compared to the pristine NbS2 compound and has a clear band dispersion in the kz direction despite its layered structure. Our photoemission study demonstrates the out-of-plane electronic correlations introduced by the Co intercalation, thus offering a different perspective on this compound. Finally, we propose how Fermi level tuning could lead to exotic phases such as spin density wave instability.},
doi = {10.1103/physrevb.105.l121107},
journal = {Physical Review. B},
number = 12,
volume = 105,
place = {United States},
year = {Mon Mar 14 00:00:00 EDT 2022},
month = {Mon Mar 14 00:00:00 EDT 2022}
}
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