Effect of water vapor on high-temperature oxidation of NiAl alloy

Zhu, Dingding; Wang, Xinli; Zhao, Jun; Lu, Jian; Zhou, Yichun; Cai, Canying; Huang, Jianyu; Zhou, Guangwen

doi:10.1016/j.corsci.2020.108963

Title: Effect of water vapor on high-temperature oxidation of NiAl alloy

Journal Article · Fri Aug 28 00:00:00 UTC 2020 · Corrosion Science

DOI: https://doi.org/10.1016/j.corsci.2020.108963 · OSTI ID:1850716

Zhu, Dingding ^[1]; Wang, Xinli ^[2]; Zhao, Jun ^[3]; Lu, Jian ^[4]; Zhou, Yichun ^[2]; Cai, Canying ^[2]; Huang, Jianyu ^[5]; Zhou, Guangwen ^[6]

Xiangtan Univ. (China). School of Materials Science and Engineering; State Univ. of New York (SUNY), Binghamton, NY (United States)
Xiangtan Univ. (China). School of Materials Science and Engineering
Yanshan Univ., Qinhuangdao (China). State Key Lab. of Metastable Materials Science and Technology. Clean Nano Energy Center
City Univ. of Hong Kong, Kowloon (Hong Kong). Dept. of Mechanical Engineering; City Univ. of Hong Kong Shenzhen Research Inst., Shenzhen (China). Center for Advanced Structural Materials
Xiangtan Univ. (China). School of Materials Science and Engineering; Yanshan Univ., Qinhuangdao (China). State Key Lab. of Metastable Materials Science and Technology. Clean Nano Energy Center
State Univ. of New York (SUNY), Binghamton, NY (United States). Dept. of Mechanical Engineering & Materials Science. Engineering Program

The high-temperature oxidation of NiAl is studied with dry oxygen and water vapor. The oxidation in H₂O results in a thicker Al₂O₃ oxide scale than that in O₂. The oxide scale formed initially is a single layer of γ-Al₂O₃ that subsequently transforms into a α-Al₂O₃/γ-Al₂O₃ bilayer structure, in which the inner α-Al2O3 layer formed in H2O has a higher porosity than that in O₂. Finally, further density functional theory calculations show that H protons derived from H₂O molecules penetrate into the oxide lattice and boost the formation of lattice vacancies in both α-Al₂O₃ and γ-Al₂O₃, thus enhancing the oxide scale growth.

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Research Organization:: State Univ. of New York (SUNY), Albany, NY (United States)

Sponsoring Organization:: National Key R&D Program of China; National Natural Science Foundation of China (NSFC); USDOE Office of Science (SC)

Grant/Contract Number:: SC0001135

OSTI ID:: 1850716

Journal Information:: Corrosion Science, Journal Name: Corrosion Science Journal Issue: C Vol. 177; ISSN 0010-938X

Publisher:: ElsevierCopyright Statement

Country of Publication:: United States

Language:: English

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Title: Effect of water vapor on high-temperature oxidation of NiAl alloy

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