Impact of Mineral Reactive Surface Area on Forecasting Geological Carbon Sequestration in a CO2-EOR Field
Abstract
Mineral reactive surface area (RSA) is one of the key factors that control mineral reactions, as it describes how much mineral is accessible and can participate in reactions. This work aims to evaluate the impact of mineral RSA on numerical simulations for CO2 storage at depleted oil fields. The Farnsworth Unit (FWU) in northern Texas was chosen as a case study. A simplified model was used to screen representative cases from 87 RSA combinations to reduce the computational cost. Three selected cases with low, mid, and high RSA values were used for the FWU model. Results suggest that the impact of RSA values on CO2 mineral trapping is more complex than it is on individual reactions. While the low RSA case predicted negligible porosity change and an insignificant amount of CO2 mineral trapping for the FWU model, the mid and high RSA cases forecasted up to 1.19% and 5.04% of porosity reduction due to mineral reactions, and 2.46% and 9.44% of total CO2 trapped in minerals by the end of the 600-year simulation, respectively. The presence of hydrocarbons affects geochemical reactions and can lead to net CO2 mineral trapping, whereas mineral dissolution is forecasted when hydrocarbons are removed from themore »
- Authors:
- Publication Date:
- Research Org.:
- New Mexico Institute of Mining and Technology, Socorro, NM (United States)
- Sponsoring Org.:
- USDOE Office of Fossil Energy (FE)
- OSTI Identifier:
- 1771240
- Alternate Identifier(s):
- OSTI ID: 1849092
- Grant/Contract Number:
- FC26-05NT42591
- Resource Type:
- Published Article
- Journal Name:
- Energies
- Additional Journal Information:
- Journal Name: Energies Journal Volume: 14 Journal Issue: 6; Journal ID: ISSN 1996-1073
- Publisher:
- MDPI AG
- Country of Publication:
- Switzerland
- Language:
- English
- Subject:
- 58 GEOSCIENCES; Energy & Fuels; geological carbon sequestration; reactive surface area; mineral trapping; enhanced oil recovery with CO2 (CO2-EOR); geochemical reactions; risk assessment
Citation Formats
Jia, Wei, Xiao, Ting, Wu, Zhidi, Dai, Zhenxue, and McPherson, Brian. Impact of Mineral Reactive Surface Area on Forecasting Geological Carbon Sequestration in a CO2-EOR Field. Switzerland: N. p., 2021.
Web. doi:10.3390/en14061608.
Jia, Wei, Xiao, Ting, Wu, Zhidi, Dai, Zhenxue, & McPherson, Brian. Impact of Mineral Reactive Surface Area on Forecasting Geological Carbon Sequestration in a CO2-EOR Field. Switzerland. https://doi.org/10.3390/en14061608
Jia, Wei, Xiao, Ting, Wu, Zhidi, Dai, Zhenxue, and McPherson, Brian. Sun .
"Impact of Mineral Reactive Surface Area on Forecasting Geological Carbon Sequestration in a CO2-EOR Field". Switzerland. https://doi.org/10.3390/en14061608.
@article{osti_1771240,
title = {Impact of Mineral Reactive Surface Area on Forecasting Geological Carbon Sequestration in a CO2-EOR Field},
author = {Jia, Wei and Xiao, Ting and Wu, Zhidi and Dai, Zhenxue and McPherson, Brian},
abstractNote = {Mineral reactive surface area (RSA) is one of the key factors that control mineral reactions, as it describes how much mineral is accessible and can participate in reactions. This work aims to evaluate the impact of mineral RSA on numerical simulations for CO2 storage at depleted oil fields. The Farnsworth Unit (FWU) in northern Texas was chosen as a case study. A simplified model was used to screen representative cases from 87 RSA combinations to reduce the computational cost. Three selected cases with low, mid, and high RSA values were used for the FWU model. Results suggest that the impact of RSA values on CO2 mineral trapping is more complex than it is on individual reactions. While the low RSA case predicted negligible porosity change and an insignificant amount of CO2 mineral trapping for the FWU model, the mid and high RSA cases forecasted up to 1.19% and 5.04% of porosity reduction due to mineral reactions, and 2.46% and 9.44% of total CO2 trapped in minerals by the end of the 600-year simulation, respectively. The presence of hydrocarbons affects geochemical reactions and can lead to net CO2 mineral trapping, whereas mineral dissolution is forecasted when hydrocarbons are removed from the system.},
doi = {10.3390/en14061608},
journal = {Energies},
number = 6,
volume = 14,
place = {Switzerland},
year = {Sun Mar 14 00:00:00 EST 2021},
month = {Sun Mar 14 00:00:00 EST 2021}
}
https://doi.org/10.3390/en14061608
Works referenced in this record:
The impact of mineral reactive surface area variation on simulated mineral reactions and reaction rates
journal, January 2021
- Qin, Fanqi; Beckingham, Lauren E.
