Ferromagnetic order beyond the superconducting dome in a cuprate superconductor
Abstract
According to conventional wisdom, the extraordinary properties of the cuprate high-temperature superconductors arise from doping a strongly correlated antiferromagnetic insulator. The highly overdoped cuprates—whose doping lies beyond the dome of superconductivity—are considered to be conventional Fermi liquid metals. We report the emergence of itinerant ferromagnetic order below 4 kelvin for doping beyond the superconducting dome in thin films of electron-doped La 2– x Ce x CuO 4 (LCCO). The existence of this ferromagnetic order is evidenced by negative, anisotropic, and hysteretic magnetoresistance, hysteretic magnetization, and the polar Kerr effect, all of which are standard signatures of itinerant ferromagnetism in metals. This surprising result suggests that the overdoped cuprates are strongly influenced by electron correlations.
- Authors:
-
- Maryland Quantum Materials Center and Department of Physics, University of Maryland, College Park, MD 20742, USA.
- Geballe Laboratory for Advanced Materials, Stanford University, Stanford, CA 94305, USA., Department of Applied Physics, Stanford University, Stanford, CA 94305, USA.
- State Key Laboratory of Surface Physics, Department of Physics, Fudan University, Shanghai 200433, People’s Republic of China.
- Geballe Laboratory for Advanced Materials, Stanford University, Stanford, CA 94305, USA., Department of Applied Physics, Stanford University, Stanford, CA 94305, USA., Department of Physics, Stanford University, Stanford, CA 94305, USA., Stanford Institute for Materials and Energy Sciences (SIMES), SLAC National Accelerator Laboratory, Menlo Park, CA 94025, USA.
- Publication Date:
- Research Org.:
- SLAC National Accelerator Lab., Menlo Park, CA (United States)
- Sponsoring Org.:
- USDOE
- OSTI Identifier:
- 1616651
- Alternate Identifier(s):
- OSTI ID: 1633186
- Grant/Contract Number:
- AC02-76SF00515; DMR-1708334; FA9550-14-10332; GBMF5305
- Resource Type:
- Published Article
- Journal Name:
- Science
- Additional Journal Information:
- Journal Name: Science Journal Volume: 368 Journal Issue: 6490; Journal ID: ISSN 0036-8075
- Publisher:
- American Association for the Advancement of Science (AAAS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY
Citation Formats
Sarkar, Tarapada, Wei, D. S., Zhang, J., Poniatowski, N. R., Mandal, P. R., Kapitulnik, A., and Greene, Richard L. Ferromagnetic order beyond the superconducting dome in a cuprate superconductor. United States: N. p., 2020.
Web. doi:10.1126/science.aax1581.
Sarkar, Tarapada, Wei, D. S., Zhang, J., Poniatowski, N. R., Mandal, P. R., Kapitulnik, A., & Greene, Richard L. Ferromagnetic order beyond the superconducting dome in a cuprate superconductor. United States. https://doi.org/10.1126/science.aax1581
Sarkar, Tarapada, Wei, D. S., Zhang, J., Poniatowski, N. R., Mandal, P. R., Kapitulnik, A., and Greene, Richard L. Thu .
"Ferromagnetic order beyond the superconducting dome in a cuprate superconductor". United States. https://doi.org/10.1126/science.aax1581.
@article{osti_1616651,
title = {Ferromagnetic order beyond the superconducting dome in a cuprate superconductor},
author = {Sarkar, Tarapada and Wei, D. S. and Zhang, J. and Poniatowski, N. R. and Mandal, P. R. and Kapitulnik, A. and Greene, Richard L.},
abstractNote = {According to conventional wisdom, the extraordinary properties of the cuprate high-temperature superconductors arise from doping a strongly correlated antiferromagnetic insulator. The highly overdoped cuprates—whose doping lies beyond the dome of superconductivity—are considered to be conventional Fermi liquid metals. We report the emergence of itinerant ferromagnetic order below 4 kelvin for doping beyond the superconducting dome in thin films of electron-doped La 2– x Ce x CuO 4 (LCCO). The existence of this ferromagnetic order is evidenced by negative, anisotropic, and hysteretic magnetoresistance, hysteretic magnetization, and the polar Kerr effect, all of which are standard signatures of itinerant ferromagnetism in metals. This surprising result suggests that the overdoped cuprates are strongly influenced by electron correlations.},
doi = {10.1126/science.aax1581},
journal = {Science},
number = 6490,
volume = 368,
place = {United States},
year = {Thu Apr 30 00:00:00 EDT 2020},
month = {Thu Apr 30 00:00:00 EDT 2020}
}
https://doi.org/10.1126/science.aax1581
Web of Science
Works referenced in this record:
The phase diagram of electron-doped La2−xCexCuO4−δ
journal, January 2015
- Saadaoui, H.; Salman, Z.; Luetkens, H.
