Semiconductor quantum dots: Technological progress and future challenges
Abstract
In quantum-confined semiconductor nanostructures, electrons exhibit distinctive behavior compared with that in bulk solids. This enables the design of materials with tunable chemical, physical, electrical, and optical properties. Zero-dimensional semiconductor quantum dots (QDs) offer strong light absorption and bright narrowband emission across the visible and infrared wavelengths and have been engineered to exhibit optical gain and lasing. These properties are of interest for imaging, solar energy harvesting, displays, and communications. Here, we offer an overview of advances in the synthesis and understanding of QD nanomaterials, with a focus on colloidal QDs, and discuss their prospects in technologies such as displays and lighting, lasers, sensing, electronics, solar energy conversion, photocatalysis, and quantum information.
- Authors:
-
- Department of Electrical and Computer Engineering, University of Toronto, 35 St. George Street, Toronto, ON M5S 1A4, Canada., ICFO–Institut de Ciències Fotòniques, The Barcelona Institute of Science and Technology, Barcelona 08860, Spain.
- Department of Chemistry, University of Chicago, Chicago, IL 60637, USA.
- Chemistry Division, C-PCS, Los Alamos National Laboratory, Los Alamos, NM 87545, USA.
- University of Tokyo, Meguro, Tokyo 153-8505, Japan.
- Technische Universitat Dortmund, 44221 Dortmund, Germany.
- Department of Electrical and Computer Engineering, University of Toronto, 35 St. George Street, Toronto, ON M5S 1A4, Canada.
- Publication Date:
- Sponsoring Org.:
- USDOE
- OSTI Identifier:
- 1812116
- Grant/Contract Number:
- AC02-06CH11357; Solar Photochemistry Program; 20200213DR
- Resource Type:
- Published Article
- Journal Name:
- Science
- Additional Journal Information:
- Journal Name: Science Journal Volume: 373 Journal Issue: 6555; Journal ID: ISSN 0036-8075
- Publisher:
- American Association for the Advancement of Science (AAAS)
- Country of Publication:
- United States
- Language:
- English
Citation Formats
García de Arquer, F. Pelayo, Talapin, Dmitri V., Klimov, Victor I., Arakawa, Yasuhiko, Bayer, Manfred, and Sargent, Edward H. Semiconductor quantum dots: Technological progress and future challenges. United States: N. p., 2021.
Web. doi:10.1126/science.aaz8541.
García de Arquer, F. Pelayo, Talapin, Dmitri V., Klimov, Victor I., Arakawa, Yasuhiko, Bayer, Manfred, & Sargent, Edward H. Semiconductor quantum dots: Technological progress and future challenges. United States. https://doi.org/10.1126/science.aaz8541
García de Arquer, F. Pelayo, Talapin, Dmitri V., Klimov, Victor I., Arakawa, Yasuhiko, Bayer, Manfred, and Sargent, Edward H. Thu .
"Semiconductor quantum dots: Technological progress and future challenges". United States. https://doi.org/10.1126/science.aaz8541.
@article{osti_1812116,
title = {Semiconductor quantum dots: Technological progress and future challenges},
author = {García de Arquer, F. Pelayo and Talapin, Dmitri V. and Klimov, Victor I. and Arakawa, Yasuhiko and Bayer, Manfred and Sargent, Edward H.},
abstractNote = {In quantum-confined semiconductor nanostructures, electrons exhibit distinctive behavior compared with that in bulk solids. This enables the design of materials with tunable chemical, physical, electrical, and optical properties. Zero-dimensional semiconductor quantum dots (QDs) offer strong light absorption and bright narrowband emission across the visible and infrared wavelengths and have been engineered to exhibit optical gain and lasing. These properties are of interest for imaging, solar energy harvesting, displays, and communications. Here, we offer an overview of advances in the synthesis and understanding of QD nanomaterials, with a focus on colloidal QDs, and discuss their prospects in technologies such as displays and lighting, lasers, sensing, electronics, solar energy conversion, photocatalysis, and quantum information.},
doi = {10.1126/science.aaz8541},
journal = {Science},
number = 6555,
volume = 373,
place = {United States},
year = {Thu Aug 05 00:00:00 EDT 2021},
month = {Thu Aug 05 00:00:00 EDT 2021}
}
https://doi.org/10.1126/science.aaz8541
Works referenced in this record:
Energy storage emerging: A perspective from the Joint Center for Energy Storage Research
journal, June 2020
- Trahey, Lynn; Brushett, Fikile R.; Balsara, Nitash P.
- Proceedings of the National Academy of Sciences, Vol. 117, Issue 23
Synthesis and characterization of nearly monodisperse CdE (E = sulfur, selenium, tellurium) semiconductor nanocrystallites
journal, September 1993
- Murray, C. B.; Norris, D. J.; Bawendi, M. G.
- Journal of the American Chemical Society, Vol. 115, Issue 19, p. 8706-8715
Quantum dot solids showing state-resolved band-like transport
journal, January 2020
- Lan, Xinzheng; Chen, Menglu; Hudson, Margaret H.
- Nature Materials, Vol. 19, Issue 3
Ultrasensitive solution-cast quantum dot photodetectors
journal, July 2006
- Konstantatos, Gerasimos; Howard, Ian; Fischer, Armin
- Nature, Vol. 442, Issue 7099
Metal Halide Perovskites in Quantum Dot Solar Cells: Progress and Prospects
journal, June 2020
- Yuan, Jianyu; Hazarika, Abhijit; Zhao, Qian
- Joule, Vol. 4, Issue 6
Lattice anchoring stabilizes solution-processed semiconductors
journal, May 2019
- Liu, Mengxia; Chen, Yuelang; Tan, Chih-Shan
- Nature, Vol. 570, Issue 7759
Consensus statement for stability assessment and reporting for perovskite photovoltaics based on ISOS procedures
journal, January 2020
- Khenkin, Mark V.; Katz, Eugene A.; Abate, Antonio
- Nature Energy, Vol. 5, Issue 1
Semiconducting quantum dots for artificial photosynthesis
journal, July 2018
- Li, Xu-Bing; Tung, Chen-Ho; Wu, Li-Zhu
- Nature Reviews Chemistry, Vol. 2, Issue 8
Highly indistinguishable on-demand resonance fluorescence photons from a deterministic quantum dot micropillar device with 74% extraction efficiency
journal, January 2016
- Unsleber, Sebastian; He, Yu-Ming; Gerhardt, Stefan
- Optics Express, Vol. 24, Issue 8
Spectroscopic insights into the performance of quantum dot light-emitting diodes
journal, September 2013
- Bae, Wan Ki; Brovelli, Sergio; Klimov, Victor I.
