Review of Swift Heavy Ion Irradiation Effects in CeO2

Cureton, William F.; Tracy, Cameron L.; Lang, Maik

doi:10.3390/qubs5020019

Title: Review of Swift Heavy Ion Irradiation Effects in CeO2

Abstract

Cerium dioxide (CeO₂) exhibits complex behavior when irradiated with swift heavy ions. Modifications to this material originate from the production of atomic-scale defects, which accumulate and induce changes to the microstructure, chemistry, and material properties. As such, characterizing its radiation response requires a wide range of complementary characterization techniques to elucidate the defect formation and stability over multiple length scales, such as X-ray and neutron scattering, optical spectroscopy, and electron microscopy. In this article, recent experimental efforts are reviewed in order to holistically assess the current understanding and knowledge gaps regarding the underlying physical mechanisms that dictate the response of CeO₂ and related materials to irradiation with swift heavy ions. The recent application of novel experimental techniques has provided additional insight into the structural and chemical behavior of irradiation-induced defects, from the local, atomic-scale arrangement to the long-range structure. However, future work must carefully account for the influence of experimental conditions, with respect to both sample properties (e.g., grain size and impurity content) and ion-beam parameters (e.g., ion mass and energy), to facilitate a more direct comparison of experimental results.

Authors:

Cureton, William F.;

; Lang, Maik

Publication Date:: Wed Jun 16 00:00:00 EDT 2021

Research Org.:: Univ. of Illinois, Chicago, IL (United States); Univ. of Tennessee, Knoxville, TN (United States)

Sponsoring Org.:: USDOE National Nuclear Security Administration (NNSA), Office of Defense Programs (DP); USDOE Office of Nuclear Energy (NE), Nuclear Energy University Program (NEUP)

OSTI Identifier:: 1797516

Alternate Identifier(s):: OSTI ID: 1813554; OSTI ID: 2328667

Grant/Contract Number:: NE0008895; NA0003975; AC02-06CH11357

Resource Type:: Published Article

Journal Name:: Quantum Beam Science

Additional Journal Information:: Journal Name: Quantum Beam Science Journal Volume: 5 Journal Issue: 2; Journal ID: ISSN 2412-382X

Publisher:: MDPI AG

Country of Publication:: Switzerland

Language:: English

Subject:: 42 ENGINEERING; cerium oxide; CeO2; irradiation; swift heavy ions

Citation Formats


                    Cureton, William F., Tracy, Cameron L., and Lang, Maik. Review of Swift Heavy Ion Irradiation Effects in CeO2.  Switzerland: N. p., 2021. 
Web.  doi:10.3390/qubs5020019.

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                    Cureton, William F., Tracy, Cameron L., & Lang, Maik. Review of Swift Heavy Ion Irradiation Effects in CeO2.  Switzerland.  https://doi.org/10.3390/qubs5020019

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                    Cureton, William F., Tracy, Cameron L., and Lang, Maik. Wed .  
"Review of Swift Heavy Ion Irradiation Effects in CeO2".  Switzerland.  https://doi.org/10.3390/qubs5020019.

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@article{osti_1797516,

  title        = {Review of Swift Heavy Ion Irradiation Effects in CeO2},

  author       = {Cureton, William F. and Tracy, Cameron L. and Lang, Maik},

  abstractNote = {Cerium dioxide (CeO2) exhibits complex behavior when irradiated with swift heavy ions. Modifications to this material originate from the production of atomic-scale defects, which accumulate and induce changes to the microstructure, chemistry, and material properties. As such, characterizing its radiation response requires a wide range of complementary characterization techniques to elucidate the defect formation and stability over multiple length scales, such as X-ray and neutron scattering, optical spectroscopy, and electron microscopy. In this article, recent experimental efforts are reviewed in order to holistically assess the current understanding and knowledge gaps regarding the underlying physical mechanisms that dictate the response of CeO2 and related materials to irradiation with swift heavy ions. The recent application of novel experimental techniques has provided additional insight into the structural and chemical behavior of irradiation-induced defects, from the local, atomic-scale arrangement to the long-range structure. However, future work must carefully account for the influence of experimental conditions, with respect to both sample properties (e.g., grain size and impurity content) and ion-beam parameters (e.g., ion mass and energy), to facilitate a more direct comparison of experimental results.},

  doi          = {10.3390/qubs5020019},

  journal      = {Quantum Beam Science},

  number       = 2,

  volume       = 5,

  place        = {Switzerland},

  year         = {Wed Jun 16 00:00:00 EDT 2021},

  month        = {Wed Jun 16 00:00:00 EDT 2021}

}

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Title: Review of Swift Heavy Ion Irradiation Effects in CeO2

