Direct measurement of 59Ni(n, p) 59Co and 59Ni(n, α) 56Fe at fast-neutron energies from 500 keV to 10 MeV
Abstract
We report nuclear reaction data for neutron induced reactions on unstable nuclei are critical for a wide range of applications spanning studies of nuclear astrophysics, nuclear reactor designs, and radiochemistry diagnostics. However, nuclear data evaluations of the reaction cross sections are largely based on calculations due to the difficulty in performing this class of measurements and the resulting lack of experimental data. For neutron induced charged particle reactions at fast neutron energies, at the MeV scale, these cross section predictions are predominately driven by statistical Hauser-Feshbach calculations. In this work, we present partial and total 59Ni(n, p) and 59Ni(n, α) cross sections, measured directly with a radioactive 59Ni target, and compare the results to the present nuclear data evaluations. In addition, the results from this work are compared to a recent study of the 59Ni(n, xp) reaction cross section that was performed via an indirect surrogate ratio method. The expected energy trend of the cross section, based on the current work, is inconsistent with that of the surrogate work. This calls into question the reliability of that application of the surrogate ratio method and highlights the need for direct measurements on unstable nuclei, when feasible.
- Authors:
-
- Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
- Central Michigan Univ., Mount Pleasant, MI (United States)
- Korean Atomic Energy Reseach Institute, Daejeon (Korea, Republic of)
- Publication Date:
- Research Org.:
- Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
- Sponsoring Org.:
- USDOE National Nuclear Security Administration (NNSA); USDOE Laboratory Directed Research and Development (LDRD) Program; Korean Atomic Energy Research Institute (KAERI)
- OSTI Identifier:
- 1866958
- Report Number(s):
- LA-UR-21-25101
Journal ID: ISSN 2469-9985; TRN: US2306116
- Grant/Contract Number:
- 89233218CNA000001; NRF-2020M2A8A1000930
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Physical Review. C
- Additional Journal Information:
- Journal Volume: 105; Journal Issue: 4; Journal ID: ISSN 2469-9985
- Publisher:
- American Physical Society (APS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 73 NUCLEAR PHYSICS AND RADIATION PHYSICS; models; methods for nuclear reactions; neutron physics; nuclear reactions; nucleon induced nuclear reactions
Citation Formats
Kuvin, Sean Andrew, Lee, Hye Young, Birnbaum, Eva R., DiGiovine, Brad Joseph, Eiroa Lledo, Cecilia, Georgiadou, Anastasia, Herman, Michal W., Kawano, Toshihiko, Mocko, Veronika, Mosby, Shea Morgan, Vermeulen, Christiaan, Votaw, Daniel Gregory Jenks, Zavorka, Lukas, Perdikakis, Georgios, Tsintari, Pelagia, and Kim, Hyeong-il. Direct measurement of 59Ni(n, p) 59Co and 59Ni(n, α) 56Fe at fast-neutron energies from 500 keV to 10 MeV. United States: N. p., 2022.
Web. doi:10.1103/physrevc.105.044608.
Kuvin, Sean Andrew, Lee, Hye Young, Birnbaum, Eva R., DiGiovine, Brad Joseph, Eiroa Lledo, Cecilia, Georgiadou, Anastasia, Herman, Michal W., Kawano, Toshihiko, Mocko, Veronika, Mosby, Shea Morgan, Vermeulen, Christiaan, Votaw, Daniel Gregory Jenks, Zavorka, Lukas, Perdikakis, Georgios, Tsintari, Pelagia, & Kim, Hyeong-il. Direct measurement of 59Ni(n, p) 59Co and 59Ni(n, α) 56Fe at fast-neutron energies from 500 keV to 10 MeV. United States. https://doi.org/10.1103/physrevc.105.044608
Kuvin, Sean Andrew, Lee, Hye Young, Birnbaum, Eva R., DiGiovine, Brad Joseph, Eiroa Lledo, Cecilia, Georgiadou, Anastasia, Herman, Michal W., Kawano, Toshihiko, Mocko, Veronika, Mosby, Shea Morgan, Vermeulen, Christiaan, Votaw, Daniel Gregory Jenks, Zavorka, Lukas, Perdikakis, Georgios, Tsintari, Pelagia, and Kim, Hyeong-il. Mon .
"Direct measurement of 59Ni(n, p) 59Co and 59Ni(n, α) 56Fe at fast-neutron energies from 500 keV to 10 MeV". United States. https://doi.org/10.1103/physrevc.105.044608. https://www.osti.gov/servlets/purl/1866958.