- MRS Bulletin, Vol. 38, Issue 9
On-demand generation of indistinguishable polarization-entangled photon pairs
journal, February 2014
- Müller, M.; Bounouar, S.; Jöns, K. D.
- Nature Photonics, Vol. 8, Issue 3
Highly uniform InGaAs/GaAs quantum dots (∼15 nm) by metalorganic chemical vapor deposition
journal, September 1994
- Oshinowo, J.; Nishioka, M.; Ishida, S.
- Applied Physics Letters, Vol. 65, Issue 11
Trap states in lead chalcogenide colloidal quantum dots—origin, impact, and remedies
journal, December 2020
- Kahmann, Simon; Loi, Maria A.
- Applied Physics Reviews, Vol. 7, Issue 4
Self-photosensitization of nonphotosynthetic bacteria for solar-to-chemical production
journal, December 2015
- Sakimoto, K. K.; Wong, A. B.; Yang, P.
- Science, Vol. 351, Issue 6268
High Carrier Mobility in HgTe Quantum Dot Solids Improves Mid-IR Photodetectors
journal, August 2019
- Chen, Menglu; Lan, Xinzheng; Tang, Xin
- ACS Photonics, Vol. 6, Issue 9
Strain-Tunable GaAs Quantum Dot: A Nearly Dephasing-Free Source of Entangled Photon Pairs on Demand
journal, July 2018
- Huber, Daniel; Reindl, Marcus; Covre da Silva, Saimon Filipe
- Physical Review Letters, Vol. 121, Issue 3
Synthesis cost dictates the commercial viability of lead sulfide and perovskite quantum dot photovoltaics
journal, January 2018
- Jean, Joel; Xiao, Justin; Nick, Robert
- Energy & Environmental Science, Vol. 11, Issue 9
Colloidal quantum-dot light-emitting diodes with metal-oxide charge transport layers
journal, March 2008
- Caruge, J. M.; Halpert, J. E.; Wood, V.
- Nature Photonics, Vol. 2, Issue 4
Solution-processed upconversion photodetectors based on quantum dots
journal, March 2020
- Zhou, Wenjia; Shang, Yuequn; García de Arquer, F. Pelayo
- Nature Electronics, Vol. 3, Issue 5
Light Emission Mechanisms in CuInS 2 Quantum Dots Evaluated by Spectral Electrochemistry
journal, September 2017
- Fuhr, Addis S.; Yun, Hyeong Jin; Makarov, Nikolay S.
- ACS Photonics, Vol. 4, Issue 10
Droop-Free Colloidal Quantum Dot Light-Emitting Diodes
journal, September 2018
- Lim, Jaehoon; Park, Young-Shin; Wu, Kaifeng
- Nano Letters, Vol. 18, Issue 10
High-efficiency colloidal quantum dot infrared light-emitting diodes via engineering at the supra-nanocrystalline level
journal, December 2018
- Pradhan, Santanu; Di Stasio, Francesco; Bi, Yu
- Nature Nanotechnology, Vol. 14, Issue 1
Synthesis, properties and applications of colloidal germanium and germanium-based nanomaterials
journal, January 2013
- Vaughn II, Dimitri D.; Schaak, Raymond E.
- Chem. Soc. Rev., Vol. 42, Issue 7
Colloidal quantum dot lasers
journal, February 2021
- Park, Young-Shin; Roh, Jeongkyun; Diroll, Benjamin T.
- Nature Reviews Materials, Vol. 6, Issue 5
Efficient hybrid colloidal quantum dot/organic solar cells mediated by near-infrared sensitizing small molecules
journal, November 2019
- Baek, Se-Woong; Jun, Sunhong; Kim, Byeongsu
- Nature Energy, Vol. 4, Issue 11
Single-exciton optical gain in semiconductor nanocrystals
journal, May 2007
- Klimov, Victor I.; Ivanov, Sergei A.; Nanda, Jagjit
- Nature, Vol. 447, Issue 7143
Synthesis and Characterization of Monodisperse Nanocrystals and Close-Packed Nanocrystal Assemblies
journal, August 2000
- Murray, C. B.; Kagan, C. R.; Bawendi, M. G.
- Annual Review of Materials Science, Vol. 30, Issue 1, p. 545-610
Light Emission and Amplification in Charged CdSe Quantum Dots
journal, July 2004
- Wang, Congjun; Wehrenberg, Brian L.; Woo, Chui Y.
- The Journal of Physical Chemistry B, Vol. 108, Issue 26
Improved fidelity of triggered entangled photons from single quantum dots
journal, February 2006
- Young, Robert J.; Stevenson, R. Mark; Atkinson, Paola
- New Journal of Physics, Vol. 8, Issue 2
Breaking the Open-Circuit Voltage Deficit Floor in PbS Quantum Dot Solar Cells through Synergistic Ligand and Architecture Engineering
journal, May 2017
- Pradhan, Santanu; Stavrinadis, Alexandros; Gupta, Shuchi
- ACS Energy Letters, Vol. 2, Issue 6
Redefining near-unity luminescence in quantum dots with photothermal threshold quantum yield
journal, March 2019
- Hanifi, David A.; Bronstein, Noah D.; Koscher, Brent A.