Abstract

Citation Formats

A review of defect structure and chemistry in ceria and its solid solutions journal, January 2020

Similar local order in disordered fluorite and aperiodic pyrochlore structures journal, February 2018

XPS study of ion irradiated and unirradiated CeO2 bulk and thin film samples journal, August 2018

Role of Thermodynamics in the Shape Transformation of Embedded Metal Nanoparticles Induced by Swift Heavy-Ion Irradiation journal, March 2011

Revised effective ionic radii and systematic studies of interatomic distances in halides and chalcogenides journal, September 1976

The utilization of ceria in industrial catalysis journal, April 1999

New developments in micro-X-ray diffraction and X-ray absorption spectroscopy for high-pressure research at 16-BM-D at the Advanced Photon Source journal, July 2015

Swift heavy ions in magnetic insulators: A damage-cross-section velocity effect journal, July 1993

Ordered intermediate phases in the system CeO2Ce2O3 journal, March 1955

Radiation-Induced Reduction of Ceria in Single and Polycrystalline Thin Films journal, December 2011

Optical spectroscopy study of modifications induced in cerium dioxide by electron and ion irradiations journal, April 2019

Evidence of extended defects in pure zirconia irradiated by swift heavy ions journal, October 2006

Phase transformations in Ln 2 O 3 materials irradiated with swift heavy ions journal, November 2015

Molecular dynamics simulation of fast particle irradiation to the Gd2O3-doped CeO2 journal, December 2013

Chapter 27: The binary rare earth oxides book, January 1979

Effects of high-energy heavy ion irradiation on the crystal structure in CeO2 thin films journal, November 2013

Structural and microstructural tailoring of rare earth sesquioxides by swift heavy ion irradiation: Tailoring of rare earth sesquioxides by swift heavy ion irradiation journal, August 2016

SRIM – The stopping and range of ions in matter (2010) journal, June 2010

Radiation Tolerance of Complex Oxides journal, August 2000

Charge distribution near bulk oxygen vacancies in cerium oxides journal, May 2010

Mixed valency in cerium oxide crystallographic phases: Valence of different cerium sites by the bond valence method journal, April 2009

Heavy Ion Radiation Effects on a 130-nm COTS NVSRAM Under Different Measurement Conditions journal, May 2018

Chemical Expansion: Implications for Electrochemical Energy Storage and Conversion Devices journal, July 2014

Heavy-ion tumor therapy: Physical and radiobiological benefits journal, February 2010

Annealing-induced lattice recovery in room-temperature xenon irradiated CeO 2 : X-ray diffraction and electron energy loss spectroscopy experiments journal, February 2015

Study on effects of swift heavy ion irradiation in cerium dioxide using synchrotron radiation X-ray absorption spectroscopy journal, June 2008

Swift heavy ion irradiation induced nanoparticle formation in CeO2 thin films journal, December 2011

Cerium under the lens journal, March 2013

Probing disorder in isometric pyrochlore and related complex oxides journal, February 2016

Energetics of defect production in fluorite-structured CeO 2 induced by highly ionizing radiation journal, September 2018

Degradation of polyimide under irradiation with swift heavy ions journal, July 2005

Study on effects of swift heavy ion irradiation on the crystal structure in CeO2 doped with Gd2O3 journal, May 2011

Characterization of swift heavy ion irradiation damage in ceria journal, March 2015

Oxygen vacancy ordering within anion-deficient Ceria journal, October 2009

Electronic structure and stability of hyperstoichiometric UO 2 + x under pressure journal, July 2013

Analysis and optimization of propagation losses in LiNbO3 optical waveguides produced by swift heavy-ion irradiation journal, February 2012

Ion beam induced surface and interface engineering journal, March 2011

The Structures of C–Ce2O3+δ, Ce7O12, and Ce11O20 journal, November 1999

Thermodynamic and structural evolution of Dy2Ti2O7 pyrochlore after swift heavy ion irradiation journal, February 2018

