Systematic extraction of crystal electric-field effects and quantum magnetic model parameters in triangular rare-earth magnets

Pocs, Christopher A.; Siegfried, Peter E.; Xing, Jie; Sefat, Athena S.; Hermele, Michael; Normand, B.; Lee, Minhyea

doi:10.1103/PhysRevResearch.3.043202

Title: Systematic extraction of crystal electric-field effects and quantum magnetic model parameters in triangular rare-earth magnets

Authors:

Pocs, Christopher A.; Siegfried, Peter E.; Xing, Jie; Sefat, Athena S.; Hermele, Michael; Normand, B.;

Publication Date:: Tue Dec 21 00:00:00 EST 2021

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

OSTI Identifier:: 1836871

Resource Type:: Published Article

Journal Name:: Physical Review Research

Additional Journal Information:: Journal Name: Physical Review Research Journal Volume: 3 Journal Issue: 4; Journal ID: ISSN 2643-1564

Publisher:: American Physical Society

Country of Publication:: United States

Language:: English

Citation Formats


                    Pocs, Christopher A., Siegfried, Peter E., Xing, Jie, Sefat, Athena S., Hermele, Michael, Normand, B., and Lee, Minhyea. Systematic extraction of crystal electric-field effects and quantum magnetic model parameters in triangular rare-earth magnets.  United States: N. p., 2021. 
Web.  doi:10.1103/PhysRevResearch.3.043202.

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                    Pocs, Christopher A., Siegfried, Peter E., Xing, Jie, Sefat, Athena S., Hermele, Michael, Normand, B., & Lee, Minhyea. Systematic extraction of crystal electric-field effects and quantum magnetic model parameters in triangular rare-earth magnets.  United States.  https://doi.org/10.1103/PhysRevResearch.3.043202

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                    Pocs, Christopher A., Siegfried, Peter E., Xing, Jie, Sefat, Athena S., Hermele, Michael, Normand, B., and Lee, Minhyea. Tue .  
"Systematic extraction of crystal electric-field effects and quantum magnetic model parameters in triangular rare-earth magnets".  United States.  https://doi.org/10.1103/PhysRevResearch.3.043202.

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@article{osti_1836871,

  title        = {Systematic extraction of crystal electric-field effects and quantum magnetic model parameters in triangular rare-earth magnets},

  author       = {Pocs, Christopher A. and Siegfried, Peter E. and Xing, Jie and Sefat, Athena S. and Hermele, Michael and Normand, B. and Lee, Minhyea},

  abstractNote = {},

  doi          = {10.1103/PhysRevResearch.3.043202},

  journal      = {Physical Review Research},

  number       = 4,

  volume       = 3,

  place        = {United States},

  year         = {Tue Dec 21 00:00:00 EST 2021},

  month        = {Tue Dec 21 00:00:00 EST 2021}

}

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Title: Systematic extraction of crystal electric-field effects and quantum magnetic model parameters in triangular rare-earth magnets

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Spin Dynamics of the Spin- 1 / 2 Kagome Lattice Antiferromagnet ZnCu 3 ( OH ) 6 Cl 2 journal, March 2007

Magnetism driven by the interplay of fluctuations and frustration in the easy-axis triangular XXZ model with transverse fields journal, October 2019

Quantum Spin Ice Dynamics in the Dipole-Octupole Pyrochlore Magnet Ce 2 Zr 2 O 7 journal, May 2019

Crystal-field Hamiltonian and anisotropy in KErSe 2 and CsErSe 2 journal, April 2020

Lattice dynamics and coupled quadrupole-phonon excitations in CeAuAl 3 journal, November 2018

Mermin-Wagner physics, ( H , T ) phase diagram, and candidate quantum spin-liquid phase in the spin- 1 2 triangular-lattice antiferromagnet Ba 8 CoNb 6 O 24 journal, April 2018

Symmetry enriched U(1) topological orders for dipole-octupole doublets on a pyrochlore lattice journal, January 2017

Dirac Spin Liquid on the Spin- 1 / 2 Triangular Heisenberg Antiferromagnet journal, November 2019

Crystalline electric field excitations in the quantum spin liquid candidate NaYbSe 2 journal, January 2021

Spin liquids in geometrically perfect triangular antiferromagnets journal, March 2020

Determination of effective microscopic models for the frustrated antiferromagnets Cs 2 CuCl 4 and Cs 2 CuBr 4 by density functional methods journal, March 2011

Static and Dynamical Properties of the Spin- 1 / 2 Equilateral Triangular-Lattice Antiferromagnet Ba 3 CoSb 2 O 9 journal, February 2016

