Successive magnetic orderings in the Ising spin chain magnet DyNi5Ge3

Ge, H.; Zhang, L.; Zhao, N.; Yang, J.; Wang, L.; Zhou, L.; Fu, Y.; Li, T. T.; Song, Z. M.; Ding, F.; Xu, J. B.; Zhang, Y. F.; Wang, S. M.; Mei, J. W.; Tong, X.; Miao, P.; He, H.; Zhang, Q.; Wu, L. S.; Sheng, J. M.

doi:10.1103/physrevmaterials.6.085001

Title: Successive magnetic orderings in the Ising spin chain magnet DyNi₅Ge₃

Abstract

In this report, we investigated a new rare-earth-based one-dimensional Ising spin chain magnet DyNi₅Ge₃ by means of magnetization, specific heat, and powder neutron diffraction measurements. Due to the crystalline electrical field splitting, the magnetic Dy ions share an Ising-like ground doublet state. Owning to the local point symmetry, these Ising moments form into two canted magnetic sublattices, which were further confirmed by the angle-dependent magnetization measurement. In zero fields, two successive antiferromagnetic phase transitions were found at temperatures T_N1=6K and T_N2=5K, respectively. Only part of the moments are statically ordered in this intermediate state between T_N1 and T_N2. Powder neutron diffraction experiments at different temperatures were performed as well. Further, an incommensurate magnetic propagation vector of k_m=(0.5,0.4,0.5) was identified. The refined spin configurations through the irreducible representation analysis confirmed that these Ising spins are canted in the crystal ab plane.

Authors:

Ge, H. ^[1];

^[2]; Zhao, N. ^[1]; Yang, J. ^[1]; Wang, L. ^[1]; Zhou, L. ^[1]; Fu, Y. ^[1]; Li, T. T. ^[1]; Song, Z. M. ^[1]; Ding, F. ^[1]; Xu, J. B. ^[1];

^[1]; Wang, S. M. ^[1]; Mei, J. W. ^[3];

^[4];

^[4]; He, H. ^[5];

^[6]; Wu, L. S. ^[1]; Sheng, J. M. ^[1]

Southern University of Science and Technology (SUSTech), Shenzhen (China)
Chinese Academy of Sciences (CAS), Ganzhou (China); Southern University of Science and Technology (SUSTech), Shenzhen (China)
Southern University of Science and Technology (SUSTech), Shenzhen (China); Shenzhen Institute for Quantum Science and Engineering (China)
Chinese Academy of Sciences (CAS), Beijing (China); Spallation Neutron Source Science Center, Dongguan (China)
University of Chinese Academy of Sciences, Beijing (China)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

Publication Date:: Mon Aug 08 00:00:00 EDT 2022

Research Org.:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES); National Natural Science Foundation of China (NSFC); Guangdong Basic and Applied Basic Research Foundation; Guangdong Introducing Innovative and Entrepreneurial Teams; Shenzhen Key Laboratory of Advanced Quantum Functional Materials and Devices

OSTI Identifier:: 1883773

Grant/Contract Number:: AC05-00OR22725; 12134020; 11974157; 11875265; 12104255; 2021B1515120015; 2017ZT07C062; ZDSYS20190902092905285

Resource Type:: Accepted Manuscript

Journal Name:: Physical Review Materials

Additional Journal Information:: Journal Volume: 6; Journal Issue: 8; Journal ID: ISSN 2475-9953

Publisher:: American Physical Society (APS)

Country of Publication:: United States

Language:: English

Subject:: 36 MATERIALS SCIENCE

Citation Formats


                    Ge, H., Zhang, L., Zhao, N., Yang, J., Wang, L., Zhou, L., Fu, Y., Li, T. T., Song, Z. M., Ding, F., Xu, J. B., Zhang, Y. F., Wang, S. M., Mei, J. W., Tong, X., Miao, P., He, H., Zhang, Q., Wu, L. S., and Sheng, J. M. Successive magnetic orderings in the Ising spin chain magnet DyNi5Ge3.  United States: N. p., 2022. 
Web.  doi:10.1103/physrevmaterials.6.085001.