Oxide pyrochlores — A review journal, January 1983

Phase transformations induced by heavy ion irradiation in Gd2O3: Comparison between ballistic and electronic excitation regimes journal, November 2018

Study on the behavior of oxygen atoms in swift heavy ion irradiated CeO2 by means of synchrotron radiation X-ray photoelectron spectroscopy journal, March 2009

Nuclear waste disposal—pyrochlore (A2B2O7): Nuclear waste form for the immobilization of plutonium and “minor” actinides journal, June 2004

Stability of the Ce 2 O 3 phases: A DFT + U investigation journal, November 2007

Clarification of the properties and accumulation effects of ion tracks in CeO2 journal, June 2008

Creation of multiple nanodots by single ions journal, April 2007

Single-ion tracks in Gd 2 Zr 2 − x Ti x O 7 pyrochlores irradiated with swift heavy ions journal, June 2009

Defect accumulation in ThO2 irradiated with swift heavy ions journal, May 2014

Interpreting oxygen vacancy migration mechanisms in oxides using the layered structure motif journal, June 2015

Response of Gd2Ti2O7 and La2Ti2O7 to swift-heavy ion irradiation and annealing journal, July 2015

High-pressure x-ray diffraction study of CeO 2 to 70 GPa and pressure-induced phase transformation from the fluorite structure journal, October 1988

Review of A2B2O7 pyrochlore response to irradiation and pressure journal, October 2010

Solid-density plasma nanochannel generated by a fast single ion in condensed matter journal, March 2009

Modelling the effects of electronic excitations in ionic-covalent materials journal, April 2012

Nanoscale manipulation of the properties of solids at high pressure with relativistic heavy ions journal, September 2009

Change in magnetic properties induced by swift heavy ion irradiation in CeO2 journal, September 2012

Analysis of Ion-Irradiation Induced Lattice Expansion and Ferromagnetic State in CeO2 by Using Poisson Distribution Function journal, July 2020

Recovery and restructuring induced by fission energy ions in high burnup nuclear fuel journal, March 2009

Oxidation state of Ce in Pb 2 Sr 2 Ce 1 − x Ca x Cu 3 O 8 journal, January 1996

Phase transformations in Y2O3 thin films under swift Xe ions irradiation journal, September 2013

The Binary Rare Earth Oxides journal, June 1998

Experimental evidence of crystalline hillocks created by irradiation of CeO 2 with swift heavy ions: TEM study journal, August 2015

Characterization of ion-induced radiation effects in nuclear materials using synchrotron x-ray techniques journal, May 2015

Grain size effects on irradiated CeO2, ThO2, and UO2 journal, November 2018

Defect formation and accumulation in CeO2 irradiated with swift heavy ions journal, November 2013

Phase stability of nanostructured materials under heavy ion irradiation journal, January 1995

Liquid-like phase formation in Gd2Zr2O7 by extremely ionizing irradiation journal, June 2009

Structural modifications of Gd 2 Zr 2- x Ti x O 7 pyrochlore induced by swift heavy ions: Disordering and amorphization journal, April 2009

Study on effects of energetic ion irradiation in Gd2O3-doped CeO2 by means of synchrotron radiation X-ray spectroscopy journal, April 2012

Anomalous compressive behavior in CeO 2 nanocubes under high pressure journal, December 2008

Effect of grain size and microstructure on radiation stability of CeO 2 : an extensive study journal, January 2014

Effects of swift heavy ion irradiation on the structure of Er2O3-doped CeO2 journal, October 2010

Fundamental Phenomena and Applications of Swift Heavy Ion Irradiations book, August 2020

High-pressure Raman study of CeO 2 to 35 GPa and pressure-induced phase transformation from the fluorite structure journal, March 1988

Origin of Anomalous Lattice Expansion in Oxide Nanoparticles journal, October 2000

In situ defect annealing of swift heavy ion irradiated CeO 2 and ThO 2 using synchrotron X-ray diffraction and a hydrothermal diamond anvil cell journal, April 2015

Role of composition, bond covalency, and short-range order in the disordering of stannate pyrochlores by swift heavy ion irradiation journal, August 2016

A review of defect structure and chemistry in ceria and its solid solutions
journal, January 2020

Similar local order in disordered fluorite and aperiodic pyrochlore structures
journal, February 2018