Topography of Spin Liquids on a Triangular Lattice journal, May 2018

Magnetic pyrochlore oxides journal, January 2010

Dipolar-octupolar Ising antiferromagnetism in Sm 2 Ti 2 O 7 : A moment fragmentation candidate journal, September 2018

Effect of spin-orbit coupling on the effective-spin correlation in YbMgGaO 4 journal, March 2018

Disorder-Induced Mimicry of a Spin Liquid in YbMgGaO 4 journal, October 2017

Field-induced instability of the quantum spin liquid ground state in the J eff = 1 2 triangular-lattice compound NaYbO 2 journal, May 2019

Fractionalized excitations in the partially magnetized spin liquid candidate YbMgGaO4 journal, October 2018

Dynamical structure factor of the triangular antiferromagnet: Schwinger boson theory beyond mean field journal, November 2018

Anisotropic spin model of strong spin-orbit-coupled triangular antiferromagnets journal, July 2016

Magnetic phase diagram of the S = 1 2 triangular-lattice Heisenberg antiferromagnet Ba 3 Co Nb 2 O 9 journal, July 2014

Magnetostriction in rare-earth based antiferromagnets journal, January 2005

Structure of the magnetic excitations in the spin-1/2 triangular-lattice Heisenberg antiferromagnet Ba3CoSb2O9 journal, August 2017

Direct Determination of Exchange Parameters in Cs 2 CuBr 4 and Cs 2 CuCl 4 : High-Field Electron-Spin-Resonance Studies journal, February 2014

Gapless spin liquid of an organic triangular compound evidenced by thermodynamic measurements journal, April 2011

Relevance of the Heisenberg-Kitaev Model for the Honeycomb Lattice Iridates A 2 IrO 3 journal, March 2012

Continuous excitations of the triangular-lattice quantum spin liquid YbMgGaO4 journal, December 2016

Spin Waves and Revised Crystal Structure of Honeycomb Iridate Na 2 IrO 3 journal, March 2012

Rare-Earth Triangular Lattice Spin Liquid: A Single-Crystal Study of YbMgGaO 4 journal, October 2015

Quantum Spin Ices and Topological Phases from Dipolar-Octupolar Doublets on the Pyrochlore Lattice journal, April 2014

Spin excitations in the frustrated triangular lattice antiferromagnet NaYbO 2 journal, June 2020

Spin liquid phase of the S = 1 2 J 1 − J 2 Heisenberg model on the triangular lattice journal, July 2015

Magnetoelastic hybrid excitations in CeAuAl 3 journal, March 2019

Experimental signatures of a three-dimensional quantum spin liquid in effective spin-1/2 Ce2Zr2O7 pyrochlore journal, July 2019

Quantum spin liquid in the spin- 1 ∕ 2 triangular antiferromagnet Et Me 3 Sb [ Pd ( dmit ) 2 ] 2 journal, March 2008

Resonating valence bonds: A new kind of insulator? journal, February 1973

Spinon Fermi Surface Spin Liquid in a Triangular Lattice Antiferromagnet NaYbSe 2 journal, May 2021

Time evolution of an infinite projected entangled pair state: An efficient algorithm journal, January 2019

Experimental Realization of a 2D Fractional Quantum Spin Liquid journal, February 2001

Anisotropic field-induced ordering in the triangular-lattice quantum spin liquid NaYbSe 2 journal, December 2019

Yb delafossites: Unique exchange frustration of 4 f spin- 1 2 moments on a perfect triangular lattice journal, June 2021

Candidate Quantum Spin Liquid in the Ce 3 + Pyrochlore Stannate Ce 2 Sn 2 O 7 journal, August 2015

Crystalline electric field of Ce in trigonal symmetry: CeIr 3 Ge 7 as a model case journal, November 2018

PyCrystalField : software for calculation, analysis and fitting of crystal electric field Hamiltonians journal, February 2021

Mott Insulators in the Strong Spin-Orbit Coupling Limit: From Heisenberg to a Quantum Compass and Kitaev Models journal, January 2009

Direct evidence for dominant bond-directional interactions in a honeycomb lattice iridate Na2IrO3 journal, May 2015

Frustrated Quantum Rare-Earth Pyrochlores journal, March 2019

Unusual ordered phases of highly frustrated magnets: a review journal, April 2015

Spin Liquid State in an Organic Mott Insulator with a Triangular Lattice journal, September 2003

Dynamical Structure Factor of the J 1 − J 2 Heisenberg Model on the Triangular Lattice: Magnons, Spinons, and Gauge Fields journal, August 2019

Quantum Phase Diagram of the Triangular-Lattice $X X Z$ Model in a Magnetic Field
journal, March 2014

Two-temperature scales in the triangular-lattice Heisenberg antiferromagnet
journal, April 2019

Scale-invariant magnetic anisotropy in RuCl3 at high magnetic fields
journal, October 2020

