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Title: General Techno-Economic Analysis of CO2 Electrolysis Systems

Abstract

The electrochemical reduction of carbon dioxide (CO2) has received significant attention in academic research, although the techno-economic prospects of the technology for the large-scale production of chemicals are unclear. In this work, we briefly reviewed the current state-of-the-art CO2 reduction figures of merit, and performed an economic analysis of a generalized CO2 electrolyzer system for the production of 100 tons/day of various CO2 reduction products. While carbon monoxide and formic acid were the most economically favorable products under current conditions, higher-order alcohols such as ethanol and n-propanol could be highly promising if reasonable electrocatalytic performance benchmarks were achieved. Furthermore, we established performance targets such that if these targets are achieved, electrochemical CO2 reduction for fuels and chemicals production can become a profitable option as part of the growing renewable energy infrastructure.

Authors:
ORCiD logo [1]; ORCiD logo [1]; ORCiD logo [1]
+ Show Author Affiliations
  1. Univ. of Delaware, Newark, DE (United States)
Publication Date:
Research Org.:
Univ. of Delaware, Newark, DE (United States)
Sponsoring Org.:
USDOE Office of Fossil Energy (FE)
OSTI Identifier:
1712664
Grant/Contract Number:  
FE0029868
Resource Type:
Accepted Manuscript
Journal Name:
Industrial and Engineering Chemistry Research
Additional Journal Information:
Journal Volume: 57; Journal Issue: 6; Journal ID: ISSN 0888-5885
Publisher:
American Chemical Society (ACS)
Country of Publication:
United States
Language:
English
Subject:
37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY; carbon dioxide; electrocatalysts; electrochemical reduction; organic acids; oxides; inorganic carbon compounds

Citation Formats

Jouny, Matthew, Luc, Wesley, and Jiao, Feng. General Techno-Economic Analysis of CO2 Electrolysis Systems. United States: N. p., 2018. Web. doi:10.1021/acs.iecr.7b03514.
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Jouny, Matthew, Luc, Wesley, & Jiao, Feng. General Techno-Economic Analysis of CO2 Electrolysis Systems. United States. https://doi.org/10.1021/acs.iecr.7b03514
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Jouny, Matthew, Luc, Wesley, and Jiao, Feng. Fri . "General Techno-Economic Analysis of CO2 Electrolysis Systems". United States. https://doi.org/10.1021/acs.iecr.7b03514. https://www.osti.gov/servlets/purl/1712664.
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@article{osti_1712664,
title = {General Techno-Economic Analysis of CO2 Electrolysis Systems},
author = {Jouny, Matthew and Luc, Wesley and Jiao, Feng},
abstractNote = {The electrochemical reduction of carbon dioxide (CO2) has received significant attention in academic research, although the techno-economic prospects of the technology for the large-scale production of chemicals are unclear. In this work, we briefly reviewed the current state-of-the-art CO2 reduction figures of merit, and performed an economic analysis of a generalized CO2 electrolyzer system for the production of 100 tons/day of various CO2 reduction products. While carbon monoxide and formic acid were the most economically favorable products under current conditions, higher-order alcohols such as ethanol and n-propanol could be highly promising if reasonable electrocatalytic performance benchmarks were achieved. Furthermore, we established performance targets such that if these targets are achieved, electrochemical CO2 reduction for fuels and chemicals production can become a profitable option as part of the growing renewable energy infrastructure.},
doi = {10.1021/acs.iecr.7b03514},
journal = {Industrial and Engineering Chemistry Research},
number = 6,
volume = 57,
place = {United States},
year = {Fri Jan 19 00:00:00 EST 2018},
month = {Fri Jan 19 00:00:00 EST 2018}
}
Copy to clipboard
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    journal, February 2020

    • Kim, Seohyoung; Lindner, Steffen N.; Aslan, Selçuk
    • Nature Chemical Biology, Vol. 16, Issue 5
    • DOI: 10.1038/s41589-020-0473-5

    CO 2 reduction on gas-diffusion electrodes and why catalytic performance must be assessed at commercially-relevant conditions
    journal, January 2019

    • Burdyny, Thomas; Smith, Wilson A.
    • Energy & Environmental Science, Vol. 12, Issue 5
    • DOI: 10.1039/c8ee03134g

    Electrochemical CO 2 Reduction into Chemical Feedstocks: From Mechanistic Electrocatalysis Models to System Design
    journal, December 2018

    • Kibria, Md Golam; Edwards, Jonathan P.; Gabardo, Christine M.
    • Advanced Materials, Vol. 31, Issue 31
    • DOI: 10.1002/adma.201807166

    Understanding the Origin of Highly Selective CO 2 Electroreduction to CO on Ni,N‐doped Carbon Catalysts
    journal, January 2020