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                    Ge, H., Zhang, L., Zhao, N., Yang, J., Wang, L., Zhou, L., Fu, Y., Li, T. T., Song, Z. M., Ding, F., Xu, J. B., Zhang, Y. F., Wang, S. M., Mei, J. W., Tong, X., Miao, P., He, H., Zhang, Q., Wu, L. S., & Sheng, J. M. Successive magnetic orderings in the Ising spin chain magnet DyNi5Ge3.  United States.  https://doi.org/10.1103/physrevmaterials.6.085001

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                    Ge, H., Zhang, L., Zhao, N., Yang, J., Wang, L., Zhou, L., Fu, Y., Li, T. T., Song, Z. M., Ding, F., Xu, J. B., Zhang, Y. F., Wang, S. M., Mei, J. W., Tong, X., Miao, P., He, H., Zhang, Q., Wu, L. S., and Sheng, J. M. Mon .  
"Successive magnetic orderings in the Ising spin chain magnet DyNi5Ge3".  United States.  https://doi.org/10.1103/physrevmaterials.6.085001.  https://www.osti.gov/servlets/purl/1883773.

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@article{osti_1883773,

  title        = {Successive magnetic orderings in the Ising spin chain magnet DyNi5Ge3},

  author       = {Ge, H. and Zhang, L. and Zhao, N. and Yang, J. and Wang, L. and Zhou, L. and Fu, Y. and Li, T. T. and Song, Z. M. and Ding, F. and Xu, J. B. and Zhang, Y. F. and Wang, S. M. and Mei, J. W. and Tong, X. and Miao, P. and He, H. and Zhang, Q. and Wu, L. S. and Sheng, J. M.},

  abstractNote = {In this report, we investigated a new rare-earth-based one-dimensional Ising spin chain magnet DyNi5Ge3 by means of magnetization, specific heat, and powder neutron diffraction measurements. Due to the crystalline electrical field splitting, the magnetic Dy ions share an Ising-like ground doublet state. Owning to the local point symmetry, these Ising moments form into two canted magnetic sublattices, which were further confirmed by the angle-dependent magnetization measurement. In zero fields, two successive antiferromagnetic phase transitions were found at temperatures TN1=6K and TN2=5K, respectively. Only part of the moments are statically ordered in this intermediate state between TN1 and TN2. Powder neutron diffraction experiments at different temperatures were performed as well. Further, an incommensurate magnetic propagation vector of km=(0.5,0.4,0.5) was identified. The refined spin configurations through the irreducible representation analysis confirmed that these Ising spins are canted in the crystal ab plane.},

  doi          = {10.1103/physrevmaterials.6.085001},

  journal      = {Physical Review Materials},

  number       = 8,

  volume       = 6,

  place        = {United States},

  year         = {Mon Aug 08 00:00:00 EDT 2022},

  month        = {Mon Aug 08 00:00:00 EDT 2022}

}

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Title: Successive magnetic orderings in the Ising spin chain magnet DyNi5Ge3

Abstract

Citation Formats

Spin-stripe phase in a frustrated zigzag spin-1/2 chain journal, June 2015

Quantum Phase Transitions in an Yb-based Semiconductor YbCuS2 with an Effective Spin-1/2 Zigzag Chain journal, September 2020

One-dimensional physics in the 21st century journal, March 2016

Realization of the kagome spin ice state in a frustrated intermetallic compound journal, March 2020

Magnetic ground state of the Ising-like antiferromagnet DyScO 3 journal, October 2017

Orbital-exchange and fractional quantum number excitations in an f-electron metal, Yb 2 Pt 2 Pb journal, June 2016

Topological quantum phase transition in the Ising-like antiferromagnetic spin chain BaCo2V2O8 journal, May 2018

Multispinon Continua at Zero and Finite Temperature in a Near-Ideal Heisenberg Chain journal, September 2013

Hierarchy of Bound States in the One-Dimensional Ferromagnetic Ising Chain CoNb 2 O 6 Investigated by High-Resolution Time-Domain Terahertz Spectroscopy journal, April 2014

Magnetic, electrical and thermodynamic properties of CePd5Ge3 journal, January 2001

Recent advances in magnetic structure determination by neutron powder diffraction journal, October 1993

Magnetization Process of Atacamite: A Case of Weakly Coupled S=1/2 Sawtooth Chains journal, May 2021

Dispersions of many-body Bethe strings journal, April 2020

Metamagnetism in CePd 5 Ge 3 journal, February 2013

Magnetic transitions in the 1D chain compounds NdPd 5 Ge 3 and NdPt 5 Ge 3 journal, August 2021

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Antiferromagnetic ordering and dipolar interactions of YbAlO 3 journal, May 2019

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What is the spin of a spin wave? journal, October 1981

Quantum Criticality in an Ising Chain: Experimental Evidence for Emergent E 8 Symmetry journal, January 2010

The magnetic structures of DyNi2Ge2 journal, October 1998

Magnetic field tuning of antiferromagnetic Yb 3 Pt 4 journal, October 2011

From confined spinons to emergent fermions: Observation of elementary magnetic excitations in a transverse-field Ising chain journal, September 2016

