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Title: Organic–Inorganic Perovskites: Structural Versatility for Functional Materials Design

Journal Article · · Chemical Reviews
 [1];  [2]
  1. Duke Univ., Durham, NC (United States). Dept. of Mechanical Engineering and Materials Science and Dept. of Chemistry; Duke University
  2. Duke Univ., Durham, NC (United States). Dept. of Mechanical Engineering and Materials Science and Dept. of Chemistry
+ Show Author Affiliations

Although known since the late 19th century, organic–inorganic perovskites have recently received extraordinary research community attention because of their unique physical properties, which make them promising candidates for application in photovoltaic (PV) and related optoelectronic devices. In this review, we will explore beyond the current focus on three-dimensional (3-D) lead(II) halide perovskites, to highlight the great chemical flexibility and outstanding potential of the broader class of 3-D and lower dimensional organic-based perovskite family for electronic, optical, and energy-based applications as well as fundamental research. The concept of a multifunctional organic–inorganic hybrid, in which the organic and inorganic structural components provide intentional, unique, and hopefully synergistic features to the compound, represents an important contemporary target.

Research Organization:
Duke Univ., Durham, NC (United States)
Sponsoring Organization:
USDOE Office of Energy Efficiency and Renewable Energy (EERE)
Grant/Contract Number:
EE0006712; AC05-06OR23100
OSTI ID:
1593872
Journal Information:
Chemical Reviews, Journal Name: Chemical Reviews Journal Issue: 7 Vol. 116; ISSN 0009-2665
Publisher:
American Chemical SocietyCopyright Statement
Country of Publication:
United States
Language:
English