@article{osti_1866958,
title = {Direct measurement of 59Ni(n, p) 59Co and 59Ni(n, α) 56Fe at fast-neutron energies from 500 keV to 10 MeV},
author = {Kuvin, Sean Andrew and Lee, Hye Young and Birnbaum, Eva R. and DiGiovine, Brad Joseph and Eiroa Lledo, Cecilia and Georgiadou, Anastasia and Herman, Michal W. and Kawano, Toshihiko and Mocko, Veronika and Mosby, Shea Morgan and Vermeulen, Christiaan and Votaw, Daniel Gregory Jenks and Zavorka, Lukas and Perdikakis, Georgios and Tsintari, Pelagia and Kim, Hyeong-il},
abstractNote = {We report nuclear reaction data for neutron induced reactions on unstable nuclei are critical for a wide range of applications spanning studies of nuclear astrophysics, nuclear reactor designs, and radiochemistry diagnostics. However, nuclear data evaluations of the reaction cross sections are largely based on calculations due to the difficulty in performing this class of measurements and the resulting lack of experimental data. For neutron induced charged particle reactions at fast neutron energies, at the MeV scale, these cross section predictions are predominately driven by statistical Hauser-Feshbach calculations. In this work, we present partial and total 59Ni(n, p) and 59Ni(n, α) cross sections, measured directly with a radioactive 59Ni target, and compare the results to the present nuclear data evaluations. In addition, the results from this work are compared to a recent study of the 59Ni(n, xp) reaction cross section that was performed via an indirect surrogate ratio method. The expected energy trend of the cross section, based on the current work, is inconsistent with that of the surrogate work. This calls into question the reliability of that application of the surrogate ratio method and highlights the need for direct measurements on unstable nuclei, when feasible.},
doi = {10.1103/physrevc.105.044608},
journal = {Physical Review. C},
number = 4,
volume = 105,
place = {United States},
year = {Mon Apr 11 00:00:00 EDT 2022},
month = {Mon Apr 11 00:00:00 EDT 2022}
}
Works referenced in this record:
ENDF/B-VIII.0: The 8 th Major Release of the Nuclear Reaction Data Library with CIELO-project Cross Sections, New Standards and Thermal Scattering Data
journal, February 2018
- Brown, D. A.; Chadwick, M. B.; Capote, R.
- Nuclear Data Sheets, Vol. 148
JENDL-4.0: A New Library for Nuclear Science and Engineering
journal, January 2011
- Shibata, Keiichi; Iwamoto, Osamu; Nakagawa, Tsuneo
- Journal of Nuclear Science and Technology, Vol. 48, Issue 1
Particle identification by pulse shape discrimination in the p-i-n type semiconductor detector
journal, March 1963
- Ammerlaan, C. A. J.; Rumphorst, R. F.; Koerts, L. A. Ch.
- Nuclear Instruments and Methods, Vol. 22
Towards a More Complete and Accurate Experimental Nuclear Reaction Data Library (EXFOR): International Collaboration Between Nuclear Reaction Data Centres (NRDC)
journal, June 2014
- Otuka, N.; Dupont, E.; Semkova, V.
- Nuclear Data Sheets, Vol. 120
Modern Nuclear Data Evaluation with the TALYS Code System
journal, December 2012
- Koning, A. J.; Rochman, D.
- Nuclear Data Sheets, Vol. 113, Issue 12
RIPL – Reference Input Parameter Library for Calculation of Nuclear Reactions and Nuclear Data Evaluations
journal, December 2009
- Capote, R.; Herman, M.; Obložinský, P.
- Nuclear Data Sheets, Vol. 110, Issue 12
The Los Alamos National Laboratory Spallation Neutron Sources
journal, October 1990
- Lisowski, P. W.; Bowman, C. D.; Russell, G. J.
- Nuclear Science and Engineering, Vol. 106, Issue 2
A technique for the study of (p,n) reactions with unstable isotopes at energies relevant to astrophysics
journal, January 2021
- Gastis, P.; Perdikakis, G.; Berg, G. P. A.
- Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 985
The (n, α) Reaction in the s-process Branching Point 59Ni
journal, June 2014
- Weiß, C.; Guerrero, C.; Griesmayer, E.
- Nuclear Data Sheets, Vol. 120
Local and global nucleon optical models from 1 keV to 200 MeV
journal, January 2003
- Koning, A. J.; Delaroche, J. P.