${NaYbS}_{2}$ : A planar spin- $\frac{1}{2}$ triangular-lattice magnet and putative spin liquid
journal, December 2018

Quantum spin liquids: a review
journal, November 2016

Evidence for a spinon Fermi surface in a triangular-lattice quantum-spin-liquid candidate
journal, December 2016

Field-tunable quantum disordered ground state in the triangular-lattice antiferromagnet NaYbO2
journal, July 2019

Resonant torsion magnetometry in anisotropic quantum materials
journal, September 2018

Field-induced magnetic transition and spin fluctuations in the quantum spin-liquid candidate ${CsYbSe}_{2}$
journal, December 2019

Metal–Insulator Transitions in Pyrochlore Oxides Ln ₂ Ir ₂ O ₇
journal, September 2011

$α - {RuCl}_{3}$ : A spin-orbit assisted Mott insulator on a honeycomb lattice
journal, July 2014

Effective Spin-1/2 Moments on a Yb ³⁺ Triangular Lattice: An ESR Study
conference, March 2020

Experimental Realization of a Spin- $1 / 2$ Triangular-Lattice Heisenberg Antiferromagnet
journal, January 2012

Direct Measurement of the Spin Hamiltonian and Observation of Condensation of Magnons in the 2D Frustrated Quantum Magnet ${Cs}_{2} {CuCl}_{4}$
journal, March 2002

Instability of a quantum spin liquid in an organic triangular-lattice antiferromagnet
journal, July 2010

Extended scattering continua characteristic of spin fractionalization in the two-dimensional frustrated quantum magnet ${Cs}_{2} {CuCl}_{4}$ observed by neutron scattering
journal, October 2003

Magnetic orders and topological phases from $f$ - $d$ exchange in pyrochlore iridates
journal, December 2012

Crystal Synthesis and Frustrated Magnetism in Triangular Lattice Cs RE Se ₂ ( RE = La–Lu): Quantum Spin Liquid Candidates CsCeSe ₂ and CsYbSe ₂
journal, November 2019

Anisotropic-Exchange Magnets on a Triangular Lattice: Spin Waves, Accidental Degeneracies, and Dual Spin Liquids
journal, April 2019

Series of phase transitions and multiferroicity in the quasi-two-dimensional spin- $\frac{1}{2}$ triangular-lattice antiferromagnet ${Ba}_{3} {CoNb}_{2} O_{9}$
journal, March 2014

Quantum spin liquid ground state in the disorder free triangular lattice ${NaYbS}_{2}$
journal, December 2019

Spin Dynamics of the Spin- $1 / 2$ Kagome Lattice Antiferromagnet ${ZnCu}_{3} (OH)_{6} {Cl}_{2}$
journal, March 2007

Magnetism driven by the interplay of fluctuations and frustration in the easy-axis triangular XXZ model with transverse fields
journal, October 2019

Quantum Spin Ice Dynamics in the Dipole-Octupole Pyrochlore Magnet ${Ce}_{2} {Zr}_{2} O_{7}$
journal, May 2019

Crystal-field Hamiltonian and anisotropy in ${KErSe}_{2}$ and ${CsErSe}_{2}$
journal, April 2020

Lattice dynamics and coupled quadrupole-phonon excitations in ${CeAuAl}_{3}$
journal, November 2018

Mermin-Wagner physics, $(H, T)$ phase diagram, and candidate quantum spin-liquid phase in the spin- $\frac{1}{2}$ triangular-lattice antiferromagnet ${Ba}_{8} {CoNb}_{6} O_{24}$
journal, April 2018

Symmetry enriched U(1) topological orders for dipole-octupole doublets on a pyrochlore lattice
journal, January 2017

Dirac Spin Liquid on the Spin- $1 / 2$ Triangular Heisenberg Antiferromagnet
journal, November 2019

Crystalline electric field excitations in the quantum spin liquid candidate ${NaYbSe}_{2}$
journal, January 2021

Spin liquids in geometrically perfect triangular antiferromagnets
journal, March 2020

Determination of effective microscopic models for the frustrated antiferromagnets Cs $_{2}$ CuCl $_{4}$ and Cs $_{2}$ CuBr $_{4}$ by density functional methods
journal, March 2011

Static and Dynamical Properties of the Spin- $1 / 2$ Equilateral Triangular-Lattice Antiferromagnet ${Ba}_{3} {CoSb}_{2} O_{9}$
journal, February 2016

Topography of Spin Liquids on a Triangular Lattice
journal, May 2018

Magnetic pyrochlore oxides
journal, January 2010

Dipolar-octupolar Ising antiferromagnetism in ${Sm}_{2} {Ti}_{2} O_{7}$ : A moment fragmentation candidate
journal, September 2018

