Oxygen Loss in Layered Oxide Cathodes for Li-Ion Batteries: Mechanisms, Effects, and Mitigation

Zhang, Hanlei; Liu, Hao; Piper, Louis F. J.; Whittingham, M. Stanley; Zhou, Guangwen

doi:10.1021/acs.chemrev.1c00327

Title: Oxygen Loss in Layered Oxide Cathodes for Li-Ion Batteries: Mechanisms, Effects, and Mitigation

Journal Article · 12 January 2022 · Chemical Reviews

DOI: https://doi.org/10.1021/acs.chemrev.1c00327 · OSTI ID:1864774

Zhang, Hanlei ^[1];

^[2]; Piper, Louis F. J. ^[3];

^[2];

^[2]

State Univ. of New York (SUNY), Binghamton, NY (United States); SUNY Binghamton
State Univ. of New York (SUNY), Binghamton, NY (United States)
State Univ. of New York (SUNY), Binghamton, NY (United States); Univ. of Warwick, Coventry (United Kingdom)

Layered lithium transition metal oxides derived from LiMO₂ (M = Co, Ni, Mn, etc.) have been widely adopted as the cathodes of Li-ion batteries for portable electronics, electric vehicles, and energy storage. Oxygen loss in the layered oxides is one of the major factors leading to cycling-induced structural degradation and its associated fade in electrochemical performance. Herein, we review recent progress in understanding the phenomena of oxygen loss and the resulting structural degradation in layered oxide cathodes. We first present the major driving forces leading to the oxygen loss and then describe the associated structural degradation resulting from the oxygen loss. Here, we follow this analysis with a discussion of the kinetic pathways that enable oxygen loss, and then we address the resulting electrochemical fade. Finally, we review the possible approaches toward mitigating oxygen loss and the associated electrochemical fade as well as detail novel analytical methods for probing the oxygen loss.

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Research Organization:: State Univ. of New York (SUNY), Binghamton, NY (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: SC0012583

OSTI ID:: 1864774

Journal Information:: Chemical Reviews, Journal Name: Chemical Reviews Journal Issue: 6 Vol. 122; ISSN 0009-2665

Publisher:: American Chemical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

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Long-Term Low-Rate Cycling of LiCoO ₂ /Graphite Li-Ion Cells at 55°C Smith, A. J.; Dahn, Hannah M.; Burns, J. C. Journal of The Electrochemical Society, Vol. 159, Issue 6 https://doi.org/10.1149/2.056206jes	journal	January 2012
Analysis of Rate-Limiting Factors in Thick Electrodes for Electric Vehicle Applications Lee, Byoung-Sun; Wu, Zhaohui; Petrova, Victoria Journal of The Electrochemical Society, Vol. 165, Issue 3 https://doi.org/10.1149/2.0571803jes	journal	January 2018
Changing of SEI Film and Electrochemical Properties about MCMB Electrodes during Long-Term Charge/Discharge Cycles Yang, Lijie; Cheng, Xinqun; Ma, Yulin Journal of The Electrochemical Society, Vol. 160, Issue 11 https://doi.org/10.1149/2.064311jes	journal	January 2013
Correlative Microscopy-Based Approach for Analyzing Microscopic Impurities in Carbon Black for Lithium-Ion Battery Applications Poozhikunnath, Abhinav; Favata, Joseph; Ahmadi, Bahar Journal of The Electrochemical Society, Vol. 166, Issue 14 https://doi.org/10.1149/2.0761914jes	journal	January 2019
Decomposition of LiPF ₆ in High Energy Lithium-Ion Batteries Studied with Online Electrochemical Mass Spectrometry Guéguen, Aurélie; Streich, Daniel; He, Minglong Journal of The Electrochemical Society, Vol. 163, Issue 6 https://doi.org/10.1149/2.0981606jes	journal	January 2016
A Wide Range of Testing Results on an Excellent Lithium-Ion Cell Chemistry to be used as Benchmarks for New Battery Technologies Harlow, Jessie E.; Ma, Xiaowei; Li, Jing Journal of The Electrochemical Society, Vol. 166, Issue 13 https://doi.org/10.1149/2.0981913jes	journal	January 2019
The Role of Oxygen Release from Li- and Mn-Rich Layered Oxides during the First Cycles Investigated by On-Line Electrochemical Mass Spectrometry Strehle, Benjamin; Kleiner, Karin; Jung, Roland Journal of The Electrochemical Society, Vol. 164, Issue 2 https://doi.org/10.1149/2.1001702jes	journal	December 2016
Enhanced Electrochemical Performance of Li _1.2 Mn _0.54 Ni _0.13 Co _0.13 O ₂ via L-Ascorbic Acid-Based Treatment as Cathode Material for Li-Ion Batteries Pang, Shengli; Zhu, Meng; Xu, Kaijie Journal of The Electrochemical Society, Vol. 165, Issue 9 https://doi.org/10.1149/2.1481809jes	journal	January 2018
Understanding the structure and structural degradation mechanisms in high-voltage, lithium-manganese–rich lithium-ion battery cathode oxides: A review of materials diagnostics Mohanty, Debasish; Li, Jianlin; Nagpure, Shrikant C. MRS Energy & Sustainability, Vol. 2 https://doi.org/10.1557/mre.2015.16	journal	January 2015
X-Ray Determination of Electron-Density Distributions in Oxides, MgO, MnO, CoO, and NiO, and Atomic Scattering Factors of their Constituent Atoms Sasaki, Satoshi; Fujino, Kiyoshi; TakÉUchi, Yoshio Proceedings of the Japan Academy. Ser. B: Physical and Biological Sciences, Vol. 55, Issue 2 https://doi.org/10.2183/pjab.55.43	journal	January 1979
The Formation, Detriment and Solution of Residual Lithium Compounds on Ni-Rich Layered Oxides in Lithium-Ion Batteries Chen, Anqi; Wang, Kun; Li, Jiaojiao Frontiers in Energy Research, Vol. 8 https://doi.org/10.3389/fenrg.2020.593009	journal	December 2020
Application of Operando X-ray Diffractometry in Various Aspects of the Investigations of Lithium/Sodium-Ion Batteries Zhu, Wen; Wang, Yuesheng; Liu, Dongqiang Energies, Vol. 11, Issue 11 https://doi.org/10.3390/en11112963	journal	November 2018
A Bottom-Up Approach to Lithium-Ion Battery Cost Modeling with a Focus on Cathode Active Materials Wentker, Marc; Greenwood, Matthew; Leker, Jens Energies, Vol. 12, Issue 3 https://doi.org/10.3390/en12030504	journal	February 2019
Comparative Issues of Cathode Materials for Li-Ion Batteries Julien, Christian; Mauger, Alain; Zaghib, Karim Inorganics, Vol. 2, Issue 1 https://doi.org/10.3390/inorganics2010132	journal	March 2014
Optimization of Layered Cathode Materials for Lithium-Ion Batteries Julien, Christian; Mauger, Alain; Zaghib, Karim Materials, Vol. 9, Issue 7 https://doi.org/10.3390/ma9070595	journal	July 2016
Lithium Ion Battery Fire And Explosion Wang, Q.; Sun, J.; Chu, Guanquan Fire Safety Science, Vol. 8 https://doi.org/10.3801/IAFSS.FSS.8-375	journal	January 2005

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