XPS study of ion irradiated and unirradiated CeO2 bulk and thin film samples
journal, August 2018

Role of Thermodynamics in the Shape Transformation of Embedded Metal Nanoparticles Induced by Swift Heavy-Ion Irradiation
journal, March 2011

Revised effective ionic radii and systematic studies of interatomic distances in halides and chalcogenides
journal, September 1976

The utilization of ceria in industrial catalysis
journal, April 1999

New developments in micro-X-ray diffraction and X-ray absorption spectroscopy for high-pressure research at 16-BM-D at the Advanced Photon Source
journal, July 2015

Swift heavy ions in magnetic insulators: A damage-cross-section velocity effect
journal, July 1993

Ordered intermediate phases in the system CeO2Ce2O3
journal, March 1955

Radiation-Induced Reduction of Ceria in Single and Polycrystalline Thin Films
journal, December 2011

Optical spectroscopy study of modifications induced in cerium dioxide by electron and ion irradiations
journal, April 2019

Evidence of extended defects in pure zirconia irradiated by swift heavy ions
journal, October 2006

Phase transformations in ${Ln}_{2} O_{3}$ materials irradiated with swift heavy ions
journal, November 2015

Molecular dynamics simulation of fast particle irradiation to the Gd2O3-doped CeO2
journal, December 2013

Chapter 27: The binary rare earth oxides
book, January 1979

Effects of high-energy heavy ion irradiation on the crystal structure in CeO2 thin films
journal, November 2013

Structural and microstructural tailoring of rare earth sesquioxides by swift heavy ion irradiation: Tailoring of rare earth sesquioxides by swift heavy ion irradiation
journal, August 2016

SRIM – The stopping and range of ions in matter (2010)
journal, June 2010

Radiation Tolerance of Complex Oxides
journal, August 2000

Charge distribution near bulk oxygen vacancies in cerium oxides
journal, May 2010

Mixed valency in cerium oxide crystallographic phases: Valence of different cerium sites by the bond valence method
journal, April 2009

Heavy Ion Radiation Effects on a 130-nm COTS NVSRAM Under Different Measurement Conditions
journal, May 2018

Chemical Expansion: Implications for Electrochemical Energy Storage and Conversion Devices
journal, July 2014

Heavy-ion tumor therapy: Physical and radiobiological benefits
journal, February 2010

Annealing-induced lattice recovery in room-temperature xenon irradiated CeO ₂ : X-ray diffraction and electron energy loss spectroscopy experiments
journal, February 2015

Study on effects of swift heavy ion irradiation in cerium dioxide using synchrotron radiation X-ray absorption spectroscopy
journal, June 2008

Swift heavy ion irradiation induced nanoparticle formation in CeO2 thin films
journal, December 2011

Cerium under the lens
journal, March 2013

Probing disorder in isometric pyrochlore and related complex oxides
journal, February 2016

Energetics of defect production in fluorite-structured ${CeO}_{2}$ induced by highly ionizing radiation
journal, September 2018

Degradation of polyimide under irradiation with swift heavy ions
journal, July 2005

Study on effects of swift heavy ion irradiation on the crystal structure in CeO2 doped with Gd2O3
journal, May 2011

Characterization of swift heavy ion irradiation damage in ceria
journal, March 2015

Oxygen vacancy ordering within anion-deficient Ceria
journal, October 2009

Electronic structure and stability of hyperstoichiometric UO $_{2 + x}$ under pressure
journal, July 2013

Analysis and optimization of propagation losses in LiNbO3 optical waveguides produced by swift heavy-ion irradiation
journal, February 2012

Ion beam induced surface and interface engineering
journal, March 2011

The Structures of C–Ce2O3+δ, Ce7O12, and Ce11O20
journal, November 1999

Thermodynamic and structural evolution of Dy2Ti2O7 pyrochlore after swift heavy ion irradiation
journal, February 2018

Oxide pyrochlores — A review
journal, January 1983

Phase transformations induced by heavy ion irradiation in Gd2O3: Comparison between ballistic and electronic excitation regimes
journal, November 2018

Study on the behavior of oxygen atoms in swift heavy ion irradiated CeO2 by means of synchrotron radiation X-ray photoelectron spectroscopy
journal, March 2009