- Applied Geochemistry, Vol. 124
Effect of reactive surface area of minerals on mineralization trapping of CO2 in saline aquifers
journal, August 2012
- Luo, Shu; Xu, Ruina; Jiang, Peixue
- Petroleum Science, Vol. 9, Issue 3
Forecasting evolution of formation water chemistry and long-term mineral alteration for GCS in a typical clastic reservoir of the Southwestern United States
journal, November 2016
- Pan, Feng; McPherson, Brian J.; Esser, Rich
- International Journal of Greenhouse Gas Control, Vol. 54
Probabilistic analysis of CO2 storage mechanisms in a CO2-EOR field using polynomial chaos expansion
journal, August 2016
- Jia, Wei; McPherson, Brian J.; Pan, Feng
- International Journal of Greenhouse Gas Control, Vol. 51
Assessment of CO2 trapping mechanisms in partially depleted oil-bearing sands
journal, October 2020
- Sun, Qian; Ampomah, William; Kutsienyo, Eusebius Junior
- Fuel, Vol. 278
Uncertainty quantification of CO2 storage using Bayesian model averaging and polynomial chaos expansion
journal, April 2018
- Jia, Wei; McPherson, Brian; Pan, Feng
- International Journal of Greenhouse Gas Control, Vol. 71
The Nanoscale Basis of CO 2 Trapping for Geologic Storage
journal, August 2015
- Bourg, Ian C.; Beckingham, Lauren E.; DePaolo, Donald J.
- Environmental Science & Technology, Vol. 49, Issue 17
Impact of Three-Phase Relative Permeability and Hysteresis Models on Forecasts of Storage Associated With CO 2 -EOR: GEOLOGICAL CO 2 SEQUESTRATION
journal, February 2018
- Jia, Wei; McPherson, Brian; Pan, Feng
- Water Resources Research, Vol. 54, Issue 2
Chemo‐mechanical Alterations Induced From CO 2 Injection in Carbonate‐Cemented Sandstone: An Experimental Study at 71 °C and 29 MPa
journal, March 2020
- Wu, Z.; Luhmann, A. J.; Rinehart, A. J.
- Journal of Geophysical Research: Solid Earth, Vol. 125, Issue 3
Overview of a Large Scale Carbon Capture, Utilization, and Storage Demonstration Project in an Active Oil Field in Texas, USA
journal, July 2017
- Balch, Robert; McPherson, Brian; Grigg, Reid
- Energy Procedia, Vol. 114
Evaluation of CO 2 Storage Mechanisms in CO 2 Enhanced Oil Recovery Sites: Application to Morrow Sandstone Reservoir
journal, September 2016
- Ampomah, William; Balch, Robert; Cather, Martha
- Energy & Fuels, Vol. 30, Issue 10
Probabilistic Risk Assessment of CO2 Trapping Mechanisms in a Sandstone CO2-EOR Field in Northern Texas, USA
journal, July 2017
- Jia, Wei; Pan, Feng; Dai, Zhenxue
- Energy Procedia, Vol. 114
Co-optimizing water-alternating-carbon dioxide injection projects using a machine learning assisted computational framework
journal, December 2020
- You, Junyu; Ampomah, William; Sun, Qian
- Applied Energy, Vol. 279
Chemical Impacts of Potential CO2 and Brine Leakage on Groundwater Quality with Quantitative Risk Assessment: A Case Study of the Farnsworth Unit
journal, December 2020
- Xiao, Ting; McPherson, Brian; Esser, Richard
- Energies, Vol. 13, Issue 24
Measurement of accessible reactive surface area in a sandstone, with application to CO2 mineralization
journal, July 2012
- Landrot, Gautier; Ajo-Franklin, Jonathan B.; Yang, Li
- Chemical Geology, Vol. 318-319
Thermo-hydro-mechanical-chemical couplings controlling CH4 production and CO2 sequestration in enhanced coalbed methane recovery
journal, April 2019
- Fan, Chaojun; Elsworth, Derek; Li, Sheng
- Energy, Vol. 173
Impacts of relative permeability formulation on forecasts of CO 2 phase behavior, phase distribution, and trapping mechanisms in a geologic carbon storage reservoir: Corrigendum
journal, October 2017
- Moodie, Nathan; Pan, Feng; Jia, Wei
- Greenhouse Gases: Science and Technology, Vol. 7, Issue 5
Effect of reactive surface area of minerals on mineralization and carbon dioxide trapping in a depleted gas reservoir
journal, February 2014
- Bolourinejad, Panteha; Shoeibi Omrani, Pejman; Herber, Rien
- International Journal of Greenhouse Gas Control, Vol. 21
Evaluation of Macroscopic Porosity-Permeability Relationships in Heterogeneous Mineral Dissolution and Precipitation Scenarios: EVALUATION OF PERMEABILITY RELATIONSHIPS
journal, December 2017
- Beckingham, Lauren E.
