Disentangling spin-orbit coupling and local magnetism in a quasi-two-dimensional electron system
Abstract
Quantum interference between time-reversed electron paths in two dimensions (2D) leads to the well-known weak localization correction to resistance. If spin-orbit coupling is present, the resistance correction is negative, termed weak antilocalization (WAL). Here, we report the observation of WAL coexisting with exchange coupling between itinerant electrons and localized magnetic moments. We use low-temperature magnetotransport measurements to investigate the quasi-two-dimensional, high-electron-density interface formed between SrTiO3 and the antiferromagnetic Mott insulator NdTiO3. As the magnetic field angle is gradually tilted away from the sample normal, the data reveal the interplay between strong k-cubic Rashba-type spin-orbit coupling and a substantial magnetic exchange interaction from local magnetic regions. The resulting quantum corrections to the conduction are in excellent agreement with existing models and allow sensitive determination of the small magnetic moments (22 μB on average), their magnetic anisotropy, and mutual coupling strength. Furthermore, this effect is expected to arise in other 2D magnetic materials systems.
- Authors:
-
- Univ. of Minnesota, Minneapolis, MN (United States)
- Publication Date:
- Research Org.:
- Univ. of Minnesota, Minneapolis, MN (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC)
- OSTI Identifier:
- 1612515
- Alternate Identifier(s):
- OSTI ID: 1547976
- Grant/Contract Number:
- SC0016371; SC-0016371
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Physical Review B
- Additional Journal Information:
- Journal Volume: 100; Journal Issue: 8; Journal ID: ISSN 2469-9950
- Publisher:
- American Physical Society (APS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; Materials Science; Physics; Magnetism; Magnetotransport; Quantum interference effects; Spin-orbit coupling; Weak antilocalization; Complex oxides; Two-dimensional electron system
Citation Formats
Cai, Xinxin, Ayino, Yilikal, Yue, Jin, Xu, Peng, Jalan, Bharat, and Pribiag, Vlad S. Disentangling spin-orbit coupling and local magnetism in a quasi-two-dimensional electron system. United States: N. p., 2019.
Web. doi:10.1103/physrevb.100.081402.
Cai, Xinxin, Ayino, Yilikal, Yue, Jin, Xu, Peng, Jalan, Bharat, & Pribiag, Vlad S. Disentangling spin-orbit coupling and local magnetism in a quasi-two-dimensional electron system. United States. https://doi.org/10.1103/physrevb.100.081402
Cai, Xinxin, Ayino, Yilikal, Yue, Jin, Xu, Peng, Jalan, Bharat, and Pribiag, Vlad S. Wed .
"Disentangling spin-orbit coupling and local magnetism in a quasi-two-dimensional electron system". United States. https://doi.org/10.1103/physrevb.100.081402. https://www.osti.gov/servlets/purl/1612515.
@article{osti_1612515,
title = {Disentangling spin-orbit coupling and local magnetism in a quasi-two-dimensional electron system},
author = {Cai, Xinxin and Ayino, Yilikal and Yue, Jin and Xu, Peng and Jalan, Bharat and Pribiag, Vlad S.},
abstractNote = {Quantum interference between time-reversed electron paths in two dimensions (2D) leads to the well-known weak localization correction to resistance. If spin-orbit coupling is present, the resistance correction is negative, termed weak antilocalization (WAL). Here, we report the observation of WAL coexisting with exchange coupling between itinerant electrons and localized magnetic moments. We use low-temperature magnetotransport measurements to investigate the quasi-two-dimensional, high-electron-density interface formed between SrTiO3 and the antiferromagnetic Mott insulator NdTiO3. As the magnetic field angle is gradually tilted away from the sample normal, the data reveal the interplay between strong k-cubic Rashba-type spin-orbit coupling and a substantial magnetic exchange interaction from local magnetic regions. The resulting quantum corrections to the conduction are in excellent agreement with existing models and allow sensitive determination of the small magnetic moments (22 μB on average), their magnetic anisotropy, and mutual coupling strength. Furthermore, this effect is expected to arise in other 2D magnetic materials systems.},
doi = {10.1103/physrevb.100.081402},
journal = {Physical Review B},
number = 8,
volume = 100,
place = {United States},
year = {Wed Aug 07 00:00:00 EDT 2019},
month = {Wed Aug 07 00:00:00 EDT 2019}
}
Web of Science
Works referenced in this record:
Coexistence of magnetic order and two-dimensional superconductivity at LaAlO3/SrTiO3 interfaces
journal, September 2011
- Li, Lu; Richter, C.; Mannhart, J.
- Nature Physics, Vol. 7, Issue 10, p. 762-766
Magnetoresistance of a weakly disordered III-V semiconductor quantum well in a magnetic field parallel to interfaces
journal, September 1997
- Mal’shukov, A. G.; Chao, K. A.; Willander, M.