- Nuclear Physics A, Vol. 713, Issue 3-4
Hydrogen generation arising from the59Ni(n, p) reaction and its impact on fission—fusion correlations
journal, October 1996
- Greenwood, L. R.; Garner, F. A.
- Journal of Nuclear Materials, Vol. 233-237
New evaluation on angular distributions and energy spectra for neutron-induced charged-particle measurements
journal, May 2020
- Kim, H. I.; Lee, H. Y.; Kawano, T.
- Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 963
Determination of reaction cross sections using surrogate reactions
journal, January 2019
- Pandey, Jyoti; Pandey, Bhawna; Pal, A.
- Physical Review C, Vol. 99, Issue 1
A holistic approach to the optimization of neutron beam transport at the LANSCE facility
journal, October 2021
- DiGiovine, B.; Zavorka, L.; Ballard, D. J.
- Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 1013
Pulse shape discrimination of charged particles with a silicon strip detector
journal, October 2001
- Lu, J.; Figuera, P.; Amorini, F.
- Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 471, Issue 3
A fission ionization detector for neutron flux measurements at a spallation source
journal, November 1993
- Wender, S. A.; Balestrini, S.; Brown, A.
- Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 336, Issue 1-2
The Effect of Irradiation on Ni-Containing Components in CANDU ® Reactor Cores: A Review
journal, June 2013
- Griffiths, M.
- AECL Nuclear Review, Vol. 2, Issue 1
Verification of the surrogate ratio method
journal, April 2010
- Chiba, Satoshi; Iwamoto, Osamu
- Physical Review C, Vol. 81, Issue 4
Compound-nuclear reaction cross sections from surrogate measurements
journal, March 2012
- Escher, Jutta E.; Burke, Jason T.; Dietrich, Frank S.
- Reviews of Modern Physics, Vol. 84, Issue 1
Nonstatistical fluctuations in the reaction cross section at fast-neutron energies from 0.6 to 6 MeV
journal, August 2020
- Kuvin, S. A.; Lee, H. Y.; Kawano, T.
- Physical Review C, Vol. 102, Issue 2
Identification of light charged particles and heavy ions in silicon detectors by means of pulse-shape discrimination
journal, June 1996
- Pausch, G.; Ortlepp, H. -G.; Bohne, W.
- IEEE Transactions on Nuclear Science, Vol. 43, Issue 3
Uncertainty-driven nuclear data evaluation including thermal (n, α ) applied to 59 Ni
journal, November 2017
- Helgesson, P.; Sjöstrand, H.; Rochman, D.
- Nuclear Data Sheets, Vol. 145
Measurements of the 59 Ni( n,α ) Cross Section for Thermal Neutrons
journal, January 1974
- Eiland, H. M.; Kirouac, G. J.
- Nuclear Science and Engineering, Vol. 53, Issue 1
Entrance channel effects on the alpha decay probabilities of neutron and proton induced reactions for target mass A=55
journal, August 2020
- Hlondo, L. R.; Lalremruata, B.
- Nuclear Physics A, Vol. 1000
The joint evaluated fission and fusion nuclear data library, JEFF-3.3
journal, July 2020
- Plompen, A. J. M.; Cabellos, O.; De Saint Jean, C.
- The European Physical Journal A, Vol. 56, Issue 7
Complementary optical-potential analysis of -particle elastic scattering and induced reactions at low energies
journal, July 2009
- Avrigeanu, M.; Obreja, A. C.; Roman, F. L.
- Atomic Data and Nuclear Data Tables, Vol. 95, Issue 4
Geant4—a simulation toolkit
journal, July 2003
- Agostinelli, S.; Allison, J.; Amako, K.
- Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 506, Issue 3
DART, a BCA Code to Assess and Compare Primary Irradiation Damage in Nuclear Materials Submitted to Neutron and Ion Flux
journal, January 2016
- Luneville, Laurence; Simeone, David
- EPJ Web of Conferences, Vol. 115
Validation of neutron-induced reactions on natural carbon using an active target at neutron energies up to 22 MeV at LANSCE
journal, July 2021
- Kuvin, S. A.; Lee, H. Y.; DiGiovine, B.
- Physical Review C, Vol. 104, Issue 1
The Inelastic Scattering of Neutrons
journal, July 1952
- Hauser, Walter; Feshbach, Herman
- Physical Review, Vol. 87, Issue 2
16 O(n, α ) cross section investigation using LENZ instrument at LANSCE
journal, January 2016
- Lee, H. Y.; Mosby, S.; Haight, R. C.
- EPJ Web of Conferences, Vol. 122