Mesoscopic analyses of the impact of morphology and operating conditions on the transport resistances in a proton-exchange-membrane fuel-cell catalyst layer
Abstract
Exploring the origins of local transport resistance and characterizing the oxygen transport resistances in the catalyst layer ( R CL ) are critical for cost reduction.
- Authors:
-
[2];
[2];
- School of Human Settlements and Civil Engineering, Xi'an Jiaotong University, Xi'an, China
- Energy Conversion Group, Energy Technologies Area, Lawrence Berkeley National Laboratory, Berkeley, USA
- Key Laboratory of Thermo-Fluid Science and Engineering of MOE, School of Energy and Power Engineering, Xi'an Jiaotong University, Xi'an, China
- Publication Date:
- Sponsoring Org.:
- USDOE
- OSTI Identifier:
- 1630166
- Grant/Contract Number:
- AC02-05CH11231
- Resource Type:
- Publisher's Accepted Manuscript
- Journal Name:
- Sustainable Energy & Fuels
- Additional Journal Information:
- Journal Name: Sustainable Energy & Fuels Journal Volume: 4 Journal Issue: 7; Journal ID: ISSN 2398-4902
- Publisher:
- Royal Society of Chemistry (RSC)
- Country of Publication:
- United Kingdom
- Language:
- English
Citation Formats
Mu, Yu-Tong, Weber, Adam Z., Gu, Zhao-Lin, Schuler, Tobias, and Tao, Wen-Quan. Mesoscopic analyses of the impact of morphology and operating conditions on the transport resistances in a proton-exchange-membrane fuel-cell catalyst layer. United Kingdom: N. p., 2020.
Web. doi:10.1039/D0SE00560F.
Mu, Yu-Tong, Weber, Adam Z., Gu, Zhao-Lin, Schuler, Tobias, & Tao, Wen-Quan. Mesoscopic analyses of the impact of morphology and operating conditions on the transport resistances in a proton-exchange-membrane fuel-cell catalyst layer. United Kingdom. https://doi.org/10.1039/D0SE00560F
Mu, Yu-Tong, Weber, Adam Z., Gu, Zhao-Lin, Schuler, Tobias, and Tao, Wen-Quan. Tue .
"Mesoscopic analyses of the impact of morphology and operating conditions on the transport resistances in a proton-exchange-membrane fuel-cell catalyst layer". United Kingdom. https://doi.org/10.1039/D0SE00560F.
@article{osti_1630166,
title = {Mesoscopic analyses of the impact of morphology and operating conditions on the transport resistances in a proton-exchange-membrane fuel-cell catalyst layer},
author = {Mu, Yu-Tong and Weber, Adam Z. and Gu, Zhao-Lin and Schuler, Tobias and Tao, Wen-Quan},
abstractNote = {Exploring the origins of local transport resistance and characterizing the oxygen transport resistances in the catalyst layer ( R CL ) are critical for cost reduction.},
doi = {10.1039/D0SE00560F},
journal = {Sustainable Energy & Fuels},
number = 7,
volume = 4,
place = {United Kingdom},
year = {Tue Jun 30 00:00:00 EDT 2020},
month = {Tue Jun 30 00:00:00 EDT 2020}
}
Free Publicly Available Full Text
Publisher's Version of Record
https://doi.org/10.1039/D0SE00560F
https://doi.org/10.1039/D0SE00560F
Other availability
Search WorldCat to find libraries that may hold this journal
Cited by: 8 works
Citation information provided by
Web of Science
Web of Science
Save to My Library
You must Sign In or Create an Account in order to save documents to your library.
Works referenced in this record:
Modeling of local gas transport in catalyst layers of PEM fuel cells
journal, April 2017
- Mashio, Tetsuya; Iden, Hiroshi; Ohma, Atsushi
- Journal of Electroanalytical Chemistry, Vol. 790
The Priority and Challenge of High-Power Performance of Low-Platinum Proton-Exchange Membrane Fuel Cells
journal, March 2016
- Kongkanand, Anusorn; Mathias, Mark F.
- The Journal of Physical Chemistry Letters, Vol. 7, Issue 7
Toward sustainable fuel cells
journal, December 2016
- Stephens, Ifan Erfyl Lester; Rossmeisl, Jan; Chorkendorff, Ib
- Science, Vol. 354, Issue 6318
Understanding the Effect of Kinetic and Mass Transport Processes in Cathode Agglomerates
journal, January 2014
- Moore, M.; Wardlaw, P.; Dobson, P.
- Journal of The Electrochemical Society, Vol. 161, Issue 8
Impact of liquid water on oxygen reaction in cathode catalyst layer of proton exchange membrane fuel cell: A simple and physically sound model
journal, June 2016
- Zhang, Xiaoxian; Gao, Yuan
- Journal of Power Sources, Vol. 318
Analysis of Oxygen-Transport Diffusion Resistance in Proton-Exchange-Membrane Fuel Cells
journal, January 2011
- Nonoyama, Nobuaki; Okazaki, Shinobu; Weber, Adam Z.