- Science, Vol. 363, Issue 6432
Mid- and Long-Wave Infrared Optoelectronics via Intraband Transitions in PbS Colloidal Quantum Dots
journal, December 2019
- Ramiro, Iñigo; Özdemir, Onur; Christodoulou, Sotirios
- Nano Letters, Vol. 20, Issue 2
Heavily Doped Semiconductor Nanocrystal Quantum Dots
journal, March 2011
- Mocatta, D.; Cohen, G.; Schattner, J.
- Science, Vol. 332, Issue 6025
Tandem luminescent solar concentrators based on engineered quantum dots
journal, January 2018
- Wu, Kaifeng; Li, Hongbo; Klimov, Victor I.
- Nature Photonics, Vol. 12, Issue 2
Particulate Photocatalysts for Water Splitting: Recent Advances and Future Prospects
journal, January 2019
- Takata, Tsuyoshi; Domen, Kazunari
- ACS Energy Letters, Vol. 4, Issue 2
Solution-processed solar cells based on environmentally friendly AgBiS2 nanocrystals
journal, June 2016
- Bernechea, María; Miller, Nichole Cates; Xercavins, Guillem
- Nature Photonics, Vol. 10, Issue 8
Quantum dot-induced phase stabilization of -CsPbI3 perovskite for high-efficiency photovoltaics
journal, October 2016
- Swarnkar, A.; Marshall, A. R.; Sanehira, E. M.
- Science, Vol. 354, Issue 6308
Fiber-Coupled Luminescent Concentrators for Medical Diagnostics, Agriculture, and Telecommunications
journal, July 2019
- Makarov, Nikolay S.; Ramasamy, Karthik; Jackson, Aaron
- ACS Nano, Vol. 13, Issue 8
PbSe Nanocrystal Solids for n- and p-Channel Thin Film Field-Effect Transistors
journal, October 2005
- Talapin, D. V.
- Science, Vol. 310, Issue 5745, p. 86-89
Detailed-balance analysis of Yb 3+ :CsPb(Cl 1−x Br x ) 3 quantum-cutting layers for high-efficiency photovoltaics under real-world conditions
journal, January 2019
- Crane, Matthew J.; Kroupa, Daniel M.; Gamelin, Daniel R.
- Energy & Environmental Science, Vol. 12, Issue 8
Solution-processed PbS quantum dot infrared photodetectors and photovoltaics
journal, January 2005
- McDonald, Steven A.; Konstantatos, Gerasimos; Zhang, Shiguo
- Nature Materials, Vol. 4, Issue 2
Indistinguishable photons from a single-photon device
journal, October 2002
- Santori, Charles; Fattal, David; Vučković, Jelena
- Nature, Vol. 419, Issue 6907
Single-Exciton Gain and Stimulated Emission Across the Infrared Telecom Band from Robust Heavily Doped PbS Colloidal Quantum Dots
journal, July 2020
- Christodoulou, Sotirios; Ramiro, Iñigo; Othonos, Andreas
- Nano Letters, Vol. 20, Issue 8
Solution-processed, high-performance light-emitting diodes based on quantum dots
journal, October 2014
- Dai, Xingliang; Zhang, Zhenxing; Jin, Yizheng
- Nature, Vol. 515, Issue 7525
Ultralong Dephasing Time in InGaAs Quantum Dots
journal, September 2001
- Borri, P.; Langbein, W.; Schneider, S.
- Physical Review Letters, Vol. 87, Issue 15
Optical Gain and Stimulated Emission in Nanocrystal Quantum Dots
journal, October 2000
- Klimov, V. I.; Mikhailovsky, A. A.; Xu, Su
- Science, Vol. 290, Issue 5490, p. 314-317
Kinetics of the self-assembly of nanocrystal superlattices measured by real-time in situ X-ray scattering
journal, March 2016
- Weidman, Mark C.; Smilgies, Detlef-M.; Tisdale, William A.
- Nature Materials, Vol. 15, Issue 7
Photovoltage field-effect transistors
journal, February 2017
- Adinolfi, Valerio; Sargent, Edward H.
- Nature, Vol. 542, Issue 7641
Accelerating the discovery of materials for clean energy in the era of smart automation
journal, April 2018
- Tabor, Daniel P.; Roch, Loïc M.; Saikin, Semion K.
- Nature Reviews Materials, Vol. 3, Issue 5
Direct optical lithography of functional inorganic nanomaterials
journal, July 2017
- Wang, Yuanyuan; Fedin, Igor; Zhang, Hao
- Science, Vol. 357, Issue 6349
Direct formation of quantum‐sized dots from uniform coherent islands of InGaAs on GaAs surfaces
journal, December 1993
- Leonard, D.; Krishnamurthy, M.; Reaves, C. M.
- Applied Physics Letters, Vol. 63, Issue 23
Long-range orientation and atomic attachment of nanocrystals in 2D honeycomb superlattices
journal, May 2014
- Boneschanscher, M. P.; Evers, W. H.; Geuchies, J. J.
- Science, Vol. 344, Issue 6190
Charge transport in semiconductors assembled from nanocrystal quantum dots
journal, June 2020
- Yazdani, Nuri; Andermatt, Samuel; Yarema, Maksym
- Nature Communications, Vol. 11, Issue 1
High-Performance CuInS 2 Quantum Dot Laminated Glass Luminescent Solar Concentrators for Windows
journal, January 2018
- Bergren, Matthew R.; Makarov, Nikolay S.; Ramasamy, Karthik
- ACS Energy Letters, Vol. 3, Issue 3
Field-emission from quantum-dot-in-perovskite solids
journal, March 2017
- García de Arquer, F. Pelayo; Gong, Xiwen; Sabatini, Randy P.
- Nature Communications, Vol. 8, Issue 1
Quantum correlation among photons from a single quantum dot at room temperature
journal, August 2000
- Michler, P.; Imamoğlu, A.; Mason, M. D.
- Nature, Vol. 406, Issue 6799
Visible quantum dot light-emitting diodes with simultaneous high brightness and efficiency
journal, February 2019
- Shen, Huaibin; Gao, Qiang; Zhang, Yanbin
- Nature Photonics, Vol. 13, Issue 3
A colloidal quantum dot infrared photodetector and its use for intraband detection
journal, May 2019
- Livache, Clément; Martinez, Bertille; Goubet, Nicolas
- Nature Communications, Vol. 10, Issue 1
Large-area luminescent solar concentrators based on ‘Stokes-shift-engineered’ nanocrystals in a mass-polymerized PMMA matrix
journal, April 2014
- Meinardi, Francesco; Colombo, Annalisa; Velizhanin, Kirill A.