- Nature Communications, Vol. 6, Issue 1
Magnetoresistance in Mn Pyrochlore: Electrical Transport in a Low Carrier Density Ferromagnet
journal, August 1998
- Majumdar, Pinaki; Littlewood, Peter
- Physical Review Letters, Vol. 81, Issue 6
Three-dimensional collective charge excitations in electron-doped copper oxide superconductors
journal, October 2018
- Hepting, M.; Chaix, L.; Huang, E. W.
- Nature, Vol. 563, Issue 7731
Modified Sagnac interferometer for high-sensitivity magneto-optic measurements at cryogenic temperatures
journal, August 2006
- Xia, Jing; Beyersdorf, Peter T.; Fejer, M. M.
- Applied Physics Letters, Vol. 89, Issue 6
Broken rotational symmetry in the pseudogap phase of a high-Tc superconductor
journal, January 2010
- Daou, R.; Chang, J.; LeBoeuf, David
- Nature, Vol. 463, Issue 7280
Competing charge, spin, and superconducting orders in underdoped
journal, August 2014
- Hücker, M.; Christensen, N. B.; Holmes, A. T.
- Physical Review B, Vol. 90, Issue 5
Correlation between scale-invariant normal-state resistivity and superconductivity in an electron-doped cuprate
journal, May 2019
- Sarkar, Tarapada; Mandal, P. R.; Poniatowski, N. R.
- Science Advances, Vol. 5, Issue 5
Anomalous Criticality in the Electrical Resistivity of La2-xSrxCuO4
journal, January 2009
- Cooper, R. A.; Wang, Y.; Vignolle, B.
- Science, Vol. 323, Issue 5914
Ubiquity of ferromagnetic signals in common diamagnetic oxide crystals
journal, June 2010
- Khalid, M.; Setzer, A.; Ziese, M.
- Physical Review B, Vol. 81, Issue 21
Emergent ferromagnetism near three-quarters filling in twisted bilayer graphene
journal, July 2019
- Sharpe, Aaron L.; Fox, Eli J.; Barnard, Arthur W.
- Science, Vol. 365, Issue 6453
From quantum matter to high-temperature superconductivity in copper oxides
journal, February 2015
- Keimer, B.; Kivelson, S. A.; Norman, M. R.
- Nature, Vol. 518, Issue 7538
Competing ferromagnetism in high-temperature copper oxide superconductors
journal, April 2007
- Kopp, A.; Ghosal, A.; Chakravarty, S.
- Proceedings of the National Academy of Sciences, Vol. 104, Issue 15
The pseudogap: friend or foe of high T c ?
journal, December 2005
- Norman, M. R.; Pines, D.; Kallin, C.
- Advances in Physics, Vol. 54, Issue 8
Quantum critical scaling at the edge of Fermi liquid stability in a cuprate superconductor
journal, May 2012
- Butch, N. P.; Jin, K.; Kirshenbaum, K.
- Proceedings of the National Academy of Sciences, Vol. 109, Issue 22
Magnetic-field induced resistivity minimum with in-plane linear magnetoresistance of the Fermi liquid in SrTiO single crystals
journal, April 2012
- Liu, Z. Q.; Lü, W. M.; Wang, X.
- Physical Review B, Vol. 85, Issue 15
Anomalous quantum criticality in the electron-doped cuprates
journal, March 2019
- Mandal, P. R.; Sarkar, Tarapada; Greene, Richard L.
- Proceedings of the National Academy of Sciences, Vol. 116, Issue 13
Observation of broken time-reversal symmetry in the heavy-fermion superconductor UPt3
journal, July 2014
- Schemm, E. R.; Gannon, W. J.; Wishne, C. M.
- Science, Vol. 345, Issue 6193
Giant magnetoresistance in Ti2Mn2O7 with the pyrochlore structure
journal, January 1996
- Shimakawa, Y.; Kubo, Y.; Manako, T.
- Nature, Vol. 379, Issue 6560
Spin scattering in ferromagnetic thin films
journal, April 1996
- Viret, M.; Vignoles, D.; Cole, D.