- Physical Review B, Vol. 56, Issue 11
Magnetic effects at the interface between non-magnetic oxides
journal, June 2007
- Brinkman, A.; Huijben, M.; van Zalk, M.
- Nature Materials, Vol. 6, Issue 7, p. 493-496
Weak-localization corrections to the conductivity of double quantum wells
journal, January 2000
- Raichev, O. E.; Vasilopoulos, P.
- Journal of Physics: Condensed Matter, Vol. 12, Issue 5
Quantum Transport in Parallel Magnetic Fields: A Realization of the Berry-Robnik Symmetry Phenomenon
journal, October 2002
- Meyer, Julia S.; Altland, Alexander; Altshuler, B. L.
- Physical Review Letters, Vol. 89, Issue 20
Quasi 2D Ultrahigh Carrier Density in a Complex Oxide Broken-Gap Heterojunction
journal, November 2015
- Xu, Peng; Droubay, Timothy C.; Jeong, Jong Seok
- Advanced Materials Interfaces, Vol. 3, Issue 2
Ferromagnetism and spin-dependent transport at a complex oxide interface
journal, March 2018
- Ayino, Yilikal; Xu, Peng; Tigre-Lazo, Juan
- Physical Review Materials, Vol. 2, Issue 3
Effect of the 110°K Phase Transition on the SrTi Conduction Bands
journal, December 1972
- Mattheiss, L. F.
- Physical Review B, Vol. 6, Issue 12
Spin-Orbit Coupling, Antilocalization, and Parallel Magnetic Fields in Quantum Dots
journal, December 2002
- Zumbühl, D. M.; Miller, J. B.; Marcus, C. M.
- Physical Review Letters, Vol. 89, Issue 27
Gate-tunable polarized phase of two-dimensional electrons at the LaAlO3/SrTiO3 interface
journal, May 2013
- Joshua, A.; Ruhman, J.; Pecker, S.
- Proceedings of the National Academy of Sciences, Vol. 110, Issue 24
Coexistence of Superconductivity and Ferromagnetism in Two Dimensions
journal, July 2011
- Dikin, D. A.; Mehta, M.; Bark, C. W.
- Physical Review Letters, Vol. 107, Issue 5, Article No. 056802
Predictive Control over Charge Density in the Two-Dimensional Electron Gas at the Polar-Nonpolar Interface
journal, September 2016
- Xu, Peng; Ayino, Yilikal; Cheng, Christopher
- Physical Review Letters, Vol. 117, Issue 10
Molecular beam epitaxy of SrTiO3 with a growth window
journal, July 2009
- Jalan, Bharat; Moetakef, Pouya; Stemmer, Susanne
- Applied Physics Letters, Vol. 95, Issue 3
Spin-Orbit Interaction and Magnetoresistance in the Two Dimensional Random System
journal, February 1980
- Hikami, S.; Larkin, A. I.; Nagaoka, Y.
- Progress of Theoretical Physics, Vol. 63, Issue 2
Nanoscale Phenomena in Oxide Heterostructures
journal, July 2014
- Sulpizio, Joseph A.; Ilani, Shahal; Irvin, Patrick
- Annual Review of Materials Research, Vol. 44, Issue 1
A New Line Defect in NdTiO 3 Perovskite
journal, October 2016
- Jeong, Jong Seok; Topsakal, Mehmet; Xu, Peng
- Nano Letters, Vol. 16, Issue 11
Random Berry phase magnetoresistance as a probe of interface roughness in Si MOSFET’s
journal, November 2001
- Mathur, H.; Baranger, Harold U.
- Physical Review B, Vol. 64, Issue 23
Electric field control of the LaAlO3/SrTiO3 interface ground state
journal, December 2008
- Caviglia, A. D.; Gariglio, S.; Reyren, N.
- Nature, Vol. 456, Issue 7222
The Structural and Magnetic Properties of Nd1−xTiO3forx= 0, 0.05, and 0.10
journal, February 1996
- Amow, G.; Greedan, J. E.
- Journal of Solid State Chemistry, Vol. 121, Issue 2
Stoichiometry-driven metal-to-insulator transition in NdTiO 3 /SrTiO 3 heterostructures
journal, February 2014
- Xu, Peng; Phelan, Daniel; Seok Jeong, Jong
- Applied Physics Letters, Vol. 104, Issue 8
Experimental Evidence of Cubic Rashba Effect in an Inversion-Symmetric Oxide
journal, May 2012
- Nakamura, H.; Koga, T.; Kimura, T.
- Physical Review Letters, Vol. 108, Issue 20
Strong spin-orbit coupling and magnetism in (111)
journal, August 2018
- Bal, V. V.; Huang, Z.; Han, K.
- Physical Review B, Vol. 98, Issue 8
Weak antilocalization and spin precession in quantum wells
journal, February 1996
- Knap, W.; Skierbiszewski, C.; Zduniak, A.
- Physical Review B, Vol. 53, Issue 7
A high-mobility electron gas at the LaAlO3/SrTiO3 heterointerface
journal, January 2004
- Ohtomo, A.; Hwang, H. Y.
- Nature, Vol. 427, Issue 6973
Effect of hole doping on the magnetic properties of the Mott-Hubbard antiferromagnetic insulator
journal, September 2006
- Sefat, Athena S.; Greedan, John E.; Cranswick, Lachlan
- Physical Review B, Vol. 74, Issue 10
Superconducting Interfaces Between Insulating Oxides
journal, August 2007
- Reyren, N.; Thiel, S.; Caviglia, A. D.
- Science, Vol. 317, Issue 5842
Weak antilocalization in quantum wells in tilted magnetic fields
journal, October 2004
- Minkov, G. M.; Germanenko, A. V.; Rut, O. E.
- Physical Review B, Vol. 70, Issue 15
Magnetoresistance in Two-Dimensional Disordered Systems: Effects of Zeeman Splitting and Spin-Orbit Scattering
journal, August 1981
- Maekawa, Sadamichi; Fukuyama, Hidetoshi
- Journal of the Physical Society of Japan, Vol. 50, Issue 8
Weak localization in ferromagnets with spin-orbit interaction
journal, September 2001
- Dugaev, V. K.; Bruno, P.; Barnaś, J.
- Physical Review B, Vol. 64, Issue 14
Photoemission from Buried Interfaces in Superlattices
journal, August 2006
- Takizawa, M.; Wadati, H.; Tanaka, K.
- Physical Review Letters, Vol. 97, Issue 5
Carrier-Controlled Ferromagnetism in
journal, June 2012
- Moetakef, Pouya; Williams, James R.; Ouellette, Daniel G.
- Physical Review X, Vol. 2, Issue 2
Granular Cu-Co alloys as interacting superparamagnets
journal, September 2001
- Allia, Paolo; Coisson, Marco; Tiberto, Paola
- Physical Review B, Vol. 64, Issue 14
Emergent nanoscale superparamagnetism at oxide interfaces
journal, August 2016
- Anahory, Y.; Embon, L.; Li, C. J.
- Nature Communications, Vol. 7, Issue 1
Electrostatic carrier doping of GdTiO 3 /SrTiO 3 interfaces
journal, December 2011
- Moetakef, Pouya; Cain, Tyler A.; Ouellette, Daniel G.
- Applied Physics Letters, Vol. 99, Issue 23
Direct imaging of the coexistence of ferromagnetism and superconductivity at the LaAlO3/SrTiO3 interface
journal, September 2011
- Bert, Julie A.; Kalisky, Beena; Bell, Christopher
- Nature Physics, Vol. 7, Issue 10, p. 767-771
Tunable Rashba Spin-Orbit Interaction at Oxide Interfaces
journal, March 2010
- Caviglia, A. D.; Gabay, M.; Gariglio, S.
- Physical Review Letters, Vol. 104, Issue 12, Article No. 126803
Two-dimensional superconductivity at a Mott insulator/band insulator interface LaTiO3/SrTiO3
journal, October 2010
- Biscaras, J.; Bergeal, N.; Kushwaha, A.
- Nature Communications, Vol. 1, Issue 1
Tuning Spin-Orbit Coupling and Superconductivity at the Interface: A Magnetotransport Study
journal, March 2010
- Ben Shalom, M.; Sachs, M.; Rakhmilevitch, D.
- Physical Review Letters, Vol. 104, Issue 12
Coexistence of superconductivity and ferromagnetism in two dimensions
text, January 2011
- Dikin, D. A.; Mehta, M.; Bark, C. W.
- arXiv
Direct imaging of the coexistence of ferromagnetism and superconductivity at the LaAlO3/SrTiO3 interface
text, January 2011
- Bert, J. A.; Kalisky, B.; Bell, C.
- arXiv
Electrostatic carrier doping of GdTiO3/SrTiO3 interfaces
text, January 2011
- Moetakef, Pouya; Cain, Tyler A.; Ouellette, Daniel G.
- arXiv
Nanoscale Phenomena in Oxide Heterostructures
text, January 2014
- Sulpizio, Joseph A.; Ilani, Shahal; Irvin, Patrick
- arXiv
Emergent nanoscale superparamagnetism at oxide interfaces
text, January 2015
- Anahory, Yonathan; Embon, Lior; Li, Chang Jian
- arXiv
A New Line Defect in NdTiO3 Perovskite
text, January 2016
- Jeong, Jong Seok; Topsakal, Mehmet; Xu, Peng
- arXiv
Weak localization in ferromagnets with spin-orbit interaction
text, January 2001
- Dugaev, V. K.; Bruno, P.; Barnas, J.
- arXiv
Weak antilocalization in quantum wells in tilted magnetic fields
text, January 2003
- Minkov, G. M.; Germanenko, A. V.; Rut, O. E.
- arXiv
Weak-localization corrections to the conductivity of double quantum wells
text, January 1999
- Raichev, O. E.; Vasilopoulos, P.
- arXiv