A historical overview of the activation and porosity of metal–organic frameworks
Abstract
Since the first reports of metal–organic frameworks (MOFs), this unique class of crystalline, porous materials has garnered increasing attention in a wide variety of applications such as gas storage and separation, catalysis, enzyme immobilization, drug delivery, water capture, and sensing. A fundamental feature of MOFs is their porosity which provides space on the micro- and meso-scale for confining and exposing their functionalities. Therefore, designing MOFs with high porosity and developing suitable activation methods for preserving and accessing their pore space have been a common theme in MOF research. Reticular chemistry allows for the facile design of MOFs from highly tunable metal nodes and organic linkers in order to realize different pore structures, topologies, and functionalities. With the hope of shedding light on future research endeavors in MOF porosity, it is worthwhile to examine the development of MOFs, with an emphasis on their porosity and how to properly access their pore space. In this review, we will provide an overview of the historic evolution of porosity and activation of MOFs, followed by a synopsis of the strategies to design and preserve permanent porosity in MOFs.
- Authors:
-
- Northwestern Univ., Evanston, IL (United States)
- Northwestern Univ., Evanston, IL (United States); Jilin Univ., Changchun (China)
- Iran Univ. of Science and Technology, Tehran (Iran)
- Fudan Univ., Shanghai (China)
- Publication Date:
- Research Org.:
- Northwestern Univ., Evanston, IL (United States); Univ. of Notre Dame, IN (United States)
- Sponsoring Org.:
- USDOE Office of Energy Efficiency and Renewable Energy (EERE); USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE National Nuclear Security Administration (NNSA)
- OSTI Identifier:
- 1848894
- Alternate Identifier(s):
- OSTI ID: 1664494
- Grant/Contract Number:
- EE0008816; FG02-03ER15457; FG02-08ER15967; NA0003763
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Chemical Society Reviews
- Additional Journal Information:
- Journal Volume: 49; Journal Issue: 20; Journal ID: ISSN 0306-0012
- Publisher:
- Royal Society of Chemistry
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY
Citation Formats
Zhang, Xuan, Chen, Zhijie, Liu, Xinyao, Hanna, Sylvia L., Wang, Xingjie, Taheri-Ledari, Reza, Maleki, Ali, Li, Peng, and Farha, Omar K. A historical overview of the activation and porosity of metal–organic frameworks. United States: N. p., 2020.
Web. doi:10.1039/d0cs00997k.
Zhang, Xuan, Chen, Zhijie, Liu, Xinyao, Hanna, Sylvia L., Wang, Xingjie, Taheri-Ledari, Reza, Maleki, Ali, Li, Peng, & Farha, Omar K. A historical overview of the activation and porosity of metal–organic frameworks. United States. https://doi.org/10.1039/d0cs00997k
Zhang, Xuan, Chen, Zhijie, Liu, Xinyao, Hanna, Sylvia L., Wang, Xingjie, Taheri-Ledari, Reza, Maleki, Ali, Li, Peng, and Farha, Omar K. Mon .
"A historical overview of the activation and porosity of metal–organic frameworks". United States. https://doi.org/10.1039/d0cs00997k. https://www.osti.gov/servlets/purl/1848894.
@article{osti_1848894,
title = {A historical overview of the activation and porosity of metal–organic frameworks},
author = {Zhang, Xuan and Chen, Zhijie and Liu, Xinyao and Hanna, Sylvia L. and Wang, Xingjie and Taheri-Ledari, Reza and Maleki, Ali and Li, Peng and Farha, Omar K.},
abstractNote = {Since the first reports of metal–organic frameworks (MOFs), this unique class of crystalline, porous materials has garnered increasing attention in a wide variety of applications such as gas storage and separation, catalysis, enzyme immobilization, drug delivery, water capture, and sensing. A fundamental feature of MOFs is their porosity which provides space on the micro- and meso-scale for confining and exposing their functionalities. Therefore, designing MOFs with high porosity and developing suitable activation methods for preserving and accessing their pore space have been a common theme in MOF research. Reticular chemistry allows for the facile design of MOFs from highly tunable metal nodes and organic linkers in order to realize different pore structures, topologies, and functionalities. With the hope of shedding light on future research endeavors in MOF porosity, it is worthwhile to examine the development of MOFs, with an emphasis on their porosity and how to properly access their pore space. In this review, we will provide an overview of the historic evolution of porosity and activation of MOFs, followed by a synopsis of the strategies to design and preserve permanent porosity in MOFs.},
doi = {10.1039/d0cs00997k},
journal = {Chemical Society Reviews},
number = 20,
volume = 49,
place = {United States},
year = {Mon Sep 21 00:00:00 EDT 2020},
month = {Mon Sep 21 00:00:00 EDT 2020}
}
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