- Nature Photonics, Vol. 8, Issue 5, p. 392-399
Multicarrier Interactions in Semiconductor Nanocrystals in Relation to the Phenomena of Auger Recombination and Carrier Multiplication
journal, March 2014
- Klimov, Victor I.
- Annual Review of Condensed Matter Physics, Vol. 5, Issue 1
Understanding intermediate-band solar cells
journal, February 2012
- Luque, Antonio; Martí, Antonio; Stanley, Colin
- Nature Photonics, Vol. 6, Issue 3
Quantum-Dot Single-Photon Sources for Entanglement Enhanced Interferometry
journal, June 2017
- Müller, M.; Vural, H.; Schneider, C.
- Physical Review Letters, Vol. 118, Issue 25
Bridging Two Worlds: Colloidal versus Epitaxial Quantum Dots
journal, May 2019
- Bayer, Manfred
- Annalen der Physik
Mid-infrared HgTe colloidal quantum dot photodetectors
journal, July 2011
- Keuleyan, Sean; Lhuillier, Emmanuel; Brajuskovic, Vuk
- Nature Photonics, Vol. 5, Issue 8
Machine Learning Accelerates Discovery of Optimal Colloidal Quantum Dot Synthesis
journal, September 2019
- Voznyy, Oleksandr; Levina, Larissa; Fan, James Z.
- ACS Nano, Vol. 13, Issue 10
Dual-band infrared imaging using stacked colloidal quantum dot photodiodes
journal, February 2019
- Tang, Xin; Ackerman, Matthew M.; Chen, Menglu
- Nature Photonics, Vol. 13, Issue 4
Current status and technological prospect of photodetectors based on two-dimensional materials
journal, December 2018
- Konstantatos, Gerasimos
- Nature Communications, Vol. 9, Issue 1
Low-threshold amplified spontaneous emission and lasing from colloidal nanocrystals of caesium lead halide perovskites
journal, August 2015
- Yakunin, Sergii; Protesescu, Loredana; Krieg, Franziska
- Nature Communications, Vol. 6, Issue 1
Rabi Oscillations of Excitons in Single Quantum Dots
journal, September 2001
- Stievater, T. H.; Li, Xiaoqin; Steel, D. G.
- Physical Review Letters, Vol. 87, Issue 13
Ligand-assisted cation-exchange engineering for high-efficiency colloidal Cs1−xFAxPbI3 quantum dot solar cells with reduced phase segregation
journal, January 2020
- Hao, Mengmeng; Bai, Yang; Zeiske, Stefan
- Nature Energy, Vol. 5, Issue 1
Regulated and Entangled Photons from a Single Quantum Dot
journal, March 2000
- Benson, Oliver; Santori, Charles; Pelton, Matthew
- Physical Review Letters, Vol. 84, Issue 11
Improved performance and stability in quantum dot solar cells through band alignment engineering
journal, May 2014
- Chuang, Chia-Hao M.; Brown, Patrick R.; Bulović, Vladimir
- Nature Materials, Vol. 13, Issue 8, p. 796-801
Themed issue on water splitting and photocatalysis
journal, January 2016
- Boettcher, Shannon W.; Mallouk, Thomas E.; Osterloh, Frank E.
- Journal of Materials Chemistry A, Vol. 4, Issue 8
Colloidal Quantum Dot Photovoltaics: Current Progress and Path to Gigawatt Scale Enabled by Smart Manufacturing
journal, August 2020
- Kirmani, Ahmad R.; Luther, Joseph M.; Abolhasani, Milad
- ACS Energy Letters, Vol. 5, Issue 9
Highly Efficient and Stable CO 2 Reduction Photocatalyst with a Hierarchical Structure of Mesoporous TiO 2 on 3D Graphene with Few-Layered MoS 2
journal, April 2018
- Jung, Hyunju; Cho, Kyeong Min; Kim, Kyoung Hwan
- ACS Sustainable Chemistry & Engineering, Vol. 6, Issue 5
Air-Stable All-Inorganic Nanocrystal Solar Cells Processed from Solution
journal, October 2005
- Gur, Ilan; Fromer, Neil A.; Geier, Michael L.
- Science, Vol. 310, Issue 5747, p. 462-465
Hong–Ou–Mandel interference of two phonons in trapped ions
journal, November 2015
- Toyoda, Kenji; Hiji, Ryoto; Noguchi, Atsushi
- Nature, Vol. 527, Issue 7576
The present status of quantum dot lasers
journal, December 1999
- Grundmann, Marius
- Physica E: Low-dimensional Systems and Nanostructures, Vol. 5, Issue 3
Thirty Years of Luminescent Solar Concentrator Research: Solar Energy for the Built Environment
journal, December 2011
- Debije, Michael G.; Verbunt, Paul P. C.
- Advanced Energy Materials, Vol. 2, Issue 1
Carbon Dots in Solar-to-Hydrogen Conversion
journal, July 2020
- Luo, Hui; Guo, Qian; Szilágyi, Petra Ágota
- Trends in Chemistry, Vol. 2, Issue 7
Electronic wave functions in semiconductor clusters: experiment and theory
journal, June 1986
- Brus, Louis
- The Journal of Physical Chemistry, Vol. 90, Issue 12, p. 2555-2560
High-efficiency quantum-dot light-emitting devices with enhanced charge injection
journal, April 2013
- Mashford, Benjamin S.; Stevenson, Matthew; Popovic, Zoran
- Nature Photonics, Vol. 7, Issue 5
Suppression of Auger Processes in Confined Structures
journal, January 2010
- Cragg, George E.; Efros, Alexander L.