- Water Resources Research, Vol. 53, Issue 12
Assignment and calibration of relative permeability by hydrostratigraphic units for multiphase flow analysis, case study: CO2-EOR operations at the Farnsworth Unit, Texas
journal, February 2019
- Moodie, Nathan; Ampomah, William; Jia, Wei
- International Journal of Greenhouse Gas Control, Vol. 81
Reactive chemical transport simulations of geologic carbon sequestration: Methods and applications
journal, September 2020
- Dai, Zhenxue; Xu, Lulu; Xiao, Ting
- Earth-Science Reviews, Vol. 208
Evaluation of trapping mechanisms in geologic CO2 sequestration: Case study of SACROC northern platform, a 35-year CO2 injection site
journal, April 2010
- Han, W. S.; McPherson, B. J.; Lichtner, P. C.
- American Journal of Science, Vol. 310, Issue 4
Chemical‐Mechanical Impacts of CO 2 Intrusion Into Heterogeneous Caprock
journal, November 2020
- Xiao, Ting; Xu, Hao; Moodie, Nathan
- Water Resources Research, Vol. 56, Issue 11
Potential chemical impacts of CO2 leakage on underground source of drinking water assessed by quantitative risk analysis
journal, July 2016
- Xiao, Ting; McPherson, Brian; Pan, Feng
- International Journal of Greenhouse Gas Control, Vol. 50
Stabilization Wedges: Solving the Climate Problem for the Next 50 Years with Current Technologies
journal, August 2004
- Pacala, S.
- Science, Vol. 305, Issue 5686
Adsorption of Gases in Multimolecular Layers
journal, February 1938
- Brunauer, Stephen; Emmett, P. H.; Teller, Edward
- Journal of the American Chemical Society, Vol. 60, Issue 2, p. 309-319
Coupled Thermo-Hydro-Mechanical-Chemical Modeling of Permeability Evolution in a CO 2 -Circulated Geothermal Reservoir
journal, May 2019
- Tao, Jing; Wu, Yu; Elsworth, Derek
- Geofluids, Vol. 2019
CO2 Sequestration and Enhanced Oil Recovery at Depleted Oil/Gas Reservoirs
journal, July 2017
- Dai, Zhenxue; Viswanathan, Hari; Xiao, Ting
- Energy Procedia, Vol. 114
An Integrated Framework for Optimizing CO 2 Sequestration and Enhanced Oil Recovery
journal, November 2013
- Dai, Zhenxue; Middleton, Richard; Viswanathan, Hari
- Environmental Science & Technology Letters, Vol. 1, Issue 1
Uncertainty analysis of carbon sequestration in an active CO2-EOR field
journal, August 2016
- Pan, Feng; McPherson, Brian J.; Dai, Zhenxue
- International Journal of Greenhouse Gas Control, Vol. 51
Evaluation of mineral reactive surface area estimates for prediction of reactivity of a multi-mineral sediment
journal, September 2016
- Beckingham, Lauren E.; Mitnick, Elizabeth H.; Steefel, Carl I.
- Geochimica et Cosmochimica Acta, Vol. 188
Quantification of CO2-cement-rock interactions at the well-caprock-reservoir interface and implications for geological CO2 storage
journal, August 2017
- Xiao, Ting; McPherson, Brian; Bordelon, Amanda
- International Journal of Greenhouse Gas Control, Vol. 63
CO 2 Accounting and Risk Analysis for CO 2 Sequestration at Enhanced Oil Recovery Sites
journal, June 2016
- Dai, Zhenxue; Viswanathan, Hari; Middleton, Richard
- Environmental Science & Technology, Vol. 50, Issue 14
Co-optimization of CO 2 -EOR and storage processes in mature oil reservoirs : Original Research Article: Co-optimization of CO
journal, August 2016
- Ampomah, William; Balch, Robert S.; Grigg, Reid B.
- Greenhouse Gases: Science and Technology, Vol. 7, Issue 1
A pore-scale mathematical modeling of fluid-particle interactions: Thermo-hydro-mechanical coupling
journal, April 2019
- Tahmasebi, Pejman; Kamrava, Serveh
- International Journal of Greenhouse Gas Control, Vol. 83
A Guide to CO2 Sequestration
journal, June 2003
- Lackner, K. S.
- Science, Vol. 300, Issue 5626, p. 1677-1678