- Physical Review B, Vol. 53, Issue 13
High Resolution Polar Kerr Effect Measurements of : Evidence for Broken Time-Reversal Symmetry in the Superconducting State
journal, October 2006
- Xia, Jing; Maeno, Yoshiteru; Beyersdorf, Peter T.
- Physical Review Letters, Vol. 97, Issue 16
Electron-doped superconductor Preparation of thin films and modified doping range for superconductivity
journal, July 2002
- Sawa, A.; Kawasaki, M.; Takagi, H.
- Physical Review B, Vol. 66, Issue 1
Surface magnetism of strontium titanate
journal, September 2016
- Coey, J. M. D.; Venkatesan, M.; Stamenov, P.
- Journal of Physics: Condensed Matter, Vol. 28, Issue 48
Spin fluctuations in a very weak itinerant ferromagnet: Y 4 Co 3
journal, May 1984
- Kolodziejczyk, A.; Spalek, J.
- Journal of Physics F: Metal Physics, Vol. 14, Issue 5
Ferromagnetism and Conductivity in Atomically Thin
journal, February 2019
- Boschker, H.; Harada, T.; Asaba, T.
- Physical Review X, Vol. 9, Issue 1
Link between spin fluctuations and electron pairing in copper oxide superconductors
journal, August 2011
- Jin, K.; Butch, N. P.; Kirshenbaum, K.
- Nature, Vol. 476, Issue 7358
Dependence of the critical temperature in overdoped copper oxides on superfluid density
journal, August 2016
- Božović, I.; He, X.; Wu, J.
- Nature, Vol. 536, Issue 7616
The Strange Metal State of the Electron-Doped Cuprates
journal, March 2020
- Greene, Richard L.; Mandal, Pampa R.; Poniatowski, Nicholas R.
- Annual Review of Condensed Matter Physics, Vol. 11, Issue 1
Anisotropic magnetoresistance in ferromagnetic 3d alloys
journal, July 1975
- McGuire, T.; Potter, R.
- IEEE Transactions on Magnetics, Vol. 11, Issue 4
Magnetic-field-induced charge-stripe order in the high-temperature superconductor YBa2Cu3Oy
journal, September 2011
- Wu, Tao; Mayaffre, Hadrien; Krämer, Steffen
- Nature, Vol. 477, Issue 7363
Evidence for broken time-reversal symmetry in the superconducting phase of
journal, April 2015
- Schemm, E. R.; Baumbach, R. E.; Tobash, P. H.
- Physical Review B, Vol. 91, Issue 14
Antiferromagnetic spin fluctuation and superconductivity
journal, July 2003
- Moriya, T. ru; Ueda, Kazuo
- Reports on Progress in Physics, Vol. 66, Issue 8
Doping a Mott insulator: Physics of high-temperature superconductivity
journal, January 2006
- Lee, Patrick A.; Nagaosa, Naoto; Wen, Xiao-Gang
- Reviews of Modern Physics, Vol. 78, Issue 1
Doping-dependent charge order correlations in electron-doped cuprates
journal, August 2016
- da Silva Neto, Eduardo H.; Yu, Biqiong; Minola, Matteo
- Science Advances, Vol. 2, Issue 8
Direct search for a ferromagnetic phase in a heavily overdoped nonsuperconducting copper oxide
journal, September 2010
- Sonier, J. E.; Kaiser, C. V.; Pacradouni, V.
- Proceedings of the National Academy of Sciences, Vol. 107, Issue 40
Progress and perspectives on electron-doped cuprates
journal, September 2010
- Armitage, N. P.; Fournier, P.; Greene, R. L.
- Reviews of Modern Physics, Vol. 82, Issue 3
Superconductivity on the border of itinerant-electron ferromagnetism in UGe2
journal, August 2000
- Saxena, S. S.; Agarwal, P.; Ahilan, K.
- Nature, Vol. 406, Issue 6796
Development of Ferromagnetic Fluctuations in Heavily Overdoped Copper Oxides
journal, August 2018
- Kurashima, Koshi; Adachi, Tadashi; Suzuki, Kensuke M.
- Physical Review Letters, Vol. 121, Issue 5
Universal T-linear resistivity and Planckian dissipation in overdoped cuprates
journal, November 2018
- Legros, A.; Benhabib, S.; Tabis, W.
- Nature Physics, Vol. 15, Issue 2
Anisotropic Thermopower and Planar Nernst Effect in Ferromagnetic Semiconductors
journal, July 2006
- Pu, Yong; Johnston-Halperin, E.; Awschalom, D. D.
- Physical Review Letters, Vol. 97, Issue 3