- Nano Letters, Vol. 10, Issue 1
Solution-processed semiconductors for next-generation photodetectors
journal, January 2017
- García de Arquer, F. Pelayo; Armin, Ardalan; Meredith, Paul
- Nature Reviews Materials, Vol. 2, Issue 3
Bright solid-state sources of indistinguishable single photons
journal, February 2013
- Gazzano, O.; Michaelis de Vasconcellos, S.; Arnold, C.
- Nature Communications, Vol. 4, Issue 1
Single Photons from a Hot Solid-State Emitter at 350 K
journal, March 2016
- Holmes, Mark J.; Kako, Satoshi; Choi, Kihyun
- ACS Photonics, Vol. 3, Issue 4
Epitaxial Dimers and Auger-Assisted Detrapping in PbS Quantum Dot Solids
journal, July 2019
- Gilmore, Rachel H.; Liu, Yun; Shcherbakov-Wu, Wenbi
- Matter, Vol. 1, Issue 1
Synthesis and Characterization of InP Quantum Dots
journal, May 1994
- Micic, Olga I.; Curtis, Calvin J.; Jones, Kim M.
- The Journal of Physical Chemistry, Vol. 98, Issue 19
Optical gain in colloidal quantum dots achieved with direct-current electrical pumping
journal, November 2017
- Lim, Jaehoon; Park, Young-Shin; Klimov, Victor I.
- Nature Materials, Vol. 17, Issue 1
Ultrafast coherent control and suppressed nuclear feedback of a single quantum dot hole qubit
journal, August 2011
- De Greve, Kristiaan; McMahon, Peter L.; Press, David
- Nature Physics, Vol. 7, Issue 11
Nanocrystals of Cesium Lead Halide Perovskites (CsPbX 3 , X = Cl, Br, and I): Novel Optoelectronic Materials Showing Bright Emission with Wide Color Gamut
journal, February 2015
- Protesescu, Loredana; Yakunin, Sergii; Bodnarchuk, Maryna I.
- Nano Letters, Vol. 15, Issue 6
Controlled Alloying of the Core–Shell Interface in CdSe/CdS Quantum Dots for Suppression of Auger Recombination
journal, April 2013
- Bae, Wan Ki; Padilha, Lazaro A.; Park, Young-Shin
- ACS Nano, Vol. 7, Issue 4
Lead Salt Quantum Dots: the Limit of Strong Quantum Confinement
journal, November 2000
- Wise, Frank W.
- Accounts of Chemical Research, Vol. 33, Issue 11
High Efficiency Carrier Multiplication in PbSe Nanocrystals: Implications for Solar Energy Conversion
journal, May 2004
- Schaller, R. D.; Klimov, V. I.
- Physical Review Letters, Vol. 92, Issue 18
Structural diversity in binary nanoparticle superlattices
journal, January 2006
- Shevchenko, Elena V.; Talapin, Dmitri V.; Kotov, Nicholas A.
- Nature, Vol. 439, Issue 7072, p. 55-59
Performance Limits of Luminescent Solar Concentrators Tested with Seed/Quantum-Well Quantum Dots in a Selective-Reflector-Based Optical Cavity
journal, December 2017
- Song, Hyung-Jun; Jeong, Byeong Guk; Lim, Jaehoon
- Nano Letters, Vol. 18, Issue 1
Red, Yellow, Green, and Blue Amplified Spontaneous Emission and Lasing Using Colloidal CdSe Nanoplatelets
journal, September 2015
- She, Chunxing; Fedin, Igor; Dolzhnikov, Dmitriy S.
- ACS Nano, Vol. 9, Issue 10
Toward Full-Color Electroluminescent Quantum Dot Displays
journal, December 2020
- Yang, Jiwoong; Choi, Moon Kee; Yang, U. Jeong
- Nano Letters, Vol. 21, Issue 1
Droplet epitaxy of semiconductor nanostructures for quantum photonic devices
journal, May 2019
- Gurioli, Massimo; Wang, Zhiming; Rastelli, Armando
- Nature Materials, Vol. 18, Issue 8
Towards zero-threshold optical gain using charged semiconductor quantum dots
journal, October 2017
- Wu, Kaifeng; Park, Young-Shin; Lim, Jaehoon
- Nature Nanotechnology, Vol. 12, Issue 12
Self-Organization of CdSe Nanocrystallites into Three-Dimensional Quantum Dot Superlattices
journal, November 1995
- Murray, C. B.; Kagan, C. R.; Bawendi, M. G.
- Science, Vol. 270, Issue 5240
Cation exchange assisted synthesis of ZnCdSe/ZnSe quantum dots with narrow emission line widths and near-unity photoluminescence quantum yields
journal, January 2020
- Jin, Xiao; Xie, Kanlin; Zhang, Tingting
- Chemical Communications, Vol. 56, Issue 45
A review of carbon quantum dots and their applications in wastewater treatment
journal, April 2020
- Rani, Umairah Abd; Ng, Law Yong; Ng, Ching Yin
- Advances in Colloid and Interface Science, Vol. 278
Semiconductor crystallites: a class of large molecules
journal, June 1990
- Steigerwald, Michael L.; Brus, Louis E.
- Accounts of Chemical Research, Vol. 23, Issue 6
Molecular beam epitaxy
journal, January 1975
- Cho, A. Y.; Arthur, J. R.
- Progress in Solid State Chemistry, Vol. 10
Monodisperse, Air-Stable PbS Nanocrystals via Precursor Stoichiometry Control
journal, May 2014
- Weidman, Mark C.; Beck, Megan E.; Hoffman, Rachel S.
- ACS Nano, Vol. 8, Issue 6
A colloidal quantum dot spectrometer
journal, July 2015
- Bao, Jie; Bawendi, Moungi G.
- Nature, Vol. 523, Issue 7558
Highly efficient large-area colourless luminescent solar concentrators using heavy-metal-free colloidal quantum dots
journal, August 2015
- Meinardi, Francesco; McDaniel, Hunter; Carulli, Francesco
- Nature Nanotechnology, Vol. 10, Issue 10
Superstructures generated from truncated tetrahedral quantum dots
journal, September 2018
- Nagaoka, Yasutaka; Tan, Rui; Li, Ruipeng
- Nature, Vol. 561, Issue 7723
Quantum-dot infrared photodetectors: Status and outlook
journal, January 2008
- Martyniuk, P.; Rogalski, A.
