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Title: Critical behavior in Ni2MnGa and Ni2Mn0.85Cu0.15Ga

Abstract

The critical behaviors of polycrystalline Ni2MnGa and Ni2Mn0.85Cu0.15Ga have been examined through high-resolution bulk magnetization measurements. The critical exponents, β and γ, were derived from modified Arrott plots using the Kouvel-Fisher method. The values of the extracted critical exponents satisfied the scaling equation of state and associated exponent relations, indicating self-consistency of the extracted values. In Ni2MnGa, the critical exponents (β = 0.401 ± 0.003, γ = 1.27 ± 0.02) indicate a deviation from the 3D-Heisenberg values toward the mean-field values, likely due to the presence of long-range Ruderman-Kittel-Kasuya-Yosida interactions. However, the critical exponents of Ni2Mn0.85Cu0.15Ga (β = 0.389 ± 0.004, γ =1.39 ± 0.02) are closer to the 3D-Heisenberg values. This indicates a weakening of the long-range exchange interactions due to the substitution of Cu in the Mn site.

Authors:
 [1];  [1];  [1];  [2];  [2];  [1]
  1. Louisiana State Univ., Baton Rouge, LA (United States)
  2. Southern Illinois Univ., Carbondale, IL (United States)
Publication Date:
Research Org.:
Southern Illinois Univ., Carbondale, IL (United States); Louisiana State Univ., Baton Rouge, LA (United States)
Sponsoring Org.:
USDOE Office of Science (SC)
OSTI Identifier:
1540183
Alternate Identifier(s):
OSTI ID: 1439397; OSTI ID: 1872884
Grant/Contract Number:  
FG02-06ER46291; SC0010521; FG02-13ER46946
Resource Type:
Accepted Manuscript
Journal Name:
Journal of Applied Physics
Additional Journal Information:
Journal Volume: 123; Journal Issue: 20; Journal ID: ISSN 0021-8979
Publisher:
American Institute of Physics (AIP)
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE; Physics; Alloys; Entropy; Heisenberg model; Exchange interactions; Polycrystalline material; Statistical mechanics; Ferromagnetism; Phase transitions; Magnetic ordering; 32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATION; magnetocaloric materials; phase transitions

Citation Formats

Saleheen, Ahmad Us, Chen, Jing-Han, Young, David P., Dubenko, Igor, Ali, Naushad, and Stadler, Shane. Critical behavior in Ni2MnGa and Ni2Mn0.85Cu0.15Ga. United States: N. p., 2018. Web. doi:10.1063/1.5025196.
Saleheen, Ahmad Us, Chen, Jing-Han, Young, David P., Dubenko, Igor, Ali, Naushad, & Stadler, Shane. Critical behavior in Ni2MnGa and Ni2Mn0.85Cu0.15Ga. United States. https://doi.org/10.1063/1.5025196
Saleheen, Ahmad Us, Chen, Jing-Han, Young, David P., Dubenko, Igor, Ali, Naushad, and Stadler, Shane. Tue . "Critical behavior in Ni2MnGa and Ni2Mn0.85Cu0.15Ga". United States. https://doi.org/10.1063/1.5025196. https://www.osti.gov/servlets/purl/1540183.
@article{osti_1540183,
title = {Critical behavior in Ni2MnGa and Ni2Mn0.85Cu0.15Ga},
author = {Saleheen, Ahmad Us and Chen, Jing-Han and Young, David P. and Dubenko, Igor and Ali, Naushad and Stadler, Shane},
abstractNote = {The critical behaviors of polycrystalline Ni2MnGa and Ni2Mn0.85Cu0.15Ga have been examined through high-resolution bulk magnetization measurements. The critical exponents, β and γ, were derived from modified Arrott plots using the Kouvel-Fisher method. The values of the extracted critical exponents satisfied the scaling equation of state and associated exponent relations, indicating self-consistency of the extracted values. In Ni2MnGa, the critical exponents (β = 0.401 ± 0.003, γ = 1.27 ± 0.02) indicate a deviation from the 3D-Heisenberg values toward the mean-field values, likely due to the presence of long-range Ruderman-Kittel-Kasuya-Yosida interactions. However, the critical exponents of Ni2Mn0.85Cu0.15Ga (β = 0.389 ± 0.004, γ =1.39 ± 0.02) are closer to the 3D-Heisenberg values. This indicates a weakening of the long-range exchange interactions due to the substitution of Cu in the Mn site.},
doi = {10.1063/1.5025196},
journal = {Journal of Applied Physics},
number = 20,
volume = 123,
place = {United States},
year = {Tue May 29 00:00:00 EDT 2018},
month = {Tue May 29 00:00:00 EDT 2018}
}

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