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Title: NMR studies of the ground states of Ni50-xCoxMn35In15 (x=1, 2.5) and Ni45Co5Mn37In13 Heusler alloys

Abstract

Three temperature-induced phase transitions at T=T1, TM/TA, and TC, related to the ferromagnetic order of the martensitic phase (FMMP), martensitic (structural) transitions (MT), and the ferromagnetic order of the austenitic phase (FMAP), respectively, have been observed in the off-stoichiometric Heusler alloys, Ni50-xCoxMn35In15 (x=1, 2.5) and Ni45Co5Mn37In13. In this work, the phase transitions temperatures are found to be depended on alloy composition. A kinetic arrest of the AP was observed for Ni47.5Co2.5Mn35In15 in the magnetization measurements during field-cooling cycle (FCC) at 50 kOe. Depending upon the cooling protocols, ZFC and FCC (at H = 50 kOe), two different ground states of the alloys can be found in Ni47.5Co2.5Mn35In15 and Ni45Co5Mn37In13 alloys. The ground states (T=4.2 K and external field H=0) of the alloys was found to be characterized by three main line: two, partially overlapping, at higher frequencies (300-450 MHz), most likely corresponding of manganese resonance lines and one at lower frequency at about 200 MHz. A significant shift in the spectrum of Ni45Co5Mn37In13 by about 100 MHz to higher frequencies was observed. The correlation of magnetizations obtained from magnetic moment and NMR studies is discussed.

Authors:
 [1];  [1]; ORCiD logo [1];  [2];  [1];  [3];  [3]; ORCiD logo [4]; ORCiD logo [5];  [5];  [5]; ORCiD logo [6];  [2];  [1]
+ Show Author Affiliations
  1. Southern Illinois Univ., Carbondale, IL (United States). Physics Dept.
  2. Louisiana State Univ., Baton Rouge, LA (United States). Dept. of Physics and Astronomy
  3. Charles Univ., Prague (Czech Republic). Dept. of Low Temperature Physics
  4. Saint-Petersburg State Univ. (Russia)
  5. Lomonosov Moscow State Univ., Moscow (Russia)
  6. Lappeenranta University of Technology (Finland). Dept. of Physics
Publication Date:
Research Org.:
Southern Illinois Univ., Carbondale, IL (United States); Louisiana State Univ., Baton Rouge, LA (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES); Academy of Finland
OSTI Identifier:
1800357
Alternate Identifier(s):
OSTI ID: 1592194; OSTI ID: 1872894
Grant/Contract Number:  
FG02-06ER46291; SC0010521; FG02-13ER46946; 318405
Resource Type:
Accepted Manuscript
Journal Name:
AIP Advances
Additional Journal Information:
Journal Volume: 10; Journal Issue: 1; Conference: 64.Annual Conference on Magnetism and Magnetic Materials, Las Vegas, NV (United States), 4-8 Nov 2019; Journal ID: ISSN 2158-3226
Publisher:
American Institute of Physics (AIP)
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE; 71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS; X-ray diffraction; Ferromagnetism; Alloys; Phase transitions; Nuclear magnetic resonance spectroscopy; magnetocaloric effect; phase transitions

Citation Formats

Aryal, Anil, Dubenko, Igor, Pandey, Sudip, Chen, Jing-Han, Talapatra, Saikat, Chlan, Vojtech, Stepankova, Helena, Matveev, Vladimir, Blinov, Mikhail, Prudnikov, Valerii, Granovsky, Alexander, Lähderanta, Erkki, Stadler, Shane, and Ali, Naushad. NMR studies of the ground states of Ni50-xCoxMn35In15 (x=1, 2.5) and Ni45Co5Mn37In13 Heusler alloys. United States: N. p., 2020. Web. doi:10.1063/1.5129976.
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Aryal, Anil, Dubenko, Igor, Pandey, Sudip, Chen, Jing-Han, Talapatra, Saikat, Chlan, Vojtech, Stepankova, Helena, Matveev, Vladimir, Blinov, Mikhail, Prudnikov, Valerii, Granovsky, Alexander, Lähderanta, Erkki, Stadler, Shane, & Ali, Naushad. NMR studies of the ground states of Ni50-xCoxMn35In15 (x=1, 2.5) and Ni45Co5Mn37In13 Heusler alloys. United States. https://doi.org/10.1063/1.5129976
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Aryal, Anil, Dubenko, Igor, Pandey, Sudip, Chen, Jing-Han, Talapatra, Saikat, Chlan, Vojtech, Stepankova, Helena, Matveev, Vladimir, Blinov, Mikhail, Prudnikov, Valerii, Granovsky, Alexander, Lähderanta, Erkki, Stadler, Shane, and Ali, Naushad. Fri . "NMR studies of the ground states of Ni50-xCoxMn35In15 (x=1, 2.5) and Ni45Co5Mn37In13 Heusler alloys". United States. https://doi.org/10.1063/1.5129976. https://www.osti.gov/servlets/purl/1800357.
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@article{osti_1800357,
title = {NMR studies of the ground states of Ni50-xCoxMn35In15 (x=1, 2.5) and Ni45Co5Mn37In13 Heusler alloys},
author = {Aryal, Anil and Dubenko, Igor and Pandey, Sudip and Chen, Jing-Han and Talapatra, Saikat and Chlan, Vojtech and Stepankova, Helena and Matveev, Vladimir and Blinov, Mikhail and Prudnikov, Valerii and Granovsky, Alexander and Lähderanta, Erkki and Stadler, Shane and Ali, Naushad},
abstractNote = {Three temperature-induced phase transitions at T=T1, TM/TA, and TC, related to the ferromagnetic order of the martensitic phase (FMMP), martensitic (structural) transitions (MT), and the ferromagnetic order of the austenitic phase (FMAP), respectively, have been observed in the off-stoichiometric Heusler alloys, Ni50-xCoxMn35In15 (x=1, 2.5) and Ni45Co5Mn37In13. In this work, the phase transitions temperatures are found to be depended on alloy composition. A kinetic arrest of the AP was observed for Ni47.5Co2.5Mn35In15 in the magnetization measurements during field-cooling cycle (FCC) at 50 kOe. Depending upon the cooling protocols, ZFC and FCC (at H = 50 kOe), two different ground states of the alloys can be found in Ni47.5Co2.5Mn35In15 and Ni45Co5Mn37In13 alloys. The ground states (T=4.2 K and external field H=0) of the alloys was found to be characterized by three main line: two, partially overlapping, at higher frequencies (300-450 MHz), most likely corresponding of manganese resonance lines and one at lower frequency at about 200 MHz. A significant shift in the spectrum of Ni45Co5Mn37In13 by about 100 MHz to higher frequencies was observed. The correlation of magnetizations obtained from magnetic moment and NMR studies is discussed.},
doi = {10.1063/1.5129976},
journal = {AIP Advances},
number = 1,
volume = 10,
place = {United States},
year = {Fri Jan 17 00:00:00 EST 2020},
month = {Fri Jan 17 00:00:00 EST 2020}
}
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https://doi.org/10.1063/1.5129976
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Works referenced in this record:

Magnetocaloric effect and multifunctional properties of Ni–Mn-based Heusler alloys
journal, October 2012

  • Dubenko, Igor; Samanta, Tapas; Kumar Pathak, Arjun
  • Journal of Magnetism and Magnetic Materials, Vol. 324, Issue 21
  • DOI: 10.1016/j.jmmm.2012.02.082

Large magnetic entropy changes in the Ni45.4Mn41.5In13.1 ferromagnetic shape memory alloy
journal, October 2006

  • Han, Z. D.; Wang, D. H.; Zhang, C. L.
  • Applied Physics Letters, Vol. 89, Issue 18
  • DOI: 10.1063/1.2385147

Giant Hall effect in Ni-Mn-In Heusler alloys
journal, September 2009

Magnetocaloric effect and magnetic-field-induced shape recovery effect at room temperature in ferromagnetic Heusler alloy Ni–Mn–Sb
journal, August 2007

Large magnetoresistance in single-crystalline Ni50Mn50−xInx alloys (x=14–16) upon martensitic transformation
journal, October 2006

  • Yu, S. Y.; Liu, Z. H.; Liu, G. D.
  • Applied Physics Letters, Vol. 89, Issue 16
  • DOI: 10.1063/1.2362581

Kinetic arrest of martensitic transformation in the NiCoMnIn metamagnetic shape memory alloy
journal, January 2008

  • Ito, Wataru; Ito, Kouhei; Umetsu, Rie Y.
  • Applied Physics Letters, Vol. 92, Issue 2
  • DOI: 10.1063/1.2833699

Transition-metal-based magnetic refrigerants for room-temperature applications
journal, January 2002

  • Tegus, O.; Brück, E.; Buschow, K. H. J.
  • Nature, Vol. 415, Issue 6868
  • DOI: 10.1038/415150a

Magnetoresistance and field-induced structural transitions in Ni50Mn50−xSnx Heusler alloys
journal, February 2008

  • Khan, Mahmud; Pathak, Arjun K.; Paudel, Moti R.
  • Journal of Magnetism and Magnetic Materials, Vol. 320, Issue 3-4
  • DOI: 10.1016/j.jmmm.2007.06.016

Microwave absorption through the martensitic and Curie transitions in Ni 45 Cr 5 Mn 37 In 13
journal, May 2018

  • Pandey, Sudip; Vyzulin, Sergey; Quetz, Abdiel
  • AIP Advances, Vol. 8, Issue 5
  • DOI: 10.1063/1.5006440

Ferromagnetic resonance in Ni-Mn based ferromagnetic Heusler alloys
journal, January 2010

Exchange bias behavior in Ni–Mn–Sb Heusler alloys
journal, August 2007

  • Khan, Mahmud; Dubenko, Igor; Stadler, Shane
  • Applied Physics Letters, Vol. 91, Issue 7
  • DOI: 10.1063/1.2772233

Delocalization and hybridization enhance the magnetocaloric effect in Cu-doped Ni 2 MnGa
journal, June 2009

The giant magnetocaloric effect of optimally prepared Gd5Si2Ge2
journal, April 2003

  • Pecharsky, A. O.; Gschneidner, K. A.; Pecharsky, V. K.
  • Journal of Applied Physics, Vol. 93, Issue 8
  • DOI: 10.1063/1.1558210

Exchange bias in bulk Ni–Mn–In-based Heusler alloys
journal, April 2009

  • Pathak, Arjun Kumar; Khan, Mahmud; Gautam, Bhoj Raj
  • Journal of Magnetism and Magnetic Materials, Vol. 321, Issue 8
  • DOI: 10.1016/j.jmmm.2008.03.008

Magnetic, transport, and magnetocaloric properties of boron doped Ni-Mn-In alloys
journal, May 2015

  • Pandey, S.; Quetz, A.; Rodionov, I. D.
  • Journal of Applied Physics, Vol. 117, Issue 18
  • DOI: 10.1063/1.4921052
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