Evidence for low-dimensional magnetic behaviour in CePt5Ge3 journal, May 2001

Spinon confinement in the one-dimensional Ising-like antiferromagnet SrCo 2 V 2 O 8 journal, April 2015

Quantum Criticality of the Ising-like Screw Chain Antiferromagnet SrCo 2 V 2 O 8 in a Transverse Magnetic Field journal, August 2019

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Novel Longitudinal Mode in the Coupled Quantum Chain Compound KCuF 3 journal, July 2000

Confinement of fractional quantum number particles in a condensed-matter system journal, November 2009

Title: Successive magnetic orderings in the Ising spin chain magnet DyNi₅Ge₃

Spin-stripe phase in a frustrated zigzag spin-1/2 chain
journal, June 2015

Quantum Phase Transitions in an Yb-based Semiconductor YbCuS₂ with an Effective Spin-1/2 Zigzag Chain
journal, September 2020

One-dimensional physics in the 21st century
journal, March 2016

Realization of the kagome spin ice state in a frustrated intermetallic compound
journal, March 2020

Magnetic ground state of the Ising-like antiferromagnet ${DyScO}_{3}$
journal, October 2017

Orbital-exchange and fractional quantum number excitations in an f-electron metal, Yb ₂ Pt ₂ Pb
journal, June 2016

Topological quantum phase transition in the Ising-like antiferromagnetic spin chain BaCo2V2O8
journal, May 2018

Multispinon Continua at Zero and Finite Temperature in a Near-Ideal Heisenberg Chain
journal, September 2013

Hierarchy of Bound States in the One-Dimensional Ferromagnetic Ising Chain ${CoNb}_{2} O_{6}$ Investigated by High-Resolution Time-Domain Terahertz Spectroscopy
journal, April 2014

Magnetic, electrical and thermodynamic properties of CePd5Ge3
journal, January 2001

Recent advances in magnetic structure determination by neutron powder diffraction
journal, October 1993

Magnetization Process of Atacamite: A Case of Weakly Coupled S=1/2 Sawtooth Chains
journal, May 2021

Dispersions of many-body Bethe strings
journal, April 2020

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journal, February 2013

Magnetic transitions in the 1D chain compounds NdPd ₅ Ge ₃ and NdPt ₅ Ge ₃
journal, August 2021

Heat transport by lattice and spin excitations in the spin-chain compounds ${SrCuO}_{2}$ and ${Sr}_{2} {CuO}_{3}$
journal, July 2001

Magnetization Plateaus in Spin Chains: “Haldane Gap” for Half-Integer Spins
journal, March 1997

Antiferromagnetic ordering and dipolar interactions of ${YbAlO}_{3}$
journal, May 2019

Quantum Criticality of an Ising-like Spin- $1 / 2$ Antiferromagnetic Chain in a Transverse Magnetic Field
journal, May 2018

Experimental observation of Bethe strings
journal, February 2018

Magnetic order of CePd5Ge3 and CePt5Ge3
journal, May 2004

Magnetic structures of RNi2Ge2 (R = Dy, Ho and Er) and YbNi2Si2
journal, July 1995

What is the spin of a spin wave?
journal, October 1981

Quantum Criticality in an Ising Chain: Experimental Evidence for Emergent E ₈ Symmetry
journal, January 2010

The magnetic structures of DyNi2Ge2
journal, October 1998

Magnetic field tuning of antiferromagnetic Yb $_{3}$ Pt $_{4}$
journal, October 2011

From confined spinons to emergent fermions: Observation of elementary magnetic excitations in a transverse-field Ising chain
journal, September 2016

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journal, May 2001

Spinon confinement in the one-dimensional Ising-like antiferromagnet ${SrCo}_{2} V_{2} O_{8}$
journal, April 2015

Quantum Criticality of the Ising-like Screw Chain Antiferromagnet ${SrCo}_{2} V_{2} O_{8}$ in a Transverse Magnetic Field
journal, August 2019

Tomonaga–Luttinger liquid behavior and spinon confinement in YbAlO3
journal, February 2019

Zur Theorie der Metalle: I. Eigenwerte und Eigenfunktionen der linearen Atomkette
journal, March 1931

An Exactly Soluble Model of a Many‐Fermion System
journal, September 1963

Novel Longitudinal Mode in the Coupled Quantum Chain Compound ${KCuF}_{3}$
journal, July 2000

Confinement of fractional quantum number particles in a condensed-matter system
journal, November 2009