Field-induced ferrohastatic phase in cubic non-Kramers doublet systems

Van Dyke, John S.; Zhang, Guanghua; Flint, Rebecca

doi:10.1103/PhysRevB.100.205122

Title: Field-induced ferrohastatic phase in cubic non-Kramers doublet systems

Journal Article · 17 November 2019 · Physical Review B

DOI: https://doi.org/10.1103/PhysRevB.100.205122 · OSTI ID:1595302

^[1]; Zhang, Guanghua ^[2]; Flint, Rebecca ^[2]

Iowa State Univ., Ames, IA (United States); Iowa State University
Iowa State Univ., Ames, IA (United States)

Cubic Pr-based compounds with $$Γ$$₃ non-Kramers doublet ground states can realize a novel heavy Fermi liquid with spinorial hybridization (“hastatic” order) that breaks time-reversal symmetry. Several Pr-“1-2-20” materials exhibit a suggestive heavy Fermi liquid stabilized in intermediate magnetic fields; these provide key insight into the quadrupolar Kondo lattice. In this work, we develop a simple yet realistic microscopic model of ferrohastatic order and elaborate its experimental signatures and behavior in field, where it is a good candidate to explain the observed heavy Fermi liquids at intermediate fields in Pr(Ir,Rh)₂Zn₂₀. In addition, we develop the Landau theory of ferrohastatic order, which allows us to understand its behavior close to the transition and explore thermodynamic signatures from magnetic susceptibility to thermal expansion.

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Research Organization:: Iowa State Univ., Ames, IA (United States)

Sponsoring Organization:: National Science Foundation (NSF); USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division

Grant/Contract Number:: SC0015891

OSTI ID:: 1595302

Journal Information:: Physical Review B, Journal Name: Physical Review B Journal Issue: 20 Vol. 100; ISSN 2469-9950; ISSN PRBMDO

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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