- Journal of The Electrochemical Society, Vol. 158, Issue 4
Mesoscopic modeling of transport resistances in a polymer-electrolyte fuel-cell catalyst layer: Analysis of hydrogen limiting currents
journal, December 2019
- Mu, Yu-Tong; Weber, Adam Z.; Gu, Zhao-Lin
- Applied Energy, Vol. 255
Lattice Boltzmann method for conjugated heat and mass transfer with general interfacial conditions
journal, October 2018
- Mu, Yu-Tong; Gu, Zhao-Lin; He, Pu
- Physical Review E, Vol. 98, Issue 4
Mathematical Modelling and Experimental Analysis of Thin, Low-Loading Fuel Cell Electrodes
journal, September 2015
- Secanell, M.; Putz, A.; Shukla, S.
- ECS Transactions, Vol. 69, Issue 17
Computational prediction of nanoscale transport characteristics and catalyst utilization in fuel cell catalyst layers by the lattice Boltzmann method
journal, June 2018
- Shin, Seungho; Kim, Ah-Reum; Um, Sukkee
- Electrochimica Acta, Vol. 275
A Critical Review of Modeling Transport Phenomena in Polymer-Electrolyte Fuel Cells
journal, January 2014
- Weber, Adam Z.; Borup, Rodney L.; Darling, Robert M.
- Journal of The Electrochemical Society, Vol. 161, Issue 12
Microstructural Analysis and Transport Resistances of Low-Platinum-Loaded PEFC Electrodes
journal, January 2017
- Cetinbas, Firat C.; Wang, Xiaohua; Ahluwalia, Rajesh K.
- Journal of The Electrochemical Society, Vol. 164, Issue 14
Simulation of the catalyst layer in PEMFC based on a novel two-phase lattice model
journal, August 2011
- Zhang, Jiejing; Yang, Wei; Xu, Li
- Electrochimica Acta, Vol. 56, Issue 20
Simulated Volcano Plot of Oxygen Reduction Reaction on Stepped Pt Surfaces
journal, March 2017
- Jinnouchi, Ryosuke; Kodama, Kensaku; Nagoya, Akihiro
- Electrochimica Acta, Vol. 230
Modeling of Oxygen Diffusion Resistance in Polymer Electrolyte Fuel Cells in the Intermediate Potential Region
journal, January 2018
- Suzuki, Takahisa; Yamada, Haruhiko; Tsusaka, Kyoko
- Journal of The Electrochemical Society, Vol. 165, Issue 3
A comprehensive review of Pt electrocatalysts for the oxygen reduction reaction: Nanostructure, activity, mechanism and carbon support in PEM fuel cells
journal, January 2017
- Sui, Sheng; Wang, Xiaoying; Zhou, Xintong
- Journal of Materials Chemistry A, Vol. 5, Issue 5
Pore Scale Simulation of Transport and Electrochemical Reactions in Reconstructed PEMFC Catalyst Layers
journal, January 2010
- Lange, Kyle J.; Sui, Pang-Chieh; Djilali, Ned
- Journal of The Electrochemical Society, Vol. 157, Issue 10
Ultrafine jagged platinum nanowires enable ultrahigh mass activity for the oxygen reduction reaction
journal, November 2016
- Li, Mufan; Zhao, Zipeng; Cheng, Tao
- Science, Vol. 354, Issue 6318
A Comparison of Models for Transport Resistance in Fuel-Cell Catalyst Layers
journal, January 2018
- Darling, Robert
- Journal of The Electrochemical Society, Vol. 165, Issue 16
Numerical Study of the Gas Purging Process of a Proton Exchange Membrane Fuel Cell
journal, May 2017
- Mu, Yu-Tong; He, Pu; Ding, Jing
- Energy Procedia, Vol. 105
Dictating Pt-Based Electrocatalyst Performance in Polymer Electrolyte Fuel Cells, from Formulation to Application
journal, November 2019
- Van Cleve, Tim; Khandavalli, Sunilkumar; Chowdhury, Anamika
- ACS Applied Materials & Interfaces, Vol. 11, Issue 50
Unexplained transport resistances for low-loaded fuel-cell catalyst layers
journal, January 2014
- Weber, Adam Z.; Kusoglu, Ahmet
- J. Mater. Chem. A, Vol. 2, Issue 41
Transport Resistances in Fuel-Cell Catalyst Layers
journal, August 2017
- Chowdhury, Anamika; Radke, Clayton J.; Weber, Adam Z.
