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Title: Chiral spin liquid with spinon Fermi surfaces in the spin-$$\frac{1}{2}$$ triangular Heisenberg model

Journal Article · · Physical Review. B
ORCiD logo [1];  [2];  [3];  [2];  [4]
  1. Beihang University, Beijing (China); OSTI
  2. The Ohio State Univ., Columbus, OH (United States)
  3. California State Univ., Northridge, CA (United States); Univ. of California, San Diego, CA (United States)
  4. California State Univ., Northridge, CA (United States)

Here, we study the interplay of competing interactions in spin-$$\frac{1}{2}$$ triangular Heisenberg model through tuning the first- ($$J_1$$), second- ($$J_2$$), and third-neighbor ($$J_ 3$$) couplings. Based on a large-scale density-matrix renormalization group calculation, we identify a quantum phase diagram of the system and discover a gapless chiral spin-liquid (CSL) phase in the intermediate $$J_2$$ and $$J_ 3$$ regime. This CSL state spontaneously breaks time-reversal symmetry with finite scalar chiral order, and it has gapless excitations implied by a vanishing spin triplet gap and a finite central charge on the cylinder. Moreover, the central charge grows rapidly with the cylinder circumference, indicating emergent spinon Fermi surfaces. To understand the numerical results we propose a parton mean-field spin-liquid state, the U(1) staggered flux state, which breaks time-reversal symmetry with chiral edge modes by adding a Chern insulator mass to Dirac spinons in the U(1) Dirac spin liquid. This state also breaks lattice rotational symmetries and possesses two spinon Fermi surfaces driven by nonzero $$J_2$$ and $$J_3$$, which naturally explains the numerical results. This realizes an example of a gapless CSL state with coexisting spinon Fermi surfaces and chiral edge states, demonstrating the rich family of interesting quantum phases emergent from competing interactions in triangular-lattice magnets.

Research Organization:
California State Univ. (CalState), Long Beach, CA (United States)
Sponsoring Organization:
Fundamental Research Funds for the Central Universities; National Natural Science Foundation of China (NSFC); National Science Foundation (NSF); USDOE Office of Science (SC), Basic Energy Sciences (BES)
Grant/Contract Number:
FG02-06ER46305
OSTI ID:
1800369
Journal Information:
Physical Review. B, Journal Name: Physical Review. B Journal Issue: 24 Vol. 100; ISSN 2469-9950
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English

References (93)