Nuclear waste disposal—pyrochlore (A2B2O7): Nuclear waste form for the immobilization of plutonium and “minor” actinides
journal, June 2004

Stability of the ${Ce}_{2} O_{3}$ phases: A $DFT + U$ investigation
journal, November 2007

Clarification of the properties and accumulation effects of ion tracks in CeO2
journal, June 2008

Creation of multiple nanodots by single ions
journal, April 2007

Single-ion tracks in ${Gd}_{2} {Zr}_{2 - x} {Ti}_{x} O_{7}$ pyrochlores irradiated with swift heavy ions
journal, June 2009

Defect accumulation in ThO2 irradiated with swift heavy ions
journal, May 2014

Interpreting oxygen vacancy migration mechanisms in oxides using the layered structure motif
journal, June 2015

Response of Gd2Ti2O7 and La2Ti2O7 to swift-heavy ion irradiation and annealing
journal, July 2015

High-pressure x-ray diffraction study of ${CeO}_{2}$ to 70 GPa and pressure-induced phase transformation from the fluorite structure
journal, October 1988

Review of A2B2O7 pyrochlore response to irradiation and pressure
journal, October 2010

Solid-density plasma nanochannel generated by a fast single ion in condensed matter
journal, March 2009

Modelling the effects of electronic excitations in ionic-covalent materials
journal, April 2012

Nanoscale manipulation of the properties of solids at high pressure with relativistic heavy ions
journal, September 2009

Change in magnetic properties induced by swift heavy ion irradiation in CeO2
journal, September 2012

Analysis of Ion-Irradiation Induced Lattice Expansion and Ferromagnetic State in CeO2 by Using Poisson Distribution Function
journal, July 2020

Recovery and restructuring induced by fission energy ions in high burnup nuclear fuel
journal, March 2009

Oxidation state of Ce in ${Pb}_{2}$ ${Sr}_{2}$ ${Ce}_{1 - x}$ ${Ca}_{x}$ ${Cu}_{3}$ $O_{8}$
journal, January 1996

Phase transformations in Y2O3 thin films under swift Xe ions irradiation
journal, September 2013

The Binary Rare Earth Oxides
journal, June 1998

Experimental evidence of crystalline hillocks created by irradiation of CeO ₂ with swift heavy ions: TEM study
journal, August 2015

Characterization of ion-induced radiation effects in nuclear materials using synchrotron x-ray techniques
journal, May 2015

Grain size effects on irradiated CeO2, ThO2, and UO2
journal, November 2018

Defect formation and accumulation in CeO2 irradiated with swift heavy ions
journal, November 2013

Phase stability of nanostructured materials under heavy ion irradiation
journal, January 1995

Liquid-like phase formation in Gd2Zr2O7 by extremely ionizing irradiation
journal, June 2009

Structural modifications of Gd ₂ Zr _{2- x} Ti _x O ₇ pyrochlore induced by swift heavy ions: Disordering and amorphization
journal, April 2009

Study on effects of energetic ion irradiation in Gd2O3-doped CeO2 by means of synchrotron radiation X-ray spectroscopy
journal, April 2012

Anomalous compressive behavior in CeO ₂ nanocubes under high pressure
journal, December 2008

Effect of grain size and microstructure on radiation stability of CeO ₂ : an extensive study
journal, January 2014

Effects of swift heavy ion irradiation on the structure of Er2O3-doped CeO2
journal, October 2010

Fundamental Phenomena and Applications of Swift Heavy Ion Irradiations
book, August 2020

High-pressure Raman study of ${CeO}_{2}$ to 35 GPa and pressure-induced phase transformation from the fluorite structure
journal, March 1988

Origin of Anomalous Lattice Expansion in Oxide Nanoparticles
journal, October 2000

In situ defect annealing of swift heavy ion irradiated CeO ₂ and ThO ₂ using synchrotron X-ray diffraction and a hydrothermal diamond anvil cell
journal, April 2015

Role of composition, bond covalency, and short-range order in the disordering of stannate pyrochlores by swift heavy ion irradiation
journal, August 2016

Effects of irradiation temperature on the response of CeO2, ThO2, and UO2 to highly ionizing radiation
journal, November 2019

Alpha-irradiation damage in CeO ₂ , UO ₂ and PuO ₂
journal, January 1984

Swift heavy ion and fission damage effects in UO2
journal, May 2000