The speciation, transformation kinetics and fate of spiked Pu (IV) in highly saline groundwater

Zhou, Xu; Dang, Haijun; Han, Xiaoyuan; Li, Weiping; Wang, Yu; Wang, Weixian; Chai, Nana

doi:10.1016/j.jconhyd.2019.103505

Title: The speciation, transformation kinetics and fate of spiked Pu (IV) in highly saline groundwater

Full Record
Other Related Research

Authors:: Zhou, Xu; Dang, Haijun; Han, Xiaoyuan; Li, Weiping; Wang, Yu; Wang, Weixian; Chai, Nana

Publication Date:: Thu Aug 01 00:00:00 EDT 2019

Sponsoring Org.:: USDOE Office of Electricity (OE), Advanced Grid Research & Development. Power Systems Engineering Research

OSTI Identifier:: 1702168

Grant/Contract Number:: 2012AA021705

Resource Type:: Publisher's Accepted Manuscript

Journal Name:: Journal of Contaminant Hydrology

Additional Journal Information:: Journal Name: Journal of Contaminant Hydrology Journal Volume: 225 Journal Issue: C; Journal ID: ISSN 0169-7722

Publisher:: Elsevier

Country of Publication:: Netherlands

Language:: English

Citation Formats


                    Zhou, Xu, Dang, Haijun, Han, Xiaoyuan, Li, Weiping, Wang, Yu, Wang, Weixian, and Chai, Nana. The speciation, transformation kinetics and fate of spiked Pu (IV) in highly saline groundwater.  Netherlands: N. p., 2019. 
Web.  doi:10.1016/j.jconhyd.2019.103505.

Copy to clipboard


                    Zhou, Xu, Dang, Haijun, Han, Xiaoyuan, Li, Weiping, Wang, Yu, Wang, Weixian, & Chai, Nana. The speciation, transformation kinetics and fate of spiked Pu (IV) in highly saline groundwater.  Netherlands.  https://doi.org/10.1016/j.jconhyd.2019.103505

Copy to clipboard


                    Zhou, Xu, Dang, Haijun, Han, Xiaoyuan, Li, Weiping, Wang, Yu, Wang, Weixian, and Chai, Nana. Thu .  
"The speciation, transformation kinetics and fate of spiked Pu (IV) in highly saline groundwater".  Netherlands.  https://doi.org/10.1016/j.jconhyd.2019.103505.

Copy to clipboard


                    
@article{osti_1702168,

  title        = {The speciation, transformation kinetics and fate of spiked Pu (IV) in highly saline groundwater},

  author       = {Zhou, Xu and Dang, Haijun and Han, Xiaoyuan and Li, Weiping and Wang, Yu and Wang, Weixian and Chai, Nana},

  abstractNote = {},

  doi          = {10.1016/j.jconhyd.2019.103505},

  journal      = {Journal of Contaminant Hydrology},

  number       = C,

  volume       = 225,

  place        = {Netherlands},

  year         = {Thu Aug 01 00:00:00 EDT 2019},

  month        = {Thu Aug 01 00:00:00 EDT 2019}

}

Copy to clipboard

Journal Article:

Free Publicly Available Full Text

Accepted Manuscript (Publisher)

Publisher's Version of Record
https://doi.org/10.1016/j.jconhyd.2019.103505

Other availability

Search WorldCat to find libraries that may hold this journal

Save / Share:

Export Metadata

Save to My Library

Similar Records in DOE PAGES and OSTI.GOV collections:

Spring flood induced shifts in Fe speciation and fate at increased salinity

Journal Article Herzog, S. D. ; Conrad, S. ; Ingri, J. ; ... - Applied Geochemistry
Cited by 9
https://doi.org/10.1016/j.apgeochem.2019.104385
Speciation and structural characterization of Plutonium and Actinide-organic complexes in surface and ground waters (Sept. 1996-Sept. 1999) & Speciation, Mobility and Fate of Actinides in the Groundwater at the Hanford Site (Sept. 1999-Sept. 2002)

Technical Report Buesseler, K O ; Dai, M ; Repeta, D J

Our first project focused on the development and testing of appropriate sampling and analytical techniques to study the association of actinides with dissolved organic complexes in subsurface waters. Our ongoing project is designed for: (1) the determination of the speciation of plutonium and other actinides (Np, U) in groundwater at the 100 and 200 areas at the Hanford Site. This includes the separation of Pu into particulate, colloidal and <1 kilo- Dalton dissolved phases and the determination of redox states and isotopic composition in each fraction; (2) the characterization of groundwater colloids, which includes submicron-sized inorganic particles and organic macromoleculesmore »« less
https://doi.org/10.2172/827049

Full Text Available
Speciation, Mobility and Fate of Actinides in the Groundwater at the Hanford Site (Sept. 1999-Sept. 2002)

Technical Report Buesseler, K O ; Dai, M ; Repeta, D J

The objectives of this project are: (1) the determination of the speciation of plutonium and other actinides (Np, U) in groundwater at the 100 and 200 areas at the Hanford Site. This includes the separation of Pu into particulate, colloidal and <1 kilo-Dalton dissolved phases and the determination of redox states and isotopic composition in each fraction; (2) the characterization of groundwater colloids, which includes submicron-sized inorganic particles and organic macromolecules (3) the prediction of the rate of transport and fate of actinides in the groundwater of the Hanford Site using a three-phase (dissolved-colloid-particulate) model.
https://doi.org/10.2172/833615

Full Text Available
Effect of fluoride in NTS groundwaters on the aqueous speciation of U, Np, Pu, Am and Eu

Technical Report Bruton, C J ; Nimz, G J

To address SNJV concerns that fluoride in Nevada Test site (NTS) groundwaters may impact radionuclide speciation and transport, NTS water quality databases were obtained and scanned for analyses with high fluoride concentrations (> 10 mg/L). The aqueous speciation of nine representative samples of these groundwaters with added trace amounts of uranium (U), neptunium (Np), plutonium (Pu), americium (Am) and europium (Eu) was then calculated with the computer code EQ3NR assuming a temperature of 25 C, using currently available thermodynamic data for these species. Under conditions where U(VI), Np(V), Pu(IV), Am(III) and Eu(III) dominate, F complexes are insignificant (<1 mole %)more »« less
https://doi.org/10.2172/15015136

Full Text Available
Isotopic Composition, Speciation and Mobility of Pu in the Groundwater at DOE Savannah River Site

Conference Dai, M ; Kelley, J M ; Buesseler, K O ; ...

No abstract prepared.

Similar Records