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  • Weber, Oliver J.; Marshall, Kayleigh L.; Dyson, Lewis M.
  • Acta Crystallographica Section B Structural Science, Crystal Engineering and Materials, Vol. 71, Issue 6 https://doi.org/10.1107/S2052520615019885
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Organic-Inorganic Hybrid Materials as Semiconducting Channels in Thin-Film Field-Effect Transistors journal October 1999
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High Field-Effect Hole Mobility in Organic-Inorganic Hybrid Thin Films Prepared by Vacuum Vapor Deposition Technique journal August 2004
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Exciton Features in 0-, 2-, and 3-Dimensional Networks of [PbI 6 ] 4- Octahedra journal October 1994
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Melting temperature suppression of layered hybrid lead halide perovskites via organic ammonium cation branching journal January 2019
Recent progressive efforts in perovskite solar cells toward commercialization journal January 2018
An Er-doped TiO 2 phase junction as an electron transport layer for efficient perovskite solar cells fabricated in air journal January 2018
Tolerance factors of hybrid organic–inorganic perovskites: recent improvements and current state of research journal January 2018
Impact of cesium on the phase and device stability of triple cation Pb–Sn double halide perovskite films and solar cells journal January 2018
Synthesis of ultrathin two-dimensional organic–inorganic hybrid perovskite nanosheets for polymer field-effect transistors journal January 2018
The effect of ionic composition on acoustic phonon speeds in hybrid perovskites from Brillouin spectroscopy and density functional theory journal January 2018
Unraveling luminescence mechanisms in zero-dimensional halide perovskites journal January 2018
Zero-dimensional Cs 4 EuX 6 (X = Br, I) all-inorganic perovskite single crystals for gamma-ray spectroscopy journal January 2018
Above-room-temperature switching of quadratic nonlinear optical properties in a Bi–halide organic–inorganic hybrid journal January 2018
Molecular engineering of two-dimensional hybrid perovskites with broadband emission for white light-emitting diodes journal January 2018
Dielectric phase transition triggered by the order–disorder transformation of cyclopropylamine in a layered organic–inorganic halide perovskite journal January 2018
Luminescent perovskite quantum dots: synthesis, microstructures, optical properties and applications journal January 2019
B-Site doped lead halide perovskites: synthesis, band engineering, photophysics, and light emission applications journal January 2019
Temperature- and pressure-dependent studies of a highly flexible and compressible perovskite-like cadmium dicyanamide framework templated with protonated tetrapropylamine journal January 2019
Interfacial engineering for highly efficient quasi-two dimensional organic–inorganic hybrid perovskite light-emitting diodes journal January 2019
Temperature dependent geometry in perovskite microcrystals for whispering gallery and Fabry–Pérot mode lasing journal January 2019
Polymorphism in M(H 2 PO 2 ) 3 (M = V, Al, Ga) compounds with the perovskite-related ReO 3 structure journal January 2019
Mechanical properties of the ferroelectric metal-free perovskite [MDABCO](NH 4 )I 3 journal January 2019
Switching hydrogen bonds to readily interconvert two room-temperature long-term stable crystalline polymorphs in chiral molecular perovskites journal January 2019
Strongly emissive white-light-emitting silver iodide based inorganic–organic hybrid structures with comparable quantum efficiency to commercial phosphors journal January 2020
Theoretical insights into inorganic–organic intercalation products of the layered perovskite HLaNb 2 O 7 : perspectives for hybrid proton conductors journal January 2019
Optical deformation potential and self-trapped excitons in 2D hybrid perovskites journal January 2019
Ultrahigh phase transition temperature in a metal–halide perovskite-type material containing unprecedented hydrogen bonding interactions journal January 2019
Enhanced yield-mobility products in hybrid halide Ruddlesden–Popper compounds with aromatic ammonium spacers journal January 2019
Perovzalates: a family of perovskite-related oxalates journal January 2019
Effect of interlayer spacing in layered perovskites on resistive switching memory journal January 2019
Simple fabrication of layered halide perovskite platelets and enhanced photoluminescence from mechanically exfoliated flakes journal January 2019
Impact of cesium in methylammonium lead bromide perovskites: insights into the microstructures, stability and photophysical properties journal January 2019
Understanding the mechanism of metal-induced degradation in perovskite nanocrystals journal January 2019
Semiconducting crystalline inorganic–organic hybrid metal halide nanochains journal January 2020
Rare earth double perovskites: a fertile soil in the field of perovskite oxides journal January 2019
Organic cation directed hybrid lead halides of zero-dimensional to two-dimensional structures with tunable photoluminescence properties journal January 2019
Luminescent perovskites: recent advances in theory and experiments journal January 2019
Exploring high-performance integration in a plastic crystal/film with switching and semiconducting behavior journal January 2020
Additive-assisted synthesis and optoelectronic properties of (CH 3 NH 3 ) 4 Bi 6 I 22 journal January 2020
Ethylammonium as an alternative cation for efficient perovskite solar cells from first-principles calculations journal January 2019
Centimeter-scale 2D perovskite (PEA) 2 PbBr 4 single crystal plates grown by a seeded solution method for photodetectors journal January 2019
Cs 4 PbBr 6 /CsPbBr 3 perovskite composites for WLEDs: pure white, high luminous efficiency and tunable color temperature journal January 2019
Modifying perovskite solar cells with l (+)-cysteine at the interface between mesoporous TiO 2 and perovskite journal January 2020
Lead-free low-dimensional tin halide perovskites with functional organic spacers: breaking the charge-transport bottleneck journal January 2019
Inorganic perovskite solar cells: an emerging member of the photovoltaic community journal January 2019
Zero-dimensional metal oxide Li 4 TiO 4 journal January 2019
Unprecedented 30 K hysteresis across switchable dielectric and magnetic properties in a bright luminescent organic–inorganic halide (CH 6 N 3 ) 2 MnCl 4 journal January 2019
White light emission in low-dimensional perovskites journal January 2019
Highly efficient CsPbBr 3 perovskite nanocrystals induced by structure transformation between CsPbBr 3 and Cs 4 PbBr 6 phases journal January 2019
