Critical review of FDM 3D printing of PLA biocomposites filled with biomass resources, characterization, biodegradability, upcycling and opportunities for biorefineries
Abstract
3D printing by fused deposition modeling (FDM) is an advanced additive manufacturing technology for making thermoplastic-based structures. Several studies have recently investigated 3D printing of polylactic acid (PLA) with biomass resources like cellulose, hemicellulose, lignin and whole biomass. Such biodegradable composites are better for the environment and can be used to replace non-biodegradable composites in a variety of applications. Therefore, a deep understanding of printing such biocomposites is needed for supporting such manufacturing. Recent developments focused on FDM printing of PLA filled with biomass resources have been critically reviewed to reveal the intricate aspects of manufacturing of such materials and characterization of the changes caused by biomass-based fillers. Properties of high molecular weight PLA, essentials of printing with PLA and conditions for filament extrusion and printing of biocomposites are discussed. Characterization results from mechanical testing, thermal analysis, viscoelastic properties, imaging and spectroscopy are reviewed for understanding the impact of filling biomass resources in PLA by printing. The latter sections discuss applications, upcycling & recycling and future opportunities for biorefineries.
- Authors:
- Publication Date:
- Research Org.:
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
- Sponsoring Org.:
- USDOE
- OSTI Identifier:
- 1787429
- Alternate Identifier(s):
- OSTI ID: 1805017
- Grant/Contract Number:
- AC05-00OR22725
- Resource Type:
- Published Article
- Journal Name:
- Applied Materials Today
- Additional Journal Information:
- Journal Name: Applied Materials Today Journal Volume: 24 Journal Issue: C; Journal ID: ISSN 2352-9407
- Publisher:
- Elsevier
- Country of Publication:
- Netherlands
- Language:
- English
- Subject:
- 09 BIOMASS FUELS; 3D printing; Additive manufacturing; Biomass; Cellulose; Lignin; PLA; Thermoplastics; Biodegradation; Recycling; upcycling
Citation Formats
Bhagia, Samarthya, Bornani, Kamlesh, Agrawal, Ruchi, Satlewal, Alok, Ďurkovič, Jaroslav, Lagaňa, Rastislav, Bhagia, Meher, Yoo, Chang Geun, Zhao, Xianhui, Kunc, Vlastimil, Pu, Yunqiao, Ozcan, Soydan, and Ragauskas, Arthur J. Critical review of FDM 3D printing of PLA biocomposites filled with biomass resources, characterization, biodegradability, upcycling and opportunities for biorefineries. Netherlands: N. p., 2021.
Web. doi:10.1016/j.apmt.2021.101078.
Bhagia, Samarthya, Bornani, Kamlesh, Agrawal, Ruchi, Satlewal, Alok, Ďurkovič, Jaroslav, Lagaňa, Rastislav, Bhagia, Meher, Yoo, Chang Geun, Zhao, Xianhui, Kunc, Vlastimil, Pu, Yunqiao, Ozcan, Soydan, & Ragauskas, Arthur J. Critical review of FDM 3D printing of PLA biocomposites filled with biomass resources, characterization, biodegradability, upcycling and opportunities for biorefineries. Netherlands. https://doi.org/10.1016/j.apmt.2021.101078
Bhagia, Samarthya, Bornani, Kamlesh, Agrawal, Ruchi, Satlewal, Alok, Ďurkovič, Jaroslav, Lagaňa, Rastislav, Bhagia, Meher, Yoo, Chang Geun, Zhao, Xianhui, Kunc, Vlastimil, Pu, Yunqiao, Ozcan, Soydan, and Ragauskas, Arthur J. Wed .
"Critical review of FDM 3D printing of PLA biocomposites filled with biomass resources, characterization, biodegradability, upcycling and opportunities for biorefineries". Netherlands. https://doi.org/10.1016/j.apmt.2021.101078.
@article{osti_1787429,
title = {Critical review of FDM 3D printing of PLA biocomposites filled with biomass resources, characterization, biodegradability, upcycling and opportunities for biorefineries},
author = {Bhagia, Samarthya and Bornani, Kamlesh and Agrawal, Ruchi and Satlewal, Alok and Ďurkovič, Jaroslav and Lagaňa, Rastislav and Bhagia, Meher and Yoo, Chang Geun and Zhao, Xianhui and Kunc, Vlastimil and Pu, Yunqiao and Ozcan, Soydan and Ragauskas, Arthur J.},
abstractNote = {3D printing by fused deposition modeling (FDM) is an advanced additive manufacturing technology for making thermoplastic-based structures. Several studies have recently investigated 3D printing of polylactic acid (PLA) with biomass resources like cellulose, hemicellulose, lignin and whole biomass. Such biodegradable composites are better for the environment and can be used to replace non-biodegradable composites in a variety of applications. Therefore, a deep understanding of printing such biocomposites is needed for supporting such manufacturing. Recent developments focused on FDM printing of PLA filled with biomass resources have been critically reviewed to reveal the intricate aspects of manufacturing of such materials and characterization of the changes caused by biomass-based fillers. Properties of high molecular weight PLA, essentials of printing with PLA and conditions for filament extrusion and printing of biocomposites are discussed. Characterization results from mechanical testing, thermal analysis, viscoelastic properties, imaging and spectroscopy are reviewed for understanding the impact of filling biomass resources in PLA by printing. The latter sections discuss applications, upcycling & recycling and future opportunities for biorefineries.},
doi = {10.1016/j.apmt.2021.101078},
journal = {Applied Materials Today},
number = C,
volume = 24,
place = {Netherlands},
year = {Wed Sep 01 00:00:00 EDT 2021},
month = {Wed Sep 01 00:00:00 EDT 2021}
}
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