Effect of spin-orbit coupling on the effective-spin correlation in ${YbMgGaO}_{4}$
journal, March 2018

Disorder-Induced Mimicry of a Spin Liquid in ${YbMgGaO}_{4}$
journal, October 2017

Field-induced instability of the quantum spin liquid ground state in the $J_{eff} = \frac{1}{2}$ triangular-lattice compound ${NaYbO}_{2}$
journal, May 2019

Fractionalized excitations in the partially magnetized spin liquid candidate YbMgGaO4
journal, October 2018

Dynamical structure factor of the triangular antiferromagnet: Schwinger boson theory beyond mean field
journal, November 2018

Anisotropic spin model of strong spin-orbit-coupled triangular antiferromagnets
journal, July 2016

Magnetic phase diagram of the $S = \frac{1}{2}$ triangular-lattice Heisenberg antiferromagnet ${Ba}_{3} Co {Nb}_{2} O_{9}$
journal, July 2014

Magnetostriction in rare-earth based antiferromagnets
journal, January 2005

Structure of the magnetic excitations in the spin-1/2 triangular-lattice Heisenberg antiferromagnet Ba3CoSb2O9
journal, August 2017

Direct Determination of Exchange Parameters in ${Cs}_{2} {CuBr}_{4}$ and ${Cs}_{2} {CuCl}_{4}$ : High-Field Electron-Spin-Resonance Studies
journal, February 2014

Gapless spin liquid of an organic triangular compound evidenced by thermodynamic measurements
journal, April 2011

Relevance of the Heisenberg-Kitaev Model for the Honeycomb Lattice Iridates $A_{2} {IrO}_{3}$
journal, March 2012

Continuous excitations of the triangular-lattice quantum spin liquid YbMgGaO4
journal, December 2016

Spin Waves and Revised Crystal Structure of Honeycomb Iridate ${Na}_{2} {IrO}_{3}$
journal, March 2012

Rare-Earth Triangular Lattice Spin Liquid: A Single-Crystal Study of ${YbMgGaO}_{4}$
journal, October 2015

Quantum Spin Ices and Topological Phases from Dipolar-Octupolar Doublets on the Pyrochlore Lattice
journal, April 2014

Spin excitations in the frustrated triangular lattice antiferromagnet ${NaYbO}_{2}$
journal, June 2020

Spin liquid phase of the $S = \frac{1}{2} J_{1} - J_{2}$ Heisenberg model on the triangular lattice
journal, July 2015

Magnetoelastic hybrid excitations in CeAuAl ₃
journal, March 2019

Experimental signatures of a three-dimensional quantum spin liquid in effective spin-1/2 Ce2Zr2O7 pyrochlore
journal, July 2019

Quantum spin liquid in the spin- $1 ∕ 2$ triangular antiferromagnet $Et {Me}_{3} Sb {[Pd {(dmit)}_{2}]}_{2}$
journal, March 2008

Resonating valence bonds: A new kind of insulator?
journal, February 1973

Spinon Fermi Surface Spin Liquid in a Triangular Lattice Antiferromagnet ${NaYbSe}_{2}$
journal, May 2021

Time evolution of an infinite projected entangled pair state: An efficient algorithm
journal, January 2019

Experimental Realization of a 2D Fractional Quantum Spin Liquid
journal, February 2001

Anisotropic field-induced ordering in the triangular-lattice quantum spin liquid ${NaYbSe}_{2}$
journal, December 2019

Yb delafossites: Unique exchange frustration of $4 f$ spin- $\frac{1}{2}$ moments on a perfect triangular lattice
journal, June 2021

Candidate Quantum Spin Liquid in the ${Ce}^{3 +}$ Pyrochlore Stannate ${Ce}_{2} {Sn}_{2} O_{7}$
journal, August 2015

Crystalline electric field of Ce in trigonal symmetry: ${CeIr}_{3} {Ge}_{7}$ as a model case
journal, November 2018

PyCrystalField : software for calculation, analysis and fitting of crystal electric field Hamiltonians
journal, February 2021

Mott Insulators in the Strong Spin-Orbit Coupling Limit: From Heisenberg to a Quantum Compass and Kitaev Models
journal, January 2009

Direct evidence for dominant bond-directional interactions in a honeycomb lattice iridate Na2IrO3
journal, May 2015

Frustrated Quantum Rare-Earth Pyrochlores
journal, March 2019

Unusual ordered phases of highly frustrated magnets: a review
journal, April 2015

Spin Liquid State in an Organic Mott Insulator with a Triangular Lattice
journal, September 2003

Dynamical Structure Factor of the $J_{1} - J_{2}$ Heisenberg Model on the Triangular Lattice: Magnons, Spinons, and Gauge Fields
journal, August 2019