- ECS Transactions, Vol. 80, Issue 8
Gas Transport Resistance in Polymer Electrolyte Thin Films on Oxygen Reduction Reaction Catalysts
journal, August 2015
- Liu, Hang; Epting, William K.; Litster, Shawn
- Langmuir, Vol. 31, Issue 36
Relationship between gas transport resistance in the catalyst layer and effective surface area of the catalyst
journal, April 2013
- Iden, Hiroshi; Takaichi, Satoshi; Furuya, Yoshihisa
- Journal of Electroanalytical Chemistry, Vol. 694
Pore-scale investigation of catalyst layer ingredient and structure effect in proton exchange membrane fuel cell
journal, November 2019
- Hou, Yuze; Deng, Hao; Pan, Fengwen
- Applied Energy, Vol. 253
Hybrid approach combining multiple characterization techniques and simulations for microstructural analysis of proton exchange membrane fuel cell electrodes
journal, March 2017
- Cetinbas, Firat C.; Ahluwalia, Rajesh K.; Kariuki, Nancy
- Journal of Power Sources, Vol. 344
Diffusion of Water in Nafion 115 Membranes
journal, January 2000
- Motupally, Sathya; Becker, Aaron J.; Weidner, John W.
- Journal of The Electrochemical Society, Vol. 147, Issue 9
Enhanced electrocatalytic activity of platinum supported on nitrogen modified ordered mesoporous carbon
journal, November 2011
- Guo, YunXia; He, JianPing; Wang, Tao
- Journal of Power Sources, Vol. 196, Issue 22
Three-dimensional multi-phase model of PEM fuel cell coupled with improved agglomerate sub-model of catalyst layer
journal, November 2019
- Xie, Biao; Zhang, Guobin; Xuan, Jin
- Energy Conversion and Management, Vol. 199
Confinement-Driven Increase in Ionomer Thin-Film Modulus
journal, April 2014
- Page, Kirt A.; Kusoglu, Ahmet; Stafford, Christopher M.
- Nano Letters, Vol. 14, Issue 5
Modeling and Experimental Validation of Pt Loading and Electrode Composition Effects in PEM Fuel Cells
journal, January 2015
- Hao, Liang; Moriyama, Koji; Gu, Wenbin
- Journal of The Electrochemical Society, Vol. 162, Issue 8
New Insights into Perfluorinated Sulfonic-Acid Ionomers
journal, January 2017
- Kusoglu, Ahmet; Weber, Adam Z.
- Chemical Reviews, Vol. 117, Issue 3
Analysis of the role of the microporous layer in improving polymer electrolyte fuel cell performance
journal, April 2018
- Zhou, J.; Shukla, S.; Putz, A.
- Electrochimica Acta, Vol. 268
Toyota MIRAI Fuel Cell Vehicle and Progress Toward a Future Hydrogen Society
journal, January 2015
- Yoshida, T.; Kojima, K.
- Interface magazine, Vol. 24, Issue 2
Impact of Platinum Loading and Catalyst Layer Structure on PEMFC Performance
journal, January 2013
- Owejan, Jon P.; Owejan, Jeanette E.; Gu, Wenbin
- Journal of The Electrochemical Society, Vol. 160, Issue 8
Effects of Porosity and Water Saturation on the Effective Diffusivity of a Cathode Catalyst Layer
journal, January 2017
- Fathi, H.; Raoof, A.; Mansouri, S. H.
- Journal of The Electrochemical Society, Vol. 164, Issue 4
Biaxially strained PtPb/Pt core/shell nanoplate boosts oxygen reduction catalysis
journal, December 2016
- Bu, Lingzheng; Zhang, Nan; Guo, Shaojun
- Science, Vol. 354, Issue 6318
Analysis of Reactant Gas Transport in a Catalyst Layer
conference, January 2007
- Mashio, Tetsuya; Ohma, Atsushi; Yamamoto, Shinji
- 212th ECS Meeting, ECS Transactions
The Impact of Platinum Loading on Oxygen Transport Resistance
journal, January 2012
- Greszler, Thomas A.; Caulk, David; Sinha, Puneet
- Journal of The Electrochemical Society, Vol. 159, Issue 12
Current Status and Future Development of Catalyst Materials and Catalyst Layers for Proton Exchange Membrane Fuel Cells: An Industrial Perspective
journal, February 2017
- Banham, Dustin; Ye, Siyu
- ACS Energy Letters, Vol. 2, Issue 3
Analysis of Inkjet Printed PEFC Electrodes with Varying Platinum Loading
journal, January 2016
- Shukla, S.; Stanier, D.; Saha, M. S.
- Journal of The Electrochemical Society, Vol. 163, Issue 7
Modeling Low-Platinum-Loading Effects in Fuel-Cell Catalyst Layers
journal, January 2011
- Yoon, Wonseok; Weber, Adam Z.