- Progress in Quantum Electronics, Vol. 32, Issue 3-4
Quantization of Multiparticle Auger Rates in Semiconductor Quantum Dots
journal, February 2000
- Klimov, V. I.
- Science, Vol. 287, Issue 5455
Electrically-driven single-photon sources based on colloidal quantum dots with near-optimal antibunching at room temperature
journal, October 2017
- Lin, Xing; Dai, Xingliang; Pu, Chaodan
- Nature Communications, Vol. 8, Issue 1
Multidimensional quantum well laser and temperature dependence of its threshold current
journal, June 1982
- Arakawa, Y.; Sakaki, H.
- Applied Physics Letters, Vol. 40, Issue 11
Highly efficient quantum dot near-infrared light-emitting diodes
journal, February 2016
- Gong, Xiwen; Yang, Zhenyu; Walters, Grant
- Nature Photonics, Vol. 10, Issue 4
Continuous-wave lasing in colloidal quantum dot solids enabled by facet-selective epitaxy
journal, March 2017
- Fan, Fengjia; Voznyy, Oleksandr; Sabatini, Randy P.
- Nature, Vol. 544, Issue 7648
Suppressed Auger Recombination in “Giant” Nanocrystals Boosts Optical Gain Performance
journal, October 2009
- García-Santamaría, Florencio; Chen, Yongfen; Vela, Javier
- Nano Letters, Vol. 9, Issue 10
Colloidal Quantum Dots Intraband Photodetectors
journal, October 2014
- Deng, Zhiyou; Jeong, Kwang Seob; Guyot-Sionnest, Philippe
- ACS Nano, Vol. 8, Issue 11
Efficiency Limit of Colloidal Quantum Dot Solar Cells: Effect of Optical Interference on Active Layer Absorption
journal, November 2019
- Kim, Taewan; Jin, Xing; Song, Jung Hoon
- ACS Energy Letters, Vol. 5, Issue 1
Hybrid graphene–quantum dot phototransistors with ultrahigh gain
journal, May 2012
- Konstantatos, Gerasimos; Badioli, Michela; Gaudreau, Louis
- Nature Nanotechnology, Vol. 7, Issue 6
A Low-Temperature Solution Phase Route for the Synthesis of Silicon Nanoclusters
journal, January 1996
- Bley, Richard A.; Kauzlarich, Susan M.
- Journal of the American Chemical Society, Vol. 118, Issue 49
Solution-processed inorganic bulk nano-heterojunctions and their application to solar cells
journal, July 2012
- Rath, Arup K.; Bernechea, Maria; Martinez, Luis
- Nature Photonics, Vol. 6, Issue 8
Growth by molecular beam epitaxy and characterization of InAs/GaAs strained‐layer superlattices
journal, November 1985
- Goldstein, L.; Glas, F.; Marzin, J. Y.
- Applied Physics Letters, Vol. 47, Issue 10
Coherent Manipulation of Coupled Electron Spins in Semiconductor Quantum Dots
journal, September 2005
- Petta, J. R.
- Science, Vol. 309, Issue 5744
PbS Colloidal Quantum Dot Inks for Infrared Solar Cells
journal, November 2020
- Zheng, Siyu; Chen, Jingxuan; Johansson, Erik M. J.
- iScience, Vol. 23, Issue 11
A Quantum Dot Single-Photon Turnstile Device
journal, December 2000
- Michler, P.
- Science, Vol. 290, Issue 5500
Optically pumped colloidal-quantum-dot lasing in LED-like devices with an integrated optical cavity
journal, January 2020
- Roh, Jeongkyun; Park, Young-Shin; Lim, Jaehoon
- Nature Communications, Vol. 11, Issue 1
Fast, sensitive and spectrally tuneable colloidal-quantum-dot photodetectors
journal, November 2008
- Clifford, Jason P.; Konstantatos, Gerasimos; Johnston, Keith W.
- Nature Nanotechnology, Vol. 4, Issue 1
Giant Modal Gain Coefficients in Colloidal II–VI Nanoplatelets
journal, December 2018
- Guzelturk, Burak; Pelton, Matthew; Olutas, Murat
- Nano Letters, Vol. 19, Issue 1
Efficient near-infrared light-emitting diodes based on quantum dots in layered perovskite
journal, January 2020
- Gao, Liang; Quan, Li Na; García de Arquer, F. Pelayo
- Nature Photonics, Vol. 14, Issue 4
High-performance InAs quantum-dot infrared photodetectors grown on InP substrate operating at room temperature
journal, March 2007
- Lim, H.; Tsao, S.; Zhang, W.
- Applied Physics Letters, Vol. 90, Issue 13
Luminescent greenhouse collector for solar radiation
journal, January 1976
- Weber, W. H.; Lambe, John
- Applied Optics, Vol. 15, Issue 10
Monolayer Perovskite Bridges Enable Strong Quantum Dot Coupling for Efficient Solar Cells
journal, July 2020
- Sun, Bin; Johnston, Andrew; Xu, Chao
- Joule, Vol. 4, Issue 7
Bright colloidal quantum dot light-emitting diodes enabled by efficient chlorination
journal, February 2018
- Li, Xiyan; Zhao, Yong-Biao; Fan, Fengjia
- Nature Photonics, Vol. 12, Issue 3
All-inorganic perovskite nanocrystal scintillators
journal, August 2018
- Chen, Qiushui; Wu, Jing; Ou, Xiangyu
- Nature, Vol. 561, Issue 7721
Temperature-Insensitive Eye-Opening under 10-Gb/s Modulation of 1.3-µm P-Doped Quantum-Dot Lasers without Current Adjustments
journal, July 2004
- Otsubo, Koji; Hatori, Nobuaki; Ishida, Mitsuru
- Japanese Journal of Applied Physics, Vol. 43, Issue No. 8B
Fast and Sensitive Colloidal Quantum Dot Mid-Wave Infrared Photodetectors
journal, June 2018
- Ackerman, Matthew M.; Tang, Xin; Guyot-Sionnest, Philippe
- ACS Nano, Vol. 12, Issue 7
Highly efficient and stable InP/ZnSe/ZnS quantum dot light-emitting diodes
journal, November 2019
- Won, Yu-Ho; Cho, Oul; Kim, Taehyung
- Nature, Vol. 575, Issue 7784
Effect of Auger Recombination on Lasing in Heterostructured Quantum Dots with Engineered Core/Shell Interfaces
journal, October 2015
- Park, Young-Shin; Bae, Wan Ki; Baker, Thomas
- Nano Letters, Vol. 15, Issue 11
Spectroscopic insights into high defect tolerance of Zn:CuInSe2 quantum-dot-sensitized solar cells
journal, May 2020
- Du, Jun; Singh, Rohan; Fedin, Igor
- Nature Energy, Vol. 5, Issue 5
Plastic waste as a feedstock for solar-driven H 2 generation
journal, January 2018
- Uekert, Taylor; Kuehnel, Moritz F.; Wakerley, David W.