    • Koshy, David M.; Chen, Shucheng; Lee, Dong Un
    • Angewandte Chemie, Vol. 132, Issue 10
    • DOI: 10.1002/ange.201912857

    Electroreduction of carbon dioxide to formate at high current densities using tin and tin oxide gas diffusion electrodes
    journal, July 2019

    • Sen, Sujat; Brown, Steven M.; Leonard, McLain
    • Journal of Applied Electrochemistry, Vol. 49, Issue 9
    • DOI: 10.1007/s10800-019-01332-z

    Emerging Carbon‐Based Heterogeneous Catalysts for Electrochemical Reduction of Carbon Dioxide into Value‐Added Chemicals
    journal, December 2018

    Two-dimensional copper nanosheets for electrochemical reduction of carbon monoxide to acetate
    journal, April 2019

    Selective reduction of CO to acetaldehyde with CuAg electrocatalysts
    journal, January 2020

    • Wang, Lei; Higgins, Drew C.; Ji, Yongfei
    • Proceedings of the National Academy of Sciences, Vol. 117, Issue 23
    • DOI: 10.1073/pnas.1821683117

    General technoeconomic analysis for electrochemical coproduction coupling carbon dioxide reduction with organic oxidation
    journal, November 2019

    Linkage Effect in the Heterogenization of Cobalt Complexes by Doped Graphene for Electrocatalytic CO 2 Reduction
    journal, September 2019

    • Wang, Jiong; Huang, Xiang; Xi, Shibo
    • Angewandte Chemie International Edition, Vol. 58, Issue 38
    • DOI: 10.1002/anie.201906475

    Cyclic two-step electrolysis for stable electrochemical conversion of carbon dioxide to formate
    journal, September 2019

    Electrocatalytic Reduction of Gaseous CO 2 to CO on Sn/Cu‐Nanofiber‐Based Gas Diffusion Electrodes
    journal, July 2019

    A Highly Porous Copper Electrocatalyst for Carbon Dioxide Reduction
    journal, October 2018

    • Lv, Jing-Jing; Jouny, Matthew; Luc, Wesley
    • Advanced Materials, Vol. 30, Issue 49
    • DOI: 10.1002/adma.201803111

    Surface reconstruction of AgPd nanoalloy particles during the electrocatalytic formate oxidation reaction
    journal, January 2020

    Alloy Nanocatalysts for the Electrochemical Oxygen Reduction (ORR) and the Direct Electrochemical Carbon Dioxide Reduction Reaction (CO 2 RR)
    journal, December 2018

    • Kim, Cheonghee; Dionigi, Fabio; Beermann, Vera
    • Advanced Materials, Vol. 31, Issue 31
    • DOI: 10.1002/adma.201805617

    The p‐Orbital Delocalization of Main‐Group Metals to Boost CO 2 Electroreduction
    journal, October 2018

    Cooperative CO2-to-ethanol conversion via enriched intermediates at molecule–metal catalyst interfaces
    journal, December 2019

    Constraining CO coverage on copper promotes high-efficiency ethylene electroproduction
    journal, November 2019

    Formic acid, a biomass-derived source of energy and hydrogen for biomass upgrading
    journal, January 2019

    • Valentini, Federica; Kozell, Vadym; Petrucci, Chiara
    • Energy & Environmental Science, Vol. 12, Issue 9
    • DOI: 10.1039/c9ee01747j

    Promises of Main Group Metal–Based Nanostructured Materials for Electrochemical CO 2 Reduction to Formate
    journal, November 2019

    Understanding the Origin of Highly Selective CO 2 Electroreduction to CO on Ni,N‐doped Carbon Catalysts
    journal, January 2020

    • Koshy, David M.; Chen, Shucheng; Lee, Dong Un
    • Angewandte Chemie International Edition, Vol. 59, Issue 10
    • DOI: 10.1002/anie.201912857

    High Pressure Electrochemical Reduction of CO 2 to Formic Acid/Formate: A Comparison between Bipolar Membranes and Cation Exchange Membranes
    journal, January 2019

    • Ramdin, Mahinder; Morrison, Andrew R. T.; de Groen, Mariette
    • Industrial & Engineering Chemistry Research, Vol. 58, Issue 5
    • DOI: 10.1021/acs.iecr.8b04944

    Multilayer Electrolyzer Stack Converts Carbon Dioxide to Gas Products at High Pressure with High Efficiency
    journal, June 2019

    Cyclic two-step electrolysis for stable electrochemical conversion of carbon dioxide to formate
    journal, September 2019

    General technoeconomic analysis for electrochemical coproduction coupling carbon dioxide reduction with organic oxidation
    journal, November 2019

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