In search of θ-(Pu,Zr) in binary Pu–Zr: Thermal and microstructural analyses of Pu − 30Zr alloy

Aitkaliyeva, Assel; Adkins, Cynthia A.; McKinney, Casey; Hirschhorn, Jacob; Tonks, Michael R.

doi:10.1016/j.jnucmat.2019.151875

Title: In search of θ-(Pu,Zr) in binary Pu–Zr: Thermal and microstructural analyses of Pu − 30Zr alloy

Authors:: Aitkaliyeva, Assel; Adkins, Cynthia A.; McKinney, Casey; Hirschhorn, Jacob; Tonks, Michael R.

Publication Date:: Wed Jan 01 00:00:00 EST 2020

Sponsoring Org.:: USDOE

OSTI Identifier:: 1580287

Resource Type:: Publisher's Accepted Manuscript

Journal Name:: Journal of Nuclear Materials

Additional Journal Information:: Journal Name: Journal of Nuclear Materials Journal Volume: 528 Journal Issue: C; Journal ID: ISSN 0022-3115

Publisher:: Elsevier

Country of Publication:: Netherlands

Language:: English

Citation Formats


                    Aitkaliyeva, Assel, Adkins, Cynthia A., McKinney, Casey, Hirschhorn, Jacob, and Tonks, Michael R. In search of θ-(Pu,Zr) in binary Pu–Zr: Thermal and microstructural analyses of Pu − 30Zr alloy.  Netherlands: N. p., 2020. 
Web.  doi:10.1016/j.jnucmat.2019.151875.

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                    Aitkaliyeva, Assel, Adkins, Cynthia A., McKinney, Casey, Hirschhorn, Jacob, & Tonks, Michael R. In search of θ-(Pu,Zr) in binary Pu–Zr: Thermal and microstructural analyses of Pu − 30Zr alloy.  Netherlands.  https://doi.org/10.1016/j.jnucmat.2019.151875

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                    Aitkaliyeva, Assel, Adkins, Cynthia A., McKinney, Casey, Hirschhorn, Jacob, and Tonks, Michael R. Wed .  
"In search of θ-(Pu,Zr) in binary Pu–Zr: Thermal and microstructural analyses of Pu − 30Zr alloy".  Netherlands.  https://doi.org/10.1016/j.jnucmat.2019.151875.

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@article{osti_1580287,

  title        = {In search of θ-(Pu,Zr) in binary Pu–Zr: Thermal and microstructural analyses of Pu − 30Zr alloy},

  author       = {Aitkaliyeva, Assel and Adkins, Cynthia A. and McKinney, Casey and Hirschhorn, Jacob and Tonks, Michael R.},

  abstractNote = {},

  doi          = {10.1016/j.jnucmat.2019.151875},

  journal      = {Journal of Nuclear Materials},

  number       = C,

  volume       = 528,

  place        = {Netherlands},

  year         = {Wed Jan 01 00:00:00 EST 2020},

  month        = {Wed Jan 01 00:00:00 EST 2020}

}

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Works referenced in this record:

The crystal structure of ζ-Pu–Zr, ideal formula Pu ₂₈ Zr
journal, January 1979

Cromer, D. T.
Acta Crystallographica Section B Structural Crystallography and Crystal Chemistry, Vol. 35, Issue 1
DOI: 10.1107/S0567740879002430

The plutonium-zirconium phase diagram
journal, October 1960

Marples, J. A. C.
Journal of the Less Common Metals, Vol. 2, Issue 5
DOI: 10.1016/0022-5088(60)90042-4

The lattice parameters of some δ- and ϵ-plutonium alloys
journal, June 1964

Marples, J. A. C.
Journal of Physics and Chemistry of Solids, Vol. 25, Issue 6
DOI: 10.1016/0022-3697(64)90140-4

The plutonium-zirconium equilibrium diagram from 0 to 10 at% Zr
journal, April 1969

Taylor, J. M.
Journal of Nuclear Materials, Vol. 30, Issue 3
DOI: 10.1016/0022-3115(69)90253-0

Experimentally Known Properties of U-10Zr Alloys: A Critical Review
journal, April 2018

Janney, Dawn E.; Hayes, Steven L.
Nuclear Technology, Vol. 203, Issue 2
DOI: 10.1080/00295450.2018.1435137

Microstructural characterization of the as-cast and annealed Pu-10Zr alloy
journal, September 2019

Aitkaliyeva, Assel; Adkins, Cynthia A.; Hirschhorn, Jacob
Journal of Nuclear Materials, Vol. 523
DOI: 10.1016/j.jnucmat.2019.05.051

Phase diagram of the PuZr system in the Zr-rich region
journal, April 1992

Suzuki, Yasufumi; Maeda, Atsushi; Ohmichi, Toshihiko
Journal of Alloys and Compounds, Vol. 182, Issue 2
DOI: 10.1016/0925-8388(92)90590-6

Pu-Zr (plutonium-zirconium)
journal, June 1995

Okamoto, H.
Journal of Phase Equilibria, Vol. 16, Issue 3
DOI: 10.1007/BF02667321

Analysis of constituent redistribution in the γ (bcc) U–Pu–Zr alloys under gradients of temperature and concentrations
journal, June 2000

Sohn, Y. H.; Dayananda, M. A.; Hofman, G. L.
Journal of Nuclear Materials, Vol. 279, Issue 2-3
DOI: 10.1016/S0022-3115(99)00290-1

X-ray Spectrometric Analysis of Plutonium-Zirconium Alloys
journal, March 1975

Walden, J. C.; Wallace, P. L.; Magana, J. W.
Applied Spectroscopy, Vol. 29, Issue 2
DOI: 10.1366/000370275774455338

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Similar Records

Title: In search of θ-(Pu,Zr) in binary Pu–Zr: Thermal and microstructural analyses of Pu − 30Zr alloy

Citation Formats

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Title: In search of θ-(Pu,Zr) in binary Pu–Zr: Thermal and microstructural analyses of Pu − 30Zr alloy

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journal, October 1960

The lattice parameters of some δ- and ϵ-plutonium alloys
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Analysis of constituent redistribution in the γ (bcc) U–Pu–Zr alloys under gradients of temperature and concentrations
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X-ray Spectrometric Analysis of Plutonium-Zirconium Alloys
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