- Energy & Environmental Science, Vol. 11, Issue 10
Quantum dot bioconjugates for imaging, labelling and sensing
journal, June 2005
- Medintz, Igor L.; Uyeda, H. Tetsuo; Goldman, Ellen R.
- Nature Materials, Vol. 4, Issue 6, p. 435-446
Spontaneous Emission Characteristics of Quantum Well Lasers in Strong Magnetic Fields -- An Approach to Quantum-Well-Box Light Source --
journal, December 1983
- Arakawa, Yasuhiko; Sakaki, Hiroyuki; Nishioka, Masao
- Japanese Journal of Applied Physics, Vol. 22, Issue Part 2, No. 12
Quantum size effects in the redox potentials, resonance Raman spectra, and electronic spectra of CdS crystallites in aqueous solution
journal, July 1983
- Rossetti, R.; Nakahara, S.; Brus, L. E.
- The Journal of Chemical Physics, Vol. 79, Issue 2
Semiconductor Quantum Dots: An Emerging Candidate for CO 2 Photoreduction
journal, June 2019
- Wu, Hao‐Lin; Li, Xu‐Bing; Tung, Chen‐Ho
- Advanced Materials, Vol. 31, Issue 36
Hybrid organic–inorganic inks flatten the energy landscape in colloidal quantum dot solids
journal, November 2016
- Liu, Mengxia; Voznyy, Oleksandr; Sabatini, Randy
- Nature Materials, Vol. 16, Issue 2
Entangled Photon Pairs from Semiconductor Quantum Dots
journal, April 2006
- Akopian, N.; Lindner, N. H.; Poem, E.
- Physical Review Letters, Vol. 96, Issue 13
The surface science of nanocrystals
journal, January 2016
- Boles, Michael A.; Ling, Daishun; Hyeon, Taeghwan
- Nature Materials, Vol. 15, Issue 2
Origins of Low Quantum Efficiencies in Quantum Dot LEDs
journal, January 2013
- Bozyigit, Deniz; Yarema, Olesya; Wood, Vanessa
- Advanced Functional Materials, Vol. 23, Issue 24
Doped Nanocrystals
journal, March 2008
- Norris, D. J.; Efros, A. L.; Erwin, S. C.
- Science, Vol. 319, Issue 5871
Enhanced optical path and electron diffusion length enable high-efficiency perovskite tandems
journal, March 2020
- Chen, Bin; Baek, Se-Woong; Hou, Yi
- Nature Communications, Vol. 11, Issue 1
On-demand generation of background-free single photons from a solid-state source
journal, February 2018
- Schweickert, Lucas; Jöns, Klaus D.; Zeuner, Katharina D.
- Applied Physics Letters, Vol. 112, Issue 9
Deterministic generation of a cluster state of entangled photons
journal, September 2016
- Schwartz, I.; Cogan, D.; Schmidgall, E. R.
- Science, Vol. 354, Issue 6311
Electronic states of semiconductor clusters: Homogeneous and inhomogeneous broadening of the optical spectrum
journal, October 1988
- Alivisatos, A. P.; Harris, A. L.; Levinos, N. J.
- The Journal of Chemical Physics, Vol. 89, Issue 7
Low Dark Current High Gain InAs Quantum Dot Avalanche Photodiodes Monolithically Grown on Si
journal, January 2020
- Chen, Baile; Wan, Yating; Xie, Zhiyang
- ACS Photonics, Vol. 7, Issue 2
Mode Locking of Electron Spin Coherences in Singly Charged Quantum Dots
journal, July 2006
- Greilich, A.
- Science, Vol. 313, Issue 5785
Quantum-dot-in-perovskite solids
journal, July 2015
- Ning, Zhijun; Gong, Xiwen; Comin, Riccardo
- Nature, Vol. 523, Issue 7560
Quantum-Dot Light-Emitting Diodes for Large-Area Displays: Towards the Dawn of Commercialization
journal, March 2017
- Dai, Xingliang; Deng, Yunzhou; Peng, Xiaogang
- Advanced Materials, Vol. 29, Issue 14
Quantum Dot Luminescent Concentrator Cavity Exhibiting 30-fold Concentration
journal, August 2015
- Bronstein, Noah D.; Yao, Yuan; Xu, Lu
- ACS Photonics, Vol. 2, Issue 11
Surface Traps in Colloidal Quantum Dots: A Combined Experimental and Theoretical Perspective
journal, October 2017
- Giansante, Carlo; Infante, Ivan
- The Journal of Physical Chemistry Letters, Vol. 8, Issue 20
Lead sulphide nanocrystal photodetector technologies
journal, January 2016
- Saran, Rinku; Curry, Richard J.
- Nature Photonics, Vol. 10, Issue 2
Road Map for Nanocrystal Based Infrared Photodetectors
journal, November 2018
- Livache, Clément; Martinez, Bertille; Goubet, Nicolas
- Frontiers in Chemistry, Vol. 6
Setting Carriers Free: Healing Faulty Interfaces Promotes Delocalization and Transport in Nanocrystal Solids
journal, November 2019
- Walravens, Willem; Solano, Eduardo; Geenen, Filip
- ACS Nano, Vol. 13, Issue 11
Sub–single-exciton lasing using charged quantum dots coupled to a distributed feedback cavity
journal, August 2019
- Kozlov, Oleg V.; Park, Young-Shin; Roh, Jeongkyun
- Science, Vol. 365, Issue 6454
Luminescent solar concentrators for building-integrated photovoltaics
journal, November 2017
- Meinardi, Francesco; Bruni, Francesco; Brovelli, Sergio
- Nature Reviews Materials, Vol. 2, Issue 12
Coherent single-photon emission from colloidal lead halide perovskite quantum dots
journal, February 2019
- Utzat, Hendrik; Sun, Weiwei; Kaplan, Alexander E. K.
- Science, Vol. 363, Issue 6431
Designing the Surfaces of Semiconductor Quantum Dots for Colloidal Photocatalysis
journal, April 2017
- Weiss, Emily A.
- ACS Energy Letters, Vol. 2, Issue 5
Photocatalytic fixation of nitrogen to ammonia: state-of-the-art advancements and future prospects
journal, January 2018
- Chen, Xingzhu; Li, Neng; Kong, Zhouzhou
- Materials Horizons, Vol. 5, Issue 1
A tunable library of substituted thiourea precursors to metal sulfide nanocrystals
journal, June 2015
- Hendricks, M. P.; Campos, M. P.; Cleveland, G. T.
- Science, Vol. 348, Issue 6240
Solar-driven reforming of lignocellulose to H2 with a CdS/CdOx photocatalyst
journal, March 2017
- Wakerley, David W.; Kuehnel, Moritz F.; Orchard, Katherine L.
- Nature Energy, Vol. 2, Issue 4
Self-doped colloidal semiconductor nanocrystals with intraband transitions in steady state
journal, January 2018
- Kim, Jihye; Choi, Dongsun; Jeong, Kwang Seob
- Chemical Communications, Vol. 54, Issue 61
Designed Assembly and Integration of Colloidal Nanocrystals for Device Applications
journal, December 2015
- Yang, Jiwoong; Choi, Moon Kee; Kim, Dae-Hyeong
- Advanced Materials, Vol. 28, Issue 6
The coordination chemistry of nanocrystal surfaces
journal, February 2015
- Owen, Jonathan
- Science, Vol. 347, Issue 6222
Colloidal Synthesis of Semiconductor Quantum Dots toward Large-Scale Production: A Review
journal, February 2018
- Pu, Yuan; Cai, Fuhong; Wang, Dan
- Industrial & Engineering Chemistry Research, Vol. 57, Issue 6
Near-optimal single-photon sources in the solid state
journal, March 2016
- Somaschi, N.; Giesz, V.; De Santis, L.
- Nature Photonics, Vol. 10, Issue 5
Enabling Visible-Light-Driven Selective CO 2 Reduction by Doping Quantum Dots: Trapping Electrons and Suppressing H 2 Evolution
journal, November 2018
- Wang, Jin; Xia, Tong; Wang, Lei
- Angewandte Chemie International Edition, Vol. 57, Issue 50
A Coherent Single-Hole Spin in a Semiconductor
journal, July 2009
- Brunner, Daniel; Gerardot, Brian D.; Dalgarno, Paul A.
- Science, Vol. 325, Issue 5936
Band-like transport, high electron mobility and high photoconductivity in all-inorganic nanocrystal arrays
journal, April 2011
- Lee, Jong-Soo; Kovalenko, Maksym V.; Huang, Jing
- Nature Nanotechnology, Vol. 6, Issue 6
Broadband image sensor array based on graphene–CMOS integration
journal, May 2017
- Goossens, Stijn; Navickaite, Gabriele; Monasterio, Carles
- Nature Photonics, Vol. 11, Issue 6
PbSe Nanocrystal-Based Infrared-to-Visible Up-Conversion Device
journal, May 2011
- Kim, Do Young; Choudhury, Kaushik Roy; Lee, Jae Woong
- Nano Letters, Vol. 11, Issue 5
Doctor-blade deposition of quantum dots onto standard window glass for low-loss large-area luminescent solar concentrators
journal, October 2016
- Li, Hongbo; Wu, Kaifeng; Lim, Jaehoon
- Nature Energy, Vol. 1, Issue 12
One-Step Synthesis of Highly Luminescent Carbon Dots in Noncoordinating Solvents
journal, August 2010
- Wang, Fu; Pang, Shuping; Wang, Long
- Chemistry of Materials, Vol. 22, Issue 16
Superfluorescence from lead halide perovskite quantum dot superlattices
journal, November 2018
- Rainò, Gabriele; Becker, Michael A.; Bodnarchuk, Maryna I.
- Nature, Vol. 563, Issue 7733
Photo-FETs: Phototransistors Enabled by 2D and 0D Nanomaterials
journal, November 2016
- Kufer, Dominik; Konstantatos, Gerasimos
- ACS Photonics, Vol. 3, Issue 12
High-efficiency, deep blue ZnCdS/Cd x Zn 1−x S/ZnS quantum-dot-light-emitting devices with an EQE exceeding 18%
journal, January 2018
- Wang, Ouyang; Wang, Lei; Li, Zhaohan
- Nanoscale, Vol. 10, Issue 12
Open-Circuit Voltage Deficit, Radiative Sub-Bandgap States, and Prospects in Quantum Dot Solar Cells
journal, April 2015
- Chuang, Chia-Hao Marcus; Maurano, Andrea; Brandt, Riley E.
- Nano Letters, Vol. 15, Issue 5
Color Converting Film With Quantum-Dots for the Liquid Crystal Displays Based on Inkjet Printing
journal, June 2019
- Huang, Bing-Le; Guo, Tai-Liang; Xu, Sheng
- IEEE Photonics Journal, Vol. 11, Issue 3