Electron scattering on magnetic impurities in metals and anomalous resistivity effects journal September 1965
The half-filled Landau level: The case for Dirac composite fermions journal April 2016
The evolution and breakdown of submesoscale instabilities text January 2018
Spin-driven ferroelectricity and possible antiferroelectricity in triangular lattice antiferromagnets ACrO2 (A = Cu, Ag, Li, or Na) text January 2008
Quantum Spin Liquids text January 2016
Resonating valence bonds: A new kind of insulator? journal February 1973
Spiral phases in easy plane J1-J2-J3 triangular antiferromagnets journal February 1995
Anyons in an exactly solved model and beyond journal January 2006
Spin liquids in frustrated magnets journal March 2010
Thermal-transport measurements in a quantum spin-liquid state of the frustrated triangular magnet κ-(BEDT-TTF)2Cu2(CN)3 journal November 2008
Continuous excitations of the triangular-lattice quantum spin liquid YbMgGaO4 journal December 2016
A high-temperature quantum spin liquid with polaron spins journal July 2017
Thermodynamic properties of a spin-1/2 spin-liquid state in a κ-type organic salt journal April 2008
Fractionalized excitations in the partially magnetized spin liquid candidate YbMgGaO4 journal October 2018
Unifying description of competing orders in two-dimensional quantum magnets journal September 2019
A quantum dipolar spin liquid journal February 2018
Emergent Chiral Spin Liquid: Fractional Quantum Hall Effect in a Kagome Heisenberg Model journal September 2014
1T-TaS 2 as a quantum spin liquid journal June 2017
Quantum spin liquids: a review journal November 2016
Neutron powder diffraction study of the two-dimensional triangular lattice antiferromagnet CuCrO 2 journal May 1990
Entanglement entropy and quantum field theory journal June 2004
Gapless fermions and gauge fields in dielectrics journal May 1989
Mean-field theory of spin-liquid states with finite energy gap and topological orders journal August 1991
Kagome´- and triangular-lattice Heisenberg antiferromagnets: Ordering from quantum fluctuations and quantum-disordered ground states with unconfined bosonic spinons journal June 1992
Gauge theory of the normal state of high- T c superconductors journal September 1992
Spin-liquid phase of the multiple-spin exchange Hamiltonian on the triangular lattice journal July 1999
Z 2 gauge theory of electron fractionalization in strongly correlated systems journal September 2000
Quantum orders and symmetric spin liquids journal April 2002
Variational study of triangular lattice spin- 1 ∕ 2 model with ring exchanges and spin liquid state in κ − ( ET ) 2 Cu 2 ( CN ) 3 journal July 2005
Inversion-symmetry breaking in the noncollinear magnetic phase of the triangular-lattice antiferromagnet Cu Fe O 2 journal June 2006
Spin Bose-metal phase in a spin- 1 2 model with ring exchange on a two-leg triangular strip journal May 2009
Quasiclassical magnetic order and its loss in a spin- 1 2 Heisenberg antiferromagnet on a triangular lattice with competing bonds journal January 2015
Global phase diagram of competing ordered and quantum spin-liquid phases on the kagome lattice journal February 2015
Spin liquid phase of the S = 1 2 J 1 − J 2 Heisenberg model on the triangular lattice journal July 2015
Competing spin-liquid states in the spin- 1 2 Heisenberg model on the triangular lattice journal October 2015
Tensor network trial states for chiral topological phases in two dimensions and a no-go theorem in any dimension journal November 2015
Projective symmetry group classification of chiral spin liquids journal March 2016
Spin liquid nature in the Heisenberg J 1 − J 2 triangular antiferromagnet journal April 2016
Symmetric Z 2 spin liquids and their neighboring phases on triangular lattice journal April 2016
Symmetry fractionalization in the topological phase of the spin- 1 2 J 1 − J 2 triangular Heisenberg model journal September 2016
Spinon Fermi surface U ( 1 ) spin liquid in the spin-orbit-coupled triangular-lattice Mott insulator YbMgGaO 4 journal August 2017
Heat transport study of the spin liquid candidate 1 T − TaS 2 journal August 2017
Investigation of the chiral antiferromagnetic Heisenberg model using projected entangled pair states journal September 2017
Gapless excitations in the ground state of 1 T − TaS 2 journal November 2017
Entanglement Spectrum as a Generalization of Entanglement Entropy: Identification of Topological Order in Non-Abelian Fractional Quantum Hall Effect States journal July 2008
Spin-Driven Ferroelectricity in Triangular Lattice Antiferromagnets A CrO 2 ( A = Cu , Ag, Li, or Na) journal August 2008
Spin Bose-Metal and Valence Bond Solid Phases in a Spin- 1 / 2 Model with Ring Exchanges on a Four-Leg Triangular Ladder journal April 2011
Kapellasite: A Kagome Quantum Spin Liquid with Competing Interactions journal July 2012
Chiral Spin Liquid in a Frustrated Anisotropic Kagome Heisenberg Model journal April 2014
Rare-Earth Triangular Lattice Spin Liquid: A Single-Crystal Study of YbMgGaO 4 journal October 2015
Interaction-Driven Spontaneous Quantum Hall Effect on a Kagome Lattice journal August 2016
Topography of Spin Liquids on a Triangular Lattice journal May 2018
Spinon Fermi Surface in a Cluster Mott Insulator Model on a Triangular Lattice and Possible Application to 1 T − Ta S 2 journal July 2018
Dirac Spin Liquid on the Spin- 1 / 2 Triangular Heisenberg Antiferromagnet journal November 2019
Normal-state properties of the uniform resonating-valence-bond state journal May 1990
Large- N expansion for frustrated quantum antiferromagnets journal April 1991
Density matrix formulation for quantum renormalization groups journal November 1992
Fractionalization in the Cuprates: Detecting the Topological Order journal January 2001
Spin Liquid State in an Organic Mott Insulator with a Triangular Lattice journal September 2003
Mott Transition from a Spin Liquid to a Fermi Liquid in the Spin-Frustrated Organic Conductor κ − ( ET ) 2 Cu 2 ( CN ) 3 journal October 2005
Magnetic Interactions in the Geometrically Frustrated Triangular Lattice Antiferromagnet CuFeO 2 journal October 2007
Hierarchy of Exchange Interactions in the Triangular-Lattice Spin Liquid YbMgGaO 4 journal July 2018
Electron scattering on magnetic impurities in metals and anomalous resistivity effects journal September 1965
Doping a Mott insulator: Physics of high-temperature superconductivity journal January 2006
Quantum spin liquid states journal April 2017
Highly Mobile Gapless Excitations in a Two-Dimensional Candidate Quantum Spin Liquid journal June 2010
Spin-Liquid Ground State of the S = 1/2 Kagome Heisenberg Antiferromagnet journal April 2011
The half-filled Landau level: The case for Dirac composite fermions journal April 2016
Physics of the Kitaev Model: Fractionalization, Dynamic Correlations, and Material Connections journal March 2018
Topological Order: From Long-Range Entangled Quantum Matter to a Unified Origin of Light and Electrons journal January 2013
The non-Abelian density matrix renormalization group algorithm journal March 2002
Physics of the Kitaev model: fractionalization, dynamical correlations, and material connections text January 2018
Fractionalization in the Cuprates: Detecting the Topological Order text January 2001
Spin Liquid versus Spin Orbit Coupling on the Triangular Lattice journal January 2018
Fractionalization in the Cuprates: Detecting the Topological Order journal January 2008
Magnetic Interaction in the Geometrically Frustrated Triangular Lattice Antiferromagnet $\rm CuFeO_2$ text January 2007
Chiral spin liquid in a frustrated anisotropic kagome Heisenberg model text January 2013
Gapless spin-liquid phase in an extended spin 1/2 triangular Heisenberg model text January 2014
The half-filled Landau level: the case for Dirac composite fermions text January 2015
A Quantum Dipolar Spin Liquid text January 2015
Projective symmetry group classification of chiral spin liquids text January 2015
Symmetry fractionalization in the topological phase of the spin-$\frac{1}{2}$ $J_1$-$J_2$ triangular Heisenberg model text January 2016
Quantum Spin Liquid States text January 2016
Continuous excitations of the triangular-lattice quantum spin liquid YbMgGaO4 text January 2016
A new high-temperature quantum spin liquid with polaron spins text January 2017
Hierarchy of exchange interactions in the triangular-lattice spin-liquid YbMgGaO$_{4}$ text January 2017
Spin Liquid versus Spin Orbit Coupling on the Triangular Lattice text January 2017
Unifying Description of Competing Orders in Two Dimensional Quantum Magnets text January 2018
Fractionalization in the cuprates: Detecting the topological order text January 2000
The Non-Abelian Density Matrix Renormalization Group Algorithm text January 2000
Anyons in an exactly solved model and beyond text January 2005
Spin-Liquid phase of the Multiple-Spin Exchange Hamiltonian on the Triangular Lattice text January 1998
Gapless Spin-Liquid Phase in an Extended Spin 1/2 Triangular Heisenberg Model journal September 2014