- Journal of The Electrochemical Society, Vol. 158, Issue 8
Computational Analysis of Gas Transport in Fuel Cell Catalyst Layer under Dry and Partially Saturated Conditions
journal, January 2019
- Sabharwal, Mayank; Pant, Lalit M.; Patel, Nilay
- Journal of The Electrochemical Society, Vol. 166, Issue 7
Understanding Impacts of Catalyst-Layer Thickness on Fuel-Cell Performance via Mathematical Modeling
journal, January 2016
- Zenyuk, Iryna V.; Das, Prodip K.; Weber, Adam Z.
- Journal of The Electrochemical Society, Vol. 163, Issue 7
Analysis of Catalyst Layer Microstructures: From Imaging to Performance
journal, July 2016
- Sabharwal, M.; Pant, L. M.; Putz, A.
- Fuel Cells, Vol. 16, Issue 6
Progress in modified carbon support materials for Pt and Pt-alloy cathode catalysts in polymer electrolyte membrane fuel cells
journal, September 2016
- Wang, Yan-Jie; Fang, Baizeng; Li, Hui
- Progress in Materials Science, Vol. 82
The Effects of Catalyst Layer Microstructure and Water Saturation on the Effective Diffusivity in PEMFC
journal, January 2018
- Zheng, Weibo; Kim, Seung Hyun
- Journal of The Electrochemical Society, Vol. 165, Issue 7
Mass-transport properties of electrosprayed Pt/C catalyst layers for polymer-electrolyte fuel cells
journal, July 2019
- Conde, Julio J.; Folgado, M. Antonia; Ferreira-Aparicio, P.
- Journal of Power Sources, Vol. 427
Fuel-Cell Catalyst-Layer Resistance via Hydrogen Limiting-Current Measurements
journal, January 2019
- Schuler, Tobias; Chowdhury, Anamika; Freiberg, Anna T.
- Journal of The Electrochemical Society, Vol. 166, Issue 7
Measurements of Pore Size Distribution, Porosity, Effective Oxygen Diffusivity, and Tortuosity of PEM Fuel Cell Electrodes
journal, June 2012
- Yu, Z.; Carter, R. N.; Zhang, J.
- Fuel Cells, Vol. 12, Issue 4
Model for investigation of oxygen transport limitation in a polymer electrolyte fuel cell
journal, January 2013
- Suzuki, Takahisa; Kudo, Kenji; Morimoto, Yu
- Journal of Power Sources, Vol. 222
Direct numerical simulation (DNS) modeling of PEFC electrodes
journal, April 2006
- Wang, Guoqing; Mukherjee, Partha P.; Wang, Chao-Yang
- Electrochimica Acta, Vol. 51, Issue 15
Tipping water balance and the Pt loading effect in polymer electrolyte fuel cells: a model-based analysis
journal, January 2018
- Muzaffar, Tasleem; Kadyk, Thomas; Eikerling, Michael
- Sustainable Energy & Fuels, Vol. 2, Issue 6
Experimental dissection of oxygen transport resistance in the components of a polymer electrolyte membrane fuel cell
journal, March 2017
- Oh, Hwanyeong; Lee, Yoo il; Lee, Guesang
- Journal of Power Sources, Vol. 345
Nanostructure/Swelling Relationships of Bulk and Thin-Film PFSA Ionomers
journal, May 2016
- Kusoglu, Ahmet; Dursch, Thomas J.; Weber, Adam Z.
- Advanced Functional Materials, Vol. 26, Issue 27
Polarization loss correction derived from hydrogen local-resistance measurement in low Pt-loaded polymer-electrolyte fuel cells
journal, June 2017
- Freiberg, Anna T. S.; Tucker, Michael C.; Weber, Adam Z.
- Electrochemistry Communications, Vol. 79
Humidity and Temperature Dependences of Oxygen Transport Resistance of Nafion Thin Film on Platinum Electrode
journal, August 2016
- Kudo, Kenji; Jinnouchi, Ryosuke; Morimoto, Yu
- Electrochimica Acta, Vol. 209
Influence of Equivalent Weight of Ionomer on Local Oxygen Transport Resistance in Cathode Catalyst Layers
journal, January 2013
- Ono, Yoshitaka; Ohma, Atsushi; Shinohara, Kazuhiko
- Journal of The Electrochemical Society, Vol. 160, Issue 8
Modeling of the operation conditions on the gas purging performance of polymer electrolyte membrane fuel cells
journal, April 2017
- Mu, Yu-Tong; He, Pu; Ding, Jing
- International Journal of Hydrogen Energy, Vol. 42, Issue 16
Exploration of significant influences of the operating conditions on the local O 2 transport in proton exchange membrane fuel cells (PEMFCs)
journal, January 2017
- Shen, Shuiyun; Cheng, Xiaojing; Wang, Chao
- Physical Chemistry Chemical Physics, Vol. 19, Issue 38