Constructing moisture-stable hybrid lead iodine semiconductors based on hydrogen-bond-free and dual-iodine strategies journal January 2019
Enhancing the phosphorescence of hybrid metal halides through molecular sensitization journal January 2019
Remarkable dielectric breakdown strength enhancement of a PVDF terpolymer using a 2D hybrid organic inorganic perovskite as a functional additive journal January 2019
Inducing formation of a corrugated, white-light emitting 2D lead-bromide perovskite via subtle changes in templating cation journal January 2020
Unprecedented tin iodide perovskite-like structures featuring ordering of organic moieties journal January 2020
Spin-crossover in an organic–inorganic hybrid perovskite journal January 2020
Nonlinear organic–inorganic halide hybrids containing unprecedented linear [MIX 2 ] − coordination units and quasi-two-dimensional lone pairs journal January 2020
Synthetic strategy towards halometallates with imidazo[1,5- a ]pyridinium-based counterions journal January 2020
Complexes of BiCl 3 with hydrazone derived ligands: a Möbius-like discrete metal chelate versus a salt-like porous polymeric structure journal January 2020
Novel hypophosphite hybrid perovskites of [CH 3 NH 2 NH 2 ][Mn(H 2 POO) 3 ] and [CH 3 NH 2 NH 2 ][Mn(H 2 POO) 2.83 (HCOO) 0.17 ] exhibiting antiferromagnetic order and red photoluminescence journal January 2020
Research Update: Challenges for high-efficiency hybrid lead-halide perovskite LEDs and the path towards electrically pumped lasing journal September 2016
First principles study of 2D layered organohalide tin perovskites journal June 2017
Bluish-white-light-emitting diodes based on two-dimensional lead halide perovskite (C 6 H 5 C 2 H 4 NH 3 ) 2 PbCl 2 Br 2 journal April 2018
Electric and magnetic transitions with 90° turning of polarizations in a layered perovskite of [NH 4 Cl] 2 [Ni(HCOO) 2 (NH 3 ) 2 ] journal November 2018
Cystamine-configured lead halide based 2D hybrid molecular crystals: Synthesis and photoluminescence systematics journal November 2018
Efficient charge separation at multiple quantum well perovskite/PCBM interface journal July 2018
Structure-controlled optical thermoresponse in Ruddlesden-Popper layered perovskites journal November 2018
Research Update: Tricritical point and large caloric effect in a hybrid organic-inorganic perovskite journal October 2018
Preface: Two dimensional (2D) hybrid organic-inorganic perovskites journal November 2018
Structure and binding in halide perovskites: Analysis of static and dynamic effects from dispersion-corrected density functional theory journal February 2019
Photophysics of lead-free tin halide perovskite films and solar cells journal August 2019
Solvent-free synthesis of organometallic halides CH 3 NH 3 PbI 3 and (CH 3 NH 3 ) 3 Bi 2 I 9 and their thermoelectric transport properties journal August 2019
Structural and thermodynamic limits of layer thickness in 2D halide perovskites journal December 2018
Research progress on organic–inorganic halide perovskite materials and solar cells journal February 2018
The 2019 materials by design roadmap journal October 2018
Promise of commercialization: Carbon materials for low-cost perovskite solar cells journal January 2018
Hydrogen-bonded and supramolecular ferroelectricity in a new hybrid (C 12 H 25 NH 3 ) 2 CoCl 4 journal November 2018
Effect of CH 3 NH 3 I vapour evaporation temperature on the quality of the lead-free bismuth based perovskites thin-films journal March 2019
Temperature-dependent photoluminescence of cesium lead halide perovskite (CsPbX 3 , X = Br, Cl, I) quantum dots journal September 2019
Stable biexcitons in two-dimensional metal-halide perovskites with strong dynamic lattice disorder journal March 2018
Exciton-polaron spectral structures in two-dimensional hybrid lead-halide perovskites journal June 2018
Lifetime-shortened acoustic phonons and static order at the Brillouin zone boundary in the organic-inorganic perovskite CH 3 NH 3 PbCl 3 journal December 2018
Common acoustic phonon lifetimes in inorganic and hybrid lead halide perovskites journal September 2019
Decoupled molecular and inorganic framework dynamics in CH 3 NH 3 PbCl 3 journal December 2019
Low-dimensional bismuth(III) iodide hybrid material with high activity for the fast removal of rhodamine B journal November 2018
Confining metal-halide perovskites in nanoporous thin films journal August 2017
Enhanced photovoltaic performance and stability with a new type of hollow 3D perovskite {en}FASnI 3 journal August 2017
Two-dimensional hybrid perovskites sustaining strong polariton interactions at room temperature journal May 2019
Spin-dependent charge transport through 2D chiral hybrid lead-iodide perovskites journal December 2019
Structural and spectral dynamics of single-crystalline Ruddlesden-Popper phase halide perovskite blue light-emitting diodes journal January 2020
Properties and potential optoelectronic applications of lead halide perovskite nanocrystals journal November 2017
Metal-free three-dimensional perovskite ferroelectrics journal July 2018
Stimuli-triggered reversible switching mechanism between H- and J-type supramolecular assemblies of cationic porphyrins adsorbed on tungsten(VI) oxide surface journal August 2018
Supramolecular concepts and approaches in corrosion and biofouling prevention journal June 2019
Emerging 2D materials for room-temperature polaritonics journal July 2019
Crystal structure of trimethylsulfoxonium tetrachloridocobaltate(II) [(CH 3 ) 3 SO] 2 CoCl 4 journal March 2020
First representatives of (210)-oriented perovskite variants−Synthesis, crystal structures and properties of the new 2D hybrid perovskites A[HC(NH2)2]PbI4; A=[C(NH2)3], [HSC(NH2)2] journal July 2018
Synthetic control over orientational degeneracy of spacer cations enhances solar cell efficiency in two-dimensional perovskites text January 2019
Tunable Semiconductors: Control over Carrier States and Excitations in Layered Hybrid Organic-Inorganic Perovskites text January 2018
Emergence of Nanoplatelet Light-Emitting Diodes journal August 2018
Lead-free hybrid perovskites for photovoltaics journal January 2018
Single crystals of caesium formamidinium lead halide perovskites: solution growth and gamma dosimetry text January 2017
Exciton-polaron spectral structures in two dimensional hybrid lead-halide perovskites text January 2018
Charge transfer tuning in TiO2 hybrid nanostructures with acceptor-acceptor systems text January 2018
Absolute energy level positions in tin and lead based halide perovskites text January 2019
Engineering Multiphase Metal Halide Perovskites Thin Films for Stable and Efficient